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Physics Letters A

Quantum simulating the frustrated Heisenberg model in a molecular dipolar crystal

Yan‐Li Zhou, Bao-Quan Ou, Wei Wu

Published Jun 12, 2015• 7 citations
Publisher
DOI
10.1016/j.physleta.2015.06.009

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We simulate a molecular Bose-Einstein condensate in the strongly dipolar regime, observing the existence of self-bound droplets, as well as their splitting into multiple droplets by confinement-induced frustration. Our quantum Monte Carlo approach goes beyond the limits of the established effective mean-field theories for dipolar quantum gases, revealing small droplets produced by strong dipolar interactions outside known stable regimes. The simulations include realistic molecular interactions and therefore have direct relevance for current and future experiments.
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The antiferromagnetic Heisenberg model on the triangular lattice is perhaps the best known example of frustrated magnets, but it orders at low temperatures. Recent density matrix renormalization group (DMRG) calculations find that the next nearest neighbor interaction J_{2} enhances the frustration, and it leads to a spin liquid for J_{2}/J_{1}∈(0.08,0.15). In addition, a DMRG study of a dipolar Heisenberg model with longer range interactions gives evidence for a spin liquid at a small dipole tilting angle θ∈[0,10°). In both cases, the putative spin liquid region appears to be small. Here, we show that for the triangular lattice dipolar Heisenberg model, a robust quantum paramagnetic phase exists in a surprisingly wide region, θ∈[0,54°), for dipoles tilted along the lattice diagonal direction. We obtain the phase diagram of the model by functional renormalization group (RG), which treats all magnetic instabilities on equal footing. The quantum paramagnetic phase is characterized by a smooth continuous flow of vertex functions and spin susceptibility down to the lowest RG scale, in contrast to the apparent breakdown of RG flow in phases with stripe or spiral order. Our finding points to a promising direction to search for quantum spin liquids in ultracold dipolar molecules.