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Influence of amplification on pulse shaping for coherent control applications

Anton du Plessis, GN Botha, LR Botha

Published Jul 1, 2011• 0 citations
OpenAlex

Abstract

We demonstrate here the importance of using low seed laser powers for amplification of shaped pulses in a typical setup for coherent control experiments. An acousto-optic programmable dispersive filter (Dazzler from FastLite) is used to shape 130 fs pulses before amplification. These devices hold many advantages as compared to other pulse shaping devices [1]. Pulse shaping must be done with care in this configuration, as will be demonstrated with a number of examples of measured pulse shapes before and after amplification.

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We demonstrate here the importance of using low seed laser powers for amplification of shaped pulses in a typical setup for coherent control experiments. An acousto-optic programmable dispersive filter (Dazzler from FastLite) is used to shape 130 fs pulses before amplification. These devices hold many advantages as compared to other pulse shaping devices [1]. Pulse shaping must be done with care in this configuration, as will be demonstrated with a number of examples of measured pulse shapes before and after amplification.
We have constructed an automated learning apparatus to control quantum systems. By directing intense shaped ultrafast laser pulses into a variety of samples and using a measurement of the system as a feedback signal, we are able to reshape the laser pulses to direct the system into a desired state. The feedback signal is the input to an adaptive learning algorithm. This algorithm programs a computer-controlled, acousto-optic modulator pulse shaper. The learning algorithm generates new shaped laser pulses based on the success of previous pulses in achieving a predetermined goal.
We have constructed an automated learning apparatus to control quantum systems. By directing intense shaped ultrafast laser pulses into a variety of samples and using a measurement of the system as a feedback signal, we are able to reshape the laser pulses to direct the quantum system into a desired physical state. The feedback signal is the input to an adaptive learning algorithm. This algorithm programs a computer-controlled, acousto-optic modulator (AOM) pulse shaper. The learning algorithm generates new shaped laser pulses based on the success of previous pulses in achieving a predetermined goal.
Quantum computing exploits the quantum-mechanical nature of matter to exist in multiple possible states simultaneously. This new approach promises to revolutionize the present form of computing. As an approach to quantum computing, we discuss ultrafast laser pulse shaping, in particular, the acousto-optic modulator based Fourier-Transform pulse-shaper, which has the ability to modulate tunable high power ultrafast laser pulses. We show that optical pulse shaping is an attractive route to quantum computing since shaped pulses can be transmitted over optical hardware and the same infrastructure can be used for computation and optical information transfer. We also address the problem of extending coherence-times for optically induced processes.
In this paper, we report on the ultrafast coherent control of excitons in quantum wells using a phase-locked pulse sequence generated by pulse-shaping techniques. The pulse-shaping system with a double liquid-crystal spatial light modulator (SLM), and a Ti3+-sapphire laser is used to generate phase-locked pulses. The ultrafast coherent control of the exciton population and polarization is demonstrated by the observation of the reflectivity change in the pump-probe and the diffracted power in the degenerate-four-wave-mixing (DFWM) measurements. In single quantum wells, good coherent control characteristics with 87% coherent carrier destruction are demonstrated at the low excitation power of 0.15 mW (∼1.1×1010 photons/cm2). In addition, the preliminary manipulation of the exciton population is demonstrated by the phase-locked triple pulses. In the case of coupled quantum wells, the modulation of the SLM is carefully controlled and the coherent control of both the exciton population and the polarization is demonstrated in the two different coupled quantum-well samples.
Controlling stimulated emission is of importance because it competes with absorption and fluorescence under intense laser excitation. We performed resonant nonlinear optical spectroscopy measurements using femtosecond pulses shaped by π- or π/2-step phase functions and carried out calculations based on density matrix representation to elucidate the experimental results. In addition, we compared enhancements obtained when using other pulse shaping functions (chirp, third-order dispersion, and a time-delayed probe). The light transmitted through the high optical density solution was dominated by an intense stimulated emission feature that was 14 times greater for shaped pulses than for transform limited pulses. Coherent enhancement depending on the frequency, temporal, and phase characteristics of the shaped pulse is responsible for the experimental observations.
Broadband low-coherence light has been applied in many fields such as optical imaging, atmospheric optical communication and laser inertial confinement fusion(ICF). It’s meaningful to investigate the temporal shaping technology of broadband low-coherence light. We propose and experimentally demonstrate a scheme of achieving all-optical arbitrary temporal shaping of broadband low-coherence light based on saturable absorption effect. Compared to traditional temporal shaping schemes such as electro-optic modulation(EOM) shaping or acousto-optic modulation(AOM) shaping, the modulation on the shaped pulse profile is much smaller, reduced from 14% (by acousto-optic modulator) to 3%(close to the ASE noise). Furthermore, we explore the evolution of shaped pulse contrast (intensity ratio between front edge and end edge) with the pump energy and contrast changing. The contrast of shaped pulse can be adjusted from 1:1.32 to 1:1.02 when pump contrast is 1:2, and from 1:2.25 to 1:1.90 when pump contrast is 1:3. And the maximum contrast of shaped pulse can reach 1:17 within the measurement accuracy. By changing the energy and contrast of pump, the contrast of the shaped pulse can be controlled flexibly. It’s useful to achieve all-optical arbitrary temporal shaping and pre-compensation during pulse amplification.