New effects can arise in quantum physics when there is strong coupling, either between atoms and light or between different quantum systems. This thesis examines an optical nanofiber atom trap as a mediator of atom-light interactions and a potential element of a hybrid quantum system. The evanescent field around the sub-wavelength waist of an optical nanofiber possesses a small mode area that increases the cooperativity between atoms and the mode, in a manner analogous to traditional cavity QED. We demonstrate trapping of
87Rb atoms with an optical nanofiber, confining hundreds of atoms with typical trap lifetimes of tens of milliseconds. We then employ single photon counting techniques to study untrapped ensembles of cold atoms around the nanofiber. A first experiment uses intensity autocorrelations of resonance fluorescence emitted into the nanofiber mode to observe a transition from classical to nonclassical photon statistics. Measuring the correlations on longer timescales reveals the motion of atoms through the optical mode, and we develop a correspondence between the transit time and atomic cloud temperature. A second experiment measures Purcell enhancement of spontaneous emission of atoms near the nanofiber by correlating their fluorescence with a known trigger event. The spontaneous decay rate of an atom near a dielectric is modified by the induced dipole and by a change in the modes of the vacuum electromagnetic field. Our observed enhancement of
6.5±0.9% over the free-space rate matches well with what one finds from mode simulations in our system.
We study the radiative decay of a cesium atom near a nanofiber in the presence of a weak magnetic field. We show that the direction of the magnetic field relative to the fiber axis plays an important role in deciding the radiative decay from the atom. We find that the decay rates for the different magnetic sublevels of the atom are spread in a wider range in the orthogonal configuration than those in the coaxial configuration. We also show that the cross decay coefficients depend substantially on the orientation of the magnetic field relative to the fiber axis.
The tight confinement of the evanescent light field around the waist of an optical nanofiber makes it a suitable tool for studying nonlinear optics in atomic media. Here, we use an optical nanofiber embedded in a cloud of laser-cooled
87Rb for near-infrared frequency up-conversion via a resonant two-photon process. Sub-nW powers of the two-photon radiation, at 780 and 776 nm, copropagate through the optical nanofiber and the generation of 420 nm photons is observed. A measurement of the Autler-Townes splitting provides a direct measurement of the Rabi frequency of the 780 nm transition. Through this method, dephasings of the system can be studied. In this work, the optical nanofiber is used as an excitation and detection tool simultaneously, and it highlights some of the advantages of using fully fibered systems for nonlinear optics with atoms.