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International Conference on Ultrafast Phenomena

Diffractive optics-based heterodyne detected three-pulse photon echo

Jennifer P. Ogilvie, Michael R. Armstrong, Andrea M. Nagy, R. J. Dwayne Miller

Published Jan 1, 2002• 6 citations
Publisher

Abstract

A novel diffractive optics-based method for performing three pulse photon echoes is demonstrated and extends the inherent passive phase stabilization of diffractive optics to this class of experiments for complete recovery of the signal field.
DOI
10.1364/up.2002.wd20

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Phase-locked optical coherence experiments were performed on the 10 fs time scale. A 13 fs cavity-dumped Ti:sapphire laser was considered as an ideal source to extend these experiments to the 10 fs time scale due to extremely high amplitude and spectral stability. Femtosecond phase-locked heterodyne detected femtosecond stimulated photon echo (PL-HSPE) proved to be very useful for exploring the details of the optical dynamics of the optical system. The PL-HSPE involves a six-dimensional experiment governed by three times between four fs pulses, two relative phases between paired pulses, and signal amplitude.