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Bulletin of the American Physical Society

Quantum correlations of light from atoms trapped around an optical nanofiber

Jeffrey A. Grover, Pablo Solano, Jennifer E. Hoffman, J. Lee, Luis A. Orozco, S. L. Rolston

Published Jun 5, 2014• 0 citations
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New effects can arise in quantum physics when there is strong coupling, either between atoms and light or between different quantum systems. This thesis examines an optical nanofiber atom trap as a mediator of atom-light interactions and a potential element of a hybrid quantum system. The evanescent field around the sub-wavelength waist of an optical nanofiber possesses a small mode area that increases the cooperativity between atoms and the mode, in a manner analogous to traditional cavity QED. We demonstrate trapping of $^{87}$Rb atoms with an optical nanofiber, confining hundreds of atoms with typical trap lifetimes of tens of milliseconds. We then employ single photon counting techniques to study untrapped ensembles of cold atoms around the nanofiber. A first experiment uses intensity autocorrelations of resonance fluorescence emitted into the nanofiber mode to observe a transition from classical to nonclassical photon statistics. Measuring the correlations on longer timescales reveals the motion of atoms through the optical mode, and we develop a correspondence between the transit time and atomic cloud temperature. A second experiment measures Purcell enhancement of spontaneous emission of atoms near the nanofiber by correlating their fluorescence with a known trigger event. The spontaneous decay rate of an atom near a dielectric is modified by the induced dipole and by a change in the modes of the vacuum electromagnetic field. Our observed enhancement of $6.5\pm0.9\%$ over the free-space rate matches well with what one finds from mode simulations in our system.

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Integrating the scalability of individually addressable arrays of optical-tweezer-trapped single atoms with the efficient light-matter interface provided by nanophotonic waveguides has been a long-standing challenge in quantum technologies based on atoms and photons. Here we realize a quantum interface between photons guided in an optical nanofiber with a diameter of 310 nm and an array of on average 155 individually addressable atoms. Using a spatial light modulator and an objective lens with NA = 0.45, single cesium atoms are trapped in a one-dimensional array of 200 optical tweezer spots with micrometer-scale trap sizes on the nanofiber. Individual atoms are addressed by spatially scanning an excitation laser beam, focused to a spot size comparable to that of the traps through the same objective lens, along the nanofiber. We confirm the single-atom nature of the individual trapping sites through photon-correlation measurements of the guided fluorescence, observing strong photon antibunching with $g^{(2)}(0) \approx 0.26$. We measure trap lifetimes of a few hundred milliseconds, with a maximum value of 460 ms, at an atom-surface separation of 670 nm without active cooling, representing an order-of-magnitude improvement over previous nanofiber traps. This platform opens a new regime for atom-photon interfaces, paving the way for scalable distributed quantum computing and quantum networks, as well as for the exploration of collective radiative effects in waveguide QED with individually addressable atoms.

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New effects can arise in quantum physics when there is strong coupling, either between atoms and light or between different quantum systems. This thesis examines an optical nanofiber atom trap as a mediator of atom-light interactions and a potential element of a hybrid quantum system. The evanescent field around the sub-wavelength waist of an optical nanofiber possesses a small mode area that increases the cooperativity between atoms and the mode, in a manner analogous to traditional cavity QED. We demonstrate trapping of 87^{87}87Rb atoms with an optical nanofiber, confining hundreds of atoms with typical trap lifetimes of tens of milliseconds. We then employ single photon counting techniques to study untrapped ensembles of cold atoms around the nanofiber. A first experiment uses intensity autocorrelations of resonance fluorescence emitted into the nanofiber mode to observe a transition from classical to nonclassical photon statistics. Measuring the correlations on longer timescales reveals the motion of atoms through the optical mode, and we develop a correspondence between the transit time and atomic cloud temperature. A second experiment measures Purcell enhancement of spontaneous emission of atoms near the nanofiber by correlating their fluorescence with a known trigger event. The spontaneous decay rate of an atom near a dielectric is modified by the induced dipole and by a change in the modes of the vacuum electromagnetic field. Our observed enhancement of 6.5±0.9%6.5\pm0.9\%6.5±0.9% over the free-space rate matches well with what one finds from mode simulations in our system.
Integrating the scalability of individually addressable arrays of optical-tweezer-trapped single atoms with the efficient light-matter interface provided by nanophotonic waveguides has been a long-standing challenge in quantum technologies based on atoms and photons. Here we realize a quantum interface between photons guided in an optical nanofiber with a diameter of 310 nm and an array of on average 155 individually addressable atoms. Using a spatial light modulator and an objective lens with NA = 0.45, single cesium atoms are trapped in a one-dimensional array of 200 optical tweezer spots with micrometer-scale trap sizes on the nanofiber. Individual atoms are addressed by spatially scanning an excitation laser beam, focused to a spot size comparable to that of the traps through the same objective lens, along the nanofiber. We confirm the single-atom nature of the individual trapping sites through photon-correlation measurements of the guided fluorescence, observing strong photon antibunching with g(2)(0)≈0.26g^{(2)}(0) \approx 0.26g(2)(0)≈0.26. We measure trap lifetimes of a few hundred milliseconds, with a maximum value of 460 ms, at an atom-surface separation of 670 nm without active cooling, representing an order-of-magnitude improvement over previous nanofiber traps. This platform opens a new regime for atom-photon interfaces, paving the way for scalable distributed quantum computing and quantum networks, as well as for the exploration of collective radiative effects in waveguide QED with individually addressable atoms.