In this thesis, I report on experiments with cold 85Rb atoms in a far-detuned one-dimensional optical lattice. These experiments are focused on creating efficient coupling between the quantized vibrational states of atoms in the optical lattice, on controlling and maintaining coherence between the vibrational states, and on developing a spectroscopy method to characterize the decay of coherence. First, I present an experimental study of the application of simple and compound pulses consisting of time-dependent spatial translations to coupling vibrational states of ultracold 85Rb atoms in the optical\nlattice. Experimental results show that a square pulse consisting of lattice displacements and a delay is more efficient than single-step and Gaussian pulses. The square pulse can be seen as an example of coherent control. Numerical calculations are in strong agreement with the experimental results. In addition, it is shown numerically that the vibrational state coupling due to such lattice manipulations is more efficient in shallow lattices than in deep lattices, in which the coupling probability approaches the harmonic\noscillator limit. Next, the effectiveness of these pulses in reviving oscillations of atoms in vibrational superposition states using a pulse-echo technique is examined. Experimental results show that the square and Gaussian pulses result in higher echo amplitudes than the single-step pulse. These echo amplitudes are an order of magnitude larger than the echo amplitudes observed previously for the motional states of atoms in optical lattices.\nWith the aim of the optimized square echo pulse, echo amplitude is measured at much\nlonger times, where a surprising coherence freeze (plateau) is observed. To investigate \nmechanisms responsible for the observed echo decay and the coherence freeze, we developed\na new two-dimensional pump-probe spectroscopy technique to monitor the evolution of frequency-frequency correlations in the system, a necessary input for understanding the decay of coherence. Through this 2D technique, we have characterized the temporal decay of frequency memory and through our simulations we find that coherence freeze is related to the shape of this memory loss function. This technique is general in that it can be applied in a variety of quantum information candidate systems to probe the nature of their decoherence.
In this thesis, I report on experiments with cold 85Rb atoms in a far-detuned one-dimensional optical lattice. These experiments are focused on creating efficient coupling between the quantized vibrational states of atoms in the optical lattice, on controlling and maintaining coherence between the vibrational states, and on developing a spectroscopy method to characterize the decay of coherence. First, I present an experimental study of the application of simple and compound pulses consisting of time-dependent spatial translations to coupling vibrational states of ultracold 85Rb atoms in the optical\nlattice. Experimental results show that a square pulse consisting of lattice displacements and a delay is more efficient than single-step and Gaussian pulses. The square pulse can be seen as an example of coherent control. Numerical calculations are in strong agreement with the experimental results. In addition, it is shown numerically that the vibrational state coupling due to such lattice manipulations is more efficient in shallow lattices than in deep lattices, in which the coupling probability approaches the harmonic\noscillator limit. Next, the effectiveness of these pulses in reviving oscillations of atoms in vibrational superposition states using a pulse-echo technique is examined. Experimental results show that the square and Gaussian pulses result in higher echo amplitudes than the single-step pulse. These echo amplitudes are an order of magnitude larger than the echo amplitudes observed previously for the motional states of atoms in optical lattices.\nWith the aim of the optimized square echo pulse, echo amplitude is measured at much\nlonger times, where a surprising coherence freeze (plateau) is observed. To investigate \nmechanisms responsible for the observed echo decay and the coherence freeze, we developed\na new two-dimensional pump-probe spectroscopy technique to monitor the evolution of frequency-frequency correlations in the system, a necessary input for understanding the decay of coherence. Through this 2D technique, we have characterized the temporal decay of frequency memory and through our simulations we find that coherence freeze is related to the shape of this memory loss function. This technique is general in that it can be applied in a variety of quantum information candidate systems to probe the nature of their decoherence.
We measure the application of simple and compound pulses consisting of time-dependent spatial translations to coupling vibrational states of ultracold 85Rb atoms in a far-detuned 1D optical lattice. The lattice wells are so shallow as to support only two bound states, and we prepare the atoms in the ground state. The lattice is oriented vertically, leading to a tilted-washboard potential analogous to those encountered in condensed-matter systems. Experimentally, we find that a square pulse consisting of lattice displacements and a delay is more efficient than single-step pulses or Gaussian pulses. This is described as an example of coherent control. It is striking that contrary to the intuition that soft pulses minimize loss, the Gaussian pulse is outperformed by the square pulse. Numerical calculations are in strong agreement with our experimental results and show the superiority of the square pulse to the single-step pulse for all lattice depths and to the Gaussian pulse for lattice depths greater than seven lattice recoil energies. We also compare the effectiveness of these pulses for reviving oscillations of atoms in vibrational superposition states using the pulse-echo technique. We find that the square and Gaussian pulses result in higher echo amplitudes than the single-step pulse. These improved echo pulses allow us to probe coherence at longer times than in the past, measuring a plateau which has yet to be explained. In addition, we show numerically that the vibrational state coupling due to such lattice manipulations is more efficient in shallow lattices than in deep lattices. The coupling probability for an optimized single-step pulse approaches 1/e as the depth goes to infinity (harmonic-oscillator limit), while in shallow lattices with large anharmonicity, the coupling probability reaches a maximum value of 0.51 for a lattice depth of five recoil energies. For square and Gaussian pulses the coupling in the lattice is even stronger, reaching maxima of 0.64 at 6 recoil energies and 0.67 at 5 recoil energies, respectively.
Summary form only given. The investigation of coherent superposition states for atoms interacting with external potentials allows a completely new class of experiments directed towards coherent trapping and guiding of neutral atoms. In addition, the process of decoherence, i.e., the collapse of superposition states, is one of the basic concepts for our understanding of the connection between classical and quantum physics. We study the creation and decay of superpositions of different components of the center-of-mass wavefunction of rubidium atoms in a one-dimensional near-resonant optical lattice. This makes it possible to gain insight into the dependence of decoherence processes on the coupling of the atoms to the light field. We discuss the dependence of the wave packet oscillations and echoes on experimental parameters (potential depth, light intensity and detuning, time delay, size of the shift, etc.). We compare our experimental results with numerical simulations of the echo effect. The observation of this new effect in the coherent wave packet motion of atoms trapped in optical potentials will allow us to selectively study the decoherence process and measure the decoherence time in regimes where this was previously impossible.
Optical lattices induced by light detuned far from the frequency of any atomic resonance transition are ideal systems in which to develop techniques for the coherent control of atomic motional and internal states. Decoherence arising from spontaneous emission can be eliminated to an arbitrary degree by varying the detuning of the optical field. The atoms trapped in these lattices are to a large extent isolated from environmental disturbances and from each other. The first step towards the coherent control of atoms in a far-detuned lattice is their preparation in a single motional state. In this thesis the preparation of atoms in the ground vibrational state of a two-dimensional far-detuned optical lattice via resolved-sideband Raman cooling is presented. This sideband-cooling scheme involves stimulated Raman transitions between bound vibrational states of a pair of magnetic ground state sublevels, followed by an irreversible step due to optical pumping, resulting in a net loss of one quantum of vibrational energy per cooling cycle. This process provides efficient cooling in two-dimensions and leads to the accumulation of a large fraction of atoms in the 2-D ground vibrational state of a potential well associated with a single Zeeman substate. Experiments aimed at improving and monitoring the characteristics of the lar-detuned lattice and the sideband-Raman cooling efficiency are also described. Parametric excitation experiments and modelling are employed to investigate the degree of anharmonicity of the optical potential and the importance of heating induced by laser intensity noise, whilst Zeeman-state analysis of the sample is performed for monitoring the distribution of atoms over different magnetic sub- states. Finally, spin-polarization experiments are carried out in order to study the paramagnetic properties of the lattice and lead to an evaluation of a spin-temperature for the sample.
The effects of reversing the sinusoidal potential every q kick periods with q = 0, l, 2,3 are examined numerically with the q = 0, 1, 2 cases being verified experimentally. I have found that when considering the energy absorption of the system the q = 1 case is qualitatively and quantitatively the same as the standard kicked rotor, while the q = 2 case is qualitatively the same as the standard kicked rotor with an effective increase in the scaled dimensionless kick strength parameter, k, of k rarr; k+ p2 .In this thesis I detail the background, implementation and results of two experiments from relatively different fields of study, both of which involve ultra-cold Rubidium atoms trapped in an optical lattice. The first is an analysis of the superpositions of vibrational states of the lattice. This includes a characterization and modelling of the dephasing of the states, an effect inherent to the lattice. It is found that the lattice geometry is a primary factor in the observed dephasing. This geometry results in position-dependent energy eigenstates in the lattice. Modelling this distribution of energies allows the accurate prediction of several experimental observables and provides useful information for future experiments. Several methods of applying pulse echoes to recover the state in the face of this dephasing are demonstrated, characterized and successfully modelled. The second set of experiments centre around using the optical lattice and Rubidium atoms as a delta-kicked rotor system. First I examine quantum resonances in the delta-kicked rotor. These are characterized by a dramatically increased energy absorption rate, in stark contrast to the momentum localization generally observed. These resonances exist when the effective Planck's constant, a parameter that determines how quantum-mechanically the system behaves, has a value of plank; d5;=rs dot;4p, for integers r and s. However only for plank; d5;=r dot;2p are resonances easily observable. Here I report on the first observation of high-order quantum resonances in a non-condensed atomic sample at values of plank; d5;=r16 dot;4p for integers r = 2--6. Quantum numerical simulations suggest that this observation of high-order resonances indicates a much longer spatial coherence than expected from an initially thermal atomic sample.
In the past fifteen years ultracold atoms confined to optical lattices, which are artificial crystals of light, have proven to be powerful tools in the study of strongly correlated many-body systems widely known from a condensed matter context. The detailed knowledge, high tunability and control of microscopic parameters has enabled the creation and control of highly non-trivial quantum systems for which a direct comparison of model calculations to experimental measurements is now possible. In order to gain precise information on the properties of ultracold gases in optical lattices, many powerful methods have been developed. In particular spectroscopic methods have enabled to probe different characteristic excitations. However, many fascinating properties of strongly interacting quantum many-body systems are not yet fully characterized. Therefore, this thesis explores further possibilities of lattice modulation spectroscopy which is a time-periodic modulation of the optical lattice amplitude. We theoretically investigate the response of different (mostly one-dimensional) cold atom systems to a lattice modulation by means of the time-dependent density matrix renormalization group method and different analytical approximations. In addition to the normal lattice modulation, we consider a superlattice modulation scheme where the lattice amplitude is modulated in a dimerized fashion, coupling to a certain class of excitations in the system. The lattice modulation spectroscopy is a versatile probe which we use to study different situations relevant for experimental applications. We show that a detection of signatures of the exotic bond order wave phase is feasible in a system of interacting fermions on a one-dimensional optical lattice with staggered energy offset. Moreover, we demonstrate that a temperature measurement of fermions confined to an optical lattice is possible as well as a determination of the interaction strength of bosonic atoms confined to a one-dimensional optical lattice. In addition, various excitations in all these systems are investigated in detail.
In this thesis, I present an experimental study of quantum control techniques for transferring population between vibrational states of atoms trapped in an optical lattice. Results from a range of techniques are compared, including techniques tested previously in the same system. In the study of the Adiabatic Rapid Passage (ARP) technique, control of population transfer is realized through varying the chirp rate and modulation amplitude of a frequency-chirped sinusoidal displacement of the lattice. Meanwhile, dependence of population transfer on the chirp direction is observed, which is explained by a model of ARP in a 3-level system. In the study of the coherent control technique, interference between a one-phonon transition at 2\omega and a two-phonon transition at omega is experimentally demonstrated. The omega and 2\omega transitions are realized by sinusoidally displacing the optical lattice at omega and sinusoidally modulating the lattice depth at 2\omega, respectively. The branching ratio of transitions to the first excited state and to higher excited states is controlled by varying the relative phase between these two pathways. The highest measured branching ratio of 17\pm2 is achieved among all the experiments using this coherent control scheme. In the study of the GRadient Ascent Pulse Engineering (GRAPE) technique, a "pulse" involving both displacement and depth-modulation of the lattice is used to transfer population. This pulse is theoretically engineered with the GRAPE algorithm to optimize the fidelity between the first excited state and the final state, when the lattice Hamiltonian without gravity for a specific lattice depth is considered. The experimental result shows that there is almost no excitation into higher excited states during population transfer from the ground to the first excited state, even when this process is affected by gravity and inhomogeneous broadening in reality. By comparing all the techniques, the GRAPE technique is found to be the best in terms of increasing population transfer into the first excited state while reducing excitation into higher excited states. On the other hand, the ARP technique creates the highest normalized population inversion, a ratio of the difference to the sum of the ground and the first excited state populations.