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arXiv:1005.2635 · Physical Review Letters

Coherence Freeze in an Optical Lattice Investigated Via Pump-Probe Spectroscopy

Samansa Maneshi, Chao Zhuang, Christopher R. Paul, Luciano Soares da Cruz, Aephraim M. Steinberg

Published Nov 4, 2010• 6 citations
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Abstract

Motivated by our observation of fast echo decay and a surprising coherence freeze, we have developed a pump-probe spectroscopy technique for vibrational states of 85Rb atoms in an optical lattice to gain information about the memory dynamics of the system. We monitor the time-dependent changes of frequencies experienced by atoms and characterize the probability distribution of these frequency trajectories. We show that the inferred distribution, unlike a naive microscopic model of the lattice, correctly predicts the main features of the observed echo decay.

DOI
10.1103/physrevlett.105.193001

Related papers

Investigation of Coherence and its Decay Mechanisms in an Optical Lattice

Samansa Maneshi

In this thesis, I report on experiments with cold 85Rb atoms in a far-detuned one-dimensional optical lattice. These experiments are focused on creating efficient coupling between the quantized vibrational states of atoms in the optical lattice, on controlling and maintaining coherence between the vibrational states, and on developing a spectroscopy method to characterize the decay of coherence. First, I present an experimental study of the application of simple and compound pulses consisting of time-dependent spatial translations to coupling vibrational states of ultracold 85Rb atoms in the optical\nlattice. Experimental results show that a square pulse consisting of lattice displacements and a delay is more efficient than single-step and Gaussian pulses. The square pulse can be seen as an example of coherent control. Numerical calculations are in strong agreement with the experimental results. In addition, it is shown numerically that the vibrational state coupling due to such lattice manipulations is more efficient in shallow lattices than in deep lattices, in which the coupling probability approaches the harmonic\noscillator limit. Next, the effectiveness of these pulses in reviving oscillations of atoms in vibrational superposition states using a pulse-echo technique is examined. Experimental results show that the square and Gaussian pulses result in higher echo amplitudes than the single-step pulse. These echo amplitudes are an order of magnitude larger than the echo amplitudes observed previously for the motional states of atoms in optical lattices.\nWith the aim of the optimized square echo pulse, echo amplitude is measured at much\nlonger times, where a surprising coherence freeze (plateau) is observed. To investigate \nmechanisms responsible for the observed echo decay and the coherence freeze, we developed\na new two-dimensional pump-probe spectroscopy technique to monitor the evolution of frequency-frequency correlations in the system, a necessary input for understanding the decay of coherence. Through this 2D technique, we have characterized the temporal decay of frequency memory and through our simulations we find that coherence freeze is related to the shape of this memory loss function. This technique is general in that it can be applied in a variety of quantum information candidate systems to probe the nature of their decoherence.

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Photon echoes of polyatomic molecules in condensed phases

Yi Jing Yan, Shaul Mukamel

A theory of optical echo spectroscopies of large polyatomic molecules in condensed phases is developed. Using phase space correlation functions, we examine the interrelationships among the following optical measurements: ordinary photon echo, stimulated photon echo, accumulated photon echo, incoherent accumulated photon echo, and pump–probe absorption. Conditions for the elimination of inhomogeneous broadening in these experiments are specified. A multimode Brownian oscillator model is used to account for high frequency molecular vibrations, as well as solvent modes, and electronic dephasing processes. The effects of quantum beats, spectral diffusion, and homogeneous dephasing on the echo signals are studied and compared in detail with pump–probe and hole burning spectroscopy.

The Journal of Chemical Physics•Jan 1, 1991•172 citations
Motivated by our observation of fast echo decay and a surprising coherence freeze, we have developed a pump-probe spectroscopy technique for vibrational states of 85Rb atoms in an optical lattice to gain information about the memory dynamics of the system. We monitor the time-dependent changes of frequencies experienced by atoms and characterize the probability distribution of these frequency trajectories. We show that the inferred distribution, unlike a naive microscopic model of the lattice, correctly predicts the main features of the observed echo decay.
In this thesis, I report on experiments with cold 85Rb atoms in a far-detuned one-dimensional optical lattice. These experiments are focused on creating efficient coupling between the quantized vibrational states of atoms in the optical lattice, on controlling and maintaining coherence between the vibrational states, and on developing a spectroscopy method to characterize the decay of coherence. First, I present an experimental study of the application of simple and compound pulses consisting of time-dependent spatial translations to coupling vibrational states of ultracold 85Rb atoms in the optical\nlattice. Experimental results show that a square pulse consisting of lattice displacements and a delay is more efficient than single-step and Gaussian pulses. The square pulse can be seen as an example of coherent control. Numerical calculations are in strong agreement with the experimental results. In addition, it is shown numerically that the vibrational state coupling due to such lattice manipulations is more efficient in shallow lattices than in deep lattices, in which the coupling probability approaches the harmonic\noscillator limit. Next, the effectiveness of these pulses in reviving oscillations of atoms in vibrational superposition states using a pulse-echo technique is examined. Experimental results show that the square and Gaussian pulses result in higher echo amplitudes than the single-step pulse. These echo amplitudes are an order of magnitude larger than the echo amplitudes observed previously for the motional states of atoms in optical lattices.\nWith the aim of the optimized square echo pulse, echo amplitude is measured at much\nlonger times, where a surprising coherence freeze (plateau) is observed. To investigate \nmechanisms responsible for the observed echo decay and the coherence freeze, we developed\na new two-dimensional pump-probe spectroscopy technique to monitor the evolution of frequency-frequency correlations in the system, a necessary input for understanding the decay of coherence. Through this 2D technique, we have characterized the temporal decay of frequency memory and through our simulations we find that coherence freeze is related to the shape of this memory loss function. This technique is general in that it can be applied in a variety of quantum information candidate systems to probe the nature of their decoherence.
We develop and study quantum and semiclassical models of Rydberg-atom spectroscopy in amplitude-modulated optical lattices. Both initial- and target-state Rydberg atoms are trapped in the lattice. Unlike in other spectroscopic schemes, the modulation-induced ponderomotive coupling between the Rydberg states is spatially periodic and perfectly phase-locked to the lattice trapping potentials. This leads to a type of sub-Doppler mechanism which we explain in detail. In our exact quantum model, we solve the time-dependent Schr\"odinger equation in the product space of center-of-mass (COM) momentum states and the internal-state space. We also develop a perturbative model based on the band structure in the lattice and Fermi's golden rule, as well as a semiclassical trajectory model in which the COM is treated classically and the internal-state dynamics quantum-mechanically. In all models we obtain the spectrum of the target Rydberg-state population versus the lattice modulation frequency, averaged over the initial thermal COM momentum distribution of the atoms. We investigate the quantum-classical correspondence of the problem in several parameter regimes and exhibit spectral features that arise from vibrational COM coherences and rotary-echo effects. Applications in Rydberg-atom spectroscopy are discussed.
Pump-probe spectroscopy is the most common time-resolved technique for investigation of electronic dynamics, and the results provide the incoherent population decay time T1{T}_{1}T1​. Here we use a modified pump-probe experiment to investigate coherent dynamics, and we demonstrate this with a measurement of the inhomogeneous dephasing time T2∗{T}_{2}^{*}T2∗​ for phosphorus impurities in silicon. The pulse sequence produces the same information as previous coherent all-optical (photon-echo-based) techniques but is simpler. The probe signal strength is first order in the pulse area but its effect on the target state is only second order, meaning that it does not demolish the quantum information. We propose simple extensions to the technique to measure the homogeneous dephasing time T2{T}_{2}T2​, or to perform tomography of the target qubit.
Summary form only given. The investigation of coherent superposition states for atoms interacting with external potentials allows a completely new class of experiments directed towards coherent trapping and guiding of neutral atoms. In addition, the process of decoherence, i.e., the collapse of superposition states, is one of the basic concepts for our understanding of the connection between classical and quantum physics. We study the creation and decay of superpositions of different components of the center-of-mass wavefunction of rubidium atoms in a one-dimensional near-resonant optical lattice. This makes it possible to gain insight into the dependence of decoherence processes on the coupling of the atoms to the light field. We discuss the dependence of the wave packet oscillations and echoes on experimental parameters (potential depth, light intensity and detuning, time delay, size of the shift, etc.). We compare our experimental results with numerical simulations of the echo effect. The observation of this new effect in the coherent wave packet motion of atoms trapped in optical potentials will allow us to selectively study the decoherence process and measure the decoherence time in regimes where this was previously impossible.
The linear Faraday effect is used to implement a continuous measurement of the spin of a sample of laser-cooled atoms trapped in an optical lattice. One of the optical lattice beams serves also as a probe beam, thereby allowing one to monitor the atomic dynamics in real time and with minimal perturbation. A simple theory is developed to predict the measurement sensitivity and associated cost in terms of decoherence caused by the scattering of probe photons. Calculated signal-to-noise ratios in measurements of Larmor precession are found to agree with experimental data for a wide range of lattice intensity and detuning. Finally, quantum back-action is estimated by comparing the measurement sensitivity to spin projection noise, and shown to be insignificant in the current experiment. A continuous quantum measurement based on Faraday spectroscopy in optical lattices may open up new possibilities for the study of quantum feedback and classically chaotic quantum systems.
A theory of optical echo spectroscopies of large polyatomic molecules in condensed phases is developed. Using phase space correlation functions, we examine the interrelationships among the following optical measurements: ordinary photon echo, stimulated photon echo, accumulated photon echo, incoherent accumulated photon echo, and pump–probe absorption. Conditions for the elimination of inhomogeneous broadening in these experiments are specified. A multimode Brownian oscillator model is used to account for high frequency molecular vibrations, as well as solvent modes, and electronic dephasing processes. The effects of quantum beats, spectral diffusion, and homogeneous dephasing on the echo signals are studied and compared in detail with pump–probe and hole burning spectroscopy.