Surface Plasmon Polaritions(SPP) are electromagnetic waves that travel in the interface of a metal and dielectric and are coupled to collective oscillation of free electrons. SPP tomography is an imaging technique that permits the study of the interference features formed at the metal-air interface of a sample due to the superposition of SPP beams, with high fidelity. \nWe present an experimental study on the formation of SPP standing waves. We demonstrate that SPP tomography in a quantum eraser arrangement permits the detection of photons passing through the dark fringes of the observed interference pattern. We present a comprehensive explanation of how photons could pass undetected across the regions occupied by the dark fringes.
Surface Plasmon Polaritions(SPP) are electromagnetic waves that travel in the interface of a metal and dielectric and are coupled to collective oscillation of free electrons. SPP tomography is an imaging technique that permits the study of the interference features formed at the metal-air interface of a sample due to the superposition of SPP beams, with high fidelity. \nWe present an experimental study on the formation of SPP standing waves. We demonstrate that SPP tomography in a quantum eraser arrangement permits the detection of photons passing through the dark fringes of the observed interference pattern. We present a comprehensive explanation of how photons could pass undetected across the regions occupied by the dark fringes.
Surface plasmon polaritons (SPPs) are collective excitations of free electrons propagating along a metal-dielectric interface. Although some basic quantum properties of SPPs, such as the preservation of entanglement, the wave-particle duality of a single plasmon, the quantum interference of two plasmons, and the verification of entanglement generation, have been shown, more advanced quantum information protocols have yet to be demonstrated with SPPs. Here, we experimentally realize quantum state teleportation between single photons and SPPs. To achieve this, we use polarization-entangled photon pairs, coherent photon-plasmon-photon conversion on a metallic subwavelength hole array, complete Bell-state measurements and an active feed-forward technique. The results of both quantum state and quantum process tomography confirm the quantum nature of the SPP mediated teleportation. An average state fidelity of [Formula: see text] and a process fidelity of [Formula: see text], which are well above the classical limit, are achieved. Our work shows that SPPs may be useful for realizing complex quantum protocols in a photonic-plasmonic hybrid quantum network.
Light-matter interactions underlie many quantum technologies, yet whether quasiparticles formed from such interactions preserve the full quantum state of light remains unresolved. Surface plasmon polaritons (SPPs), a class of polaritons formed by interacting photons with free-electron oscillations at metal-dielectric interfaces, are prime candidates to explore this question. Here we demonstrate quantum interference between single photons and SPPs using an Au-SiNx integrated photonic-plasmonic device. Our results reveal that SPPs retain the indistinguishability of their excitation photons, establishing SPP as a viable quantum information carrier and opening a potential route toward photonic-plasmonic quantum circuitry.
Surface plasmon polaritons (SPPs) result from collective oscillations of free electrons coupled to an electromagnetic field at a plane interface between a metal and a dielectric medium. As photons, SPPs can be considered either as waves or as bosonic particles [1] and they can experience striking quantum interferences such as Hong-Ou-Mandel (HOM) effect [2]. We use in this paper a plasmonic platform (Fig.1) that can convert photons into plasmons, and separate or recombine them on a plasmonic beamsplitter [3]. Single SPPs are excited using single photons created by parametric down conversion into a periodically-poled KTP crystal. The platform is placed in a Mach-Zehnder interferometer in order to vary the path difference between SPPs before impinging on the beamsplitter. The setup allows us to revisit quantum optics experiments using SPP as carriers of the quantum of energy. Using the same device, we can test the wave-particle duality, two-particle (HOM) interference and non-local control of single plasmon interference using the entanglement between a photon and a SPP [4]. In the case of the HOM experiment, we demonstrate that the losses can be used as a new degree of freedom [5]. Playing with the dephasing between transmission and reflection coefficient of the beamsplitter, we can observe a peak instead of the usually expected dip in the HOM interference (Fig.2), i.e. an anti-coalescence effect of SPP. In this talk, we will introduce the plasmonic device main features as well as the different quantum plasmonics experiments that have been performed thanks to the SPP beamsplitter. These results are essential to understand the SPP quantum behavior or to develop hybrid plasmon-photon systems for potential future applications in quantum communication mediated by SPP. [1] JM Elson and R.H. Ritchie, Phys. Rev. B 4, 4129 (1971) [2] J.S. Fakonas et al., Nat. Phot. 8, 317 (2014) [3] M.C. Dheur et al. , Sc. Advances 2, e151574 (2016) [4] M.C. Dheur et al. ArXiv 1610.07493, B. Vest et al. ArXiv 1610.07479 [5] S. Barnett et al., Phys. Rev. A 57, 2134 (1998) Fig.1: Plasmonic platform used for the quantum optics experiment (B). It consists in two SPP launchers (A), a plasmonic beamsplitter, and two slits to convert SPP to photons in the glass substrate. The plasmonic interference can thus be probed using single photon counting modules. Fig2: HOM experiment on a lossy plasmonic beamsplitter, whose complex amplitude reflection and transmission factors are denoted r and t respectively. The usual HOM dip is observed when r = it (left), a peak in the coincidence rate is shown when r = t.
Surface plasma waves are collective oscillations of electrons that propagate along a metal-dielectric interface. In the last ten years, several groups have reproduced fundamental quantum optics experiments with surface plasmons. Observation of single-plasmon states, waveparticle duality, preservation of entanglement of photons in plasmon-assisted transmission, and more recently, two-plasmon interference have been reported. While losses are detrimental for the observation of squeezed states, they can be seen as a new degree of freedom in the design of plasmonic devices, thus revealing new quantum interference scenarios. Here we report the observation of two-plasmon quantum interference between two freely-propagating, non-guided SPPs interfering on lossy plasmonic beamsplitters. As discussed in the article "Quantum optics of lossy beam splitters" by Barnett et al. (Phys. Rev. A 57, 2134 (1998)) , the presence of losses (scattering or absorption) relaxes constraints on the reflection and transmission factors of the beamsplitter, allowing the control of their relative phase. By using this degree of freedom, we are able to observe either coalescence or anticoalescence of identical plasmons.
In this experiment, pairs of identical photons at 806 nm through a single-photon down conversion in a nonlinear crystal that are sent onto a plasmonic platform were generated. The plasmonic platform consists in several elements that are etched on a 300 nm-thick gold film on top of a silica substrate, on a total 40x40μm footprint. The input channels of the plasmonic platform are made of two unidirectional launchers. Those asymmetric 11-grooves gratings have been designed to efficiently couple a normally incident Gaussian mode into directional SPPs. The SPPs generated by each launcher then freely propagate and recombine on the surface plasmon beamsplitter (SPBS). It is made of two identical grooves in the metallic surface, oriented at 45° with respect to the propagation direction of waves. The succession of metal and air allows a scattering process that generates both a transmitted and a reflected SPP. The SPPs then propagate towards two large outcoupling strip slits. They are decoupled into photons propagating in the glass substrate on the rear of the platform.
Surface plasma waves arise from the collective oscillations of billions of electrons at the surface of a metal in unison. The simplest way to quantize these waves is by direct analogy to electromagnetic fields in free space, with the surface plasmon, the quantum of the surface plasma wave, playing the same role as the photon. It follows that surface plasmons should exhibit all of the same quantum phenomena that photons do, including quantum interference and entanglement. Unlike photons, however, surface plasmons suffer strong losses that arise from the scattering of free electrons from other electrons, phonons, and surfaces. Under some circumstances, these interactions might also cause “pure dephasing,” which entails a loss of coherence without absorption. Quantum descriptions of plasmons usually do not account for these effects explicitly, and sometimes ignore them altogether. In light of this extra microscopic complexity, it is necessary for experiments to test quantum models of surface plasmons. In this thesis, I describe two such tests that my collaborators and I performed. The first was a plasmonic version of the Hong-Ou-Mandel experiment, in which we observed two-particle quantum interference between plasmons with a visibility of 93 ± 1%. This measurement confirms that surface plasmons faithfully reproduce this effect with the same visibility and mutual coherence time, to within measurement error, as in the photonic case. The second experiment demonstrated path entanglement between surface plasmons with a visibility of 95 ± 2%, confirming that a path-entangled state can indeed survive without measurable decoherence. This measurement suggests that elastic scattering mechanisms of the type that might cause pure dephasing must have been weak enough not to significantly perturb the state of the metal under the experimental conditions we investigated. These two experiments add quantum interference and path entanglement to a growing list of quantum phenomena that surface plasmons appear to exhibit just as clearly as photons, confirming the predictions of the simplest quantum models.