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Physica C Superconductivity

Electronic excitations in strongly correlated systems; 1D vs. 2D

Sadamichi Maekawa, Takami Tohyama

Published Aug 1, 1997• 8 citations
Publisher
DOI
10.1016/s0921-4534(97)00260-8

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One of the central issues in the study of high-temperature superconducting cuprates which are composed of two-dimensional (2D) CuO 2 planes is whether the 2D systems with strong electron correlation behave as a Fermi liquid or a non-Fermi-liquid-like one-dimensional (1D) system with electron correlation. In this article, we start with the detailed examination of the electronic structure in cuprates and study theoretically the spin and charge dynamics in 1D and 2D cuprates. The theoretical background of spin-charge separation in the 1D model systems including the Hubbard and t - J models is presented. The first direct observation of collective modes of spin and charge excitations in a 1D cuprate, which are called spinons and holons respectively, in angle-resolved photoemission spectroscopy (ARPES) experiments is reviewed in the light of the theoretical results based on the numerically exact-diagonalization method. The charge and spin dynamics in 1D insulating cuprates is also discussed in connection with the spin-charge separation. The arguments are extended to the 2D cuprates, and the unique aspects of the electronic properties of high-temperature superconductors are discussed. Special emphasis is placed on the d-wave-like excitations in insulating 2D cuprates observed in ARPES experiments. We explain how the excitations are caused by the spin-charge separation. The charge stripes observed in the underdoped cuprates are examined in connection with spin-charge separation in real space.
We report on a nonperturbative approach to the one-dimensional (1D) and two-dimensional (2D) Hubbard models that is capable of recovering both strong- $(U\ensuremath{\gg}t)$ and weak-coupling $(U\ensuremath{\ll}t)$ limits, with U the on-site Coulomb repulsion and t the kinetic energy. Dynamical corrections to the electron self-energy in the single particle Green function are explicitly included by expanding in terms of the 16 eigenstates that characterize two nearest neighbor sites. We first show that even when U is much smaller than the bandwidth, the Mott-Hubbard gap never closes at half filling in both 1D and 2D. Consequently, the Hubbard model at half filling is always in the strong-coupling nonperturbative regime. For both large and small U, we find that the population of nearest-neighbor singlet states approaches a value of order unity as $\stackrel{\ensuremath{\rightarrow}}{T}0$ as would be expected for antiferromagnetic order. We also find that the double occupancy is a smooth monotonic function of U and approaches the anticipated noninteracting limit of 1/41/41/4 as $\stackrel{\ensuremath{\rightarrow}}{U}0$ and vanishes as $\stackrel{\ensuremath{\rightarrow}}{U}\ensuremath{\infty}.$ Finally, we compute the heat capacity [C(T,U)][C(T,U)][C(T,U)] for both 1D and 2D. Our results for 1D at moderate to high temperatures are in quantitative agreement with those of the exact Bethe ansatz solution, differing by no more than 11%.1 In addition, we find that in 2D, the C(T,U)C(T,U)C(T,U) curves vs T for different values of U exhibit a universal crossing point at two characteristic temperatures $T\ensuremath{\approx}1.7t\ifmmode\pm\else\textpm\fi{}0.1t$ and $T\ensuremath{\approx}0.4\ifmmode\pm\else\textpm\fi{}0.1t$ as is seen universally in Hubbard models and experimentally in a wide range of strongly correlated systems such as 3He,{}^{3}\mathrm{He},3He, UBe3,{\mathrm{UBe}}_{3},UBe3​, and ${\mathrm{CeCu}}_{6\ensuremath{-}x}{\mathrm{Al}}_{x}.$ The success of this method in recovering well-established results that stem fundamentally from the Coulomb interaction suggests that local dynamics are at the heart of the physics of strongly correlated systems.
We theoretically investigate the properties of multiphoton excited states in strongly correlated one-dimensional (1D) and two-dimensional (2D) electron systems at half filling using the extended Hubbard model. In the 2D case, we find the photoexcited states where two or more than two holons and doublons are strongly bound, and the cluster of bound holons and doublons coexists with the surrounding antiferromagnetic (AF) spin order, for the realistic Coulomb interaction parameters. The holon-doublon cluster (HDC) states have a unique charge aggregation mechanism originating from the spin-spin interaction in the AF spin background as well as from the direct Coulomb interaction. In the 1D case, the HDC states are destabilized by the spin-spin interaction in contrast to the 2D case. These charge aggregation mechanisms are the outcomes of exotic natures of holons and doublons, and the difference in the mechanism between the 1D and 2D cases is due to the difference in the coupling between spin and charge degrees of freedom. We also calculate the light-induced absorption that enables us to experimentally observe the predicted HDC states.