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Bulletin of the American Physical Society

Double-pulse deexcitations in a one-dimensional strongly correlated system

Takami Tohyama, Hantao Lu, J. Bonča

Published Mar 3, 2014• 0 citations
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We investigate the ultrafast optical response of the one-dimensional half-filled extended Hubbard model exposed to two successive laser pulses. By using the time-dependent Lanczos method, we find that following the first pulse, the excitation and deexcitation process between the ground state and excitonic states can be precisely controlled by the relative temporal displacement of the pulses. The underlying physics can be understood in terms of a modified Rabi model. Our simulations clearly demonstrate the controllability of ultrafast transition between excited and deexcited phases in strongly correlated electron systems.
Encouraged by the experiments on production of antihydrogen atoms in high Rydberg states we have calculated the effect of deexcitation towards lower states by a chirped train of identical unidirectional half-cycle pulses. The calculations exploit both the one-dimensional and impulse approximations providing convenient analytical formulas for the Rydberg-to-Rydberg transition amplitudes. The calculated deexcitation is shown in terms of the mean value of localization of the Rydberg wave packet in the coordinate space, the Rydberg-state population distribution, the Husimi phase-space distribution function, and the probability density distribution, each of these measures vs the length of the applied train of half-cycle pulses. The results for chirped trains are compared with those for periodic trains and examples of higher deexcitation efficiency of the chirped trains are given.