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Acta Physica Sinica

Research on improve the SNR of ultracold cesium molecule rovibronic spectrum via best optimization parameter control

Zhang Yi-Chi, Jizhou Wu, Jie Ma, Yanting Zhao, Wang Li-Rong, Liantuan Xiao, Jia Suo-Tang

Published Jan 1, 2010• 11 citations
Publisher

Abstract

Ultracold atom photoassociation spectroscopy is significant for studying the long-range molecular potential energy structure. The signal-noise ratio of ultracold Cesium Molecule photoassociation Rovibronic Spectrum is one of the indicators as a measure of detection technology which directly affect the distinguishing ability and detection sensitivity of the spectra. We obtain an long-range ultracold cesium molecular hyperfine rovibration spectra by modulating the fluorescence spectroscopy. We find that demodulation parameters have a significant impact to the signal-noise ratio of spectra by studying the demodulation parameters such as integration time and sensitivity, which show nonlinear relation with the ratio. We achieve the optimal control of the signal-noise ratio for spectrum according to our experiment, which laid an important foundation for further studying the long-range state rovibration level of ultracold cesium molecule.

DOI
10.7498/aps.59.5418

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Ultracold atom photoassociation spectroscopy is significant for studying the long-range molecular potential energy structure. The signal-noise ratio of ultracold Cesium Molecule photoassociation Rovibronic Spectrum is one of the indicators as a measure of detection technology which directly affect the distinguishing ability and detection sensitivity of the spectra. We obtain an long-range ultracold cesium molecular hyperfine rovibration spectra by modulating the fluorescence spectroscopy. We find that demodulation parameters have a significant impact to the signal-noise ratio of spectra by studying the demodulation parameters such as integration time and sensitivity, which show nonlinear relation with the ratio. We achieve the optimal control of the signal-noise ratio for spectrum according to our experiment, which laid an important foundation for further studying the long-range state rovibration level of ultracold cesium molecule.
In the present paper, ultracold cesium atoms were obtained in magnetic optical trap using the laser cooling technology. The number of ultracold atoms is 10(7). The temperature of ultracold atoms is about 200 μK and the diameter of the ultracold atoms cloud is about 400 μm. The ultracold cesium molecules of excited states were formed using the photoassociation of ultracold atoms. The resolution of vib-rotational spectrum was studied under different scan rates of photossociation laser in the experiment. The resolution of vib-rotational spectrum becomes high when the scan rate of photossociation laser becomes slow. The cold atoms fluorescence was obtained using the high sensitive avalanche photo detector and the high resolution vib-rotational spectrum of ultracold cesium molecule in its first excited state of with dissociation limit long range state was obtained. The ultracold ground molecule was formed by controlled Raman photoassociation and the photoassociation laser must be locked to atom-molecular hyperfine transitions. The ultracold atoms photoassociation spectrum was modulated using ultra-low frequency. The first-order differential signal was optimized by changing modulation amplitude and modulation frequency. It provides a feedback signal to correct error of the laser. The laser frequency satisfies experimental requirement to form ultracold ground molecules using the controlled Raman photoassociation. This work is important for studies of ultracold atoms and molecules in confined space.
A high resolution photoassociation spectrum of ultracold cesium atoms is reported in this paper. A photoassociation laser with its frequency red detuned below 6S1/2+6P3/2 dissociation limit acts on the cold cesium atoms in magnetic optical trap and the excited ultracold molecules generated in the photoassociation process are observed. In order to obtain a high signal-to-noise ratio, the trapping laser is amplitude modulated using acousto-optic modulator and the fluorescence signal is demodulated by lock-in technique. The results are discussed using the density matrix equations.
Photoassociation spectroscopy with high resolution for 0u+(6P3/2) long-range state of ultracold cesium molecules has been measured experimentally using the modulated trap loss fluorescence spectroscopy technology. The spectral range has been extended over 60 cm-1 below the 6S1/2 + 6P3/2 dissociation limit as compared with other groups. twenty-five new observations of the Cs2 0u+ in long-range state are reported. The vibrational binding energies of these states are analyzed by using the LeRoy-Bernstein formula. The long-range parameter C3 in molecular 0u+(6P3/2) state is derived for 16.1030.010, and the corresponding molecular potential curve is depicted.
We report a method of high-sensitively detecting the weak signal in photoassociation (PA) spectra of ultracold NaCs molecules by phase sensitive-demodulated trap-loss spectra of Na atoms from a photomultiplier tube. We find that the signal-to-noise ratio (SNR) of the PA spectra is strongly dependent on the integration time and the sensitivity of the lock-in amplifier, and our results show reasonable agreement with the theoretical analyses of the SNR with the demodulation parameters. Meanwhile, we investigate the effect of the interaction time of the PA laser with the colliding Na–Cs atom pairs on the SNR of the PA spectra. The atom loss rate is dependent on both the PA-induced atom loss and the loading of the MOT. The high-sensitive detection of the excited ultracold NaCs molecules lays a solid foundation for further study of the formation and application of ultracold NaCs molecules.
Photoassociation of ultracold atoms is an important method for producing stable ultracold molecules with extensive applications. Ion spectroscopy technique, which has higher sensitivity compared with trap loss spectroscopy and fragment spectroscopy, plays an important pole in the research of photoassociation spectroscopy. Based on ion spectroscopy technique, a complete experimental system is employed to produce and detect the ultracold ground state molecules, including the equipment of photoionization and time-of-fight mass spectroscopy. Ultra-cold ground state cesium molecules are demonstrated by the ionization detection technique. The number of the ground-state molecules produced in our MOT is measured. In addition, the relationship of the time interval of the cesium atom ion and the cesium molecular ion to the metal grid voltage is studied for the optimization of the experimental parameters.