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Bulletin of the American Physical Society

Probing autoionization and AC Stark shift with attosecond transient absorption spectroscopy

Michael Chini, He Wang, C.-H. Zhang, Feng He, Shouyuan Chen, Yan Cheng, Baozhen Zhao, Yi Wu, Uwe Thumm, Zenghu Chang

Published Jun 16, 2011• 0 citations
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Strong-field manipulation of autoionizing states is a crucial aspect of electronic quantum control. Recent measurements of the attosecond transient absorption spectrum (ATAS) of helium dressed by a few-cycle visible pulse [C. Ott et al , Nature 516, 374 (2014)] provide evidence of the inversion of Fano profiles. With the support of accurate ab-initio calculations that reproduce the results of the latter experiment, here we investigate the new physics that arise from ATAS when the laser intensity is increased. In particular, we show that (i) previously unnoticed signatures of the dark 2 p 2 1 S doubly excited state are observed in the experimental spectrum, (ii) inversion of Fano profiles is predicted to be periodic in the laser intensity, and (iii) the ac-Stark shift of the higher terms in the sp + 2, n autoionizing series exceeds the ponderomotive energy, which is the result of a genuine two-electron contribution to the polarization of the excited atom.