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Optics Express

Statistically background-free, phase-preserving parametric up-conversion with faint light

Yu‐Hsiang Cheng, Tim O. Thomay, Glenn S. Solomon, Alan L. Migdall, Sergey V. Polyakov

Published Jul 9, 2015• 13 citations
Publisher

Abstract

We demonstrate up-conversion with no statistically significant background photons and a dynamic range of 15 decades. Near-infrared 920 nm photons were converted into the visible at 577 nm using periodically poled lithium niobate waveguides pumped by a 1550 nm laser. In addition to achieving statistically noiseless frequency up-conversion, we report a high degree of phase preservation (with fringe visibilities ≥ 0.97) at the single-photon level using an up-converting Mach-Zehnder interferometer. This background-free process opens a path to single-photon detection with no intrinsic dark count. Combined with a demonstrated photon-number preserving property of an up-converter, this work demonstrates the feasibility of noiseless frequency up-conversion of entangled photon pairs.

DOI
10.1364/oe.23.018671

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We demonstrate up-conversion with no statistically significant background photons and a dynamic range of 15 decades. Near-infrared 920 nm photons were converted into the visible at 577 nm using periodically poled lithium niobate waveguides pumped by a 1550 nm laser. In addition to achieving statistically noiseless frequency up-conversion, we report a high degree of phase preservation (with fringe visibilities ≥ 0.97) at the single-photon level using an up-converting Mach-Zehnder interferometer. This background-free process opens a path to single-photon detection with no intrinsic dark count. Combined with a demonstrated photon-number preserving property of an up-converter, this work demonstrates the feasibility of noiseless frequency up-conversion of entangled photon pairs.
We characterize an efficient and nearly-noiseless parametric frequency upconverter. The ultra-low noise regime is reached by the wide spectral separation between the input and pump frequencies and the low pump frequency relative to the input photons. The background of only ≈100 photons per hour is demonstrated. We demonstrate phase preservation in a frequency upconversion process at the single-photon level. We summarize our efforts to measure this ultra-low noise level, and discuss both single-photon avalanche photodiode measurements and a photon-counting transition edge sensor (TES) measurements. To reach the required accuracy, we supplemented our TES with a dark count reduction algorithm. The preservation of the coherence was demonstrated by simultaneously upconverting the input of each arm of a Mach-Zehnder interferometer through high interference fringe contrast. We observe fringe visibilities of ≥0.97 with faint coherent input.
We demonstrate background-free quantum frequency conversion of single photons from an epitaxially-grown InAs quantum dot. Single photons at \approx 980 nm are combined with a pump laser near 1550 nm inside a periodically-poled lithium niobate (PPLN) waveguide, generating single photons at \approx 600 nm. The large red-detuning between the pump and signal wavelengths ensures nearly background-free conversion, avoiding processes such as upconversion of anti-Stokes Raman scattered pump photons in the PPLN crystal. Second-order correlation measurements on the single photon stream are performed both before and after conversion, confirming the preservation of photon statistics during the frequency conversion process.
Single-photon sources based on quantum dots have been shown to exhibit almost ideal properties such as high brightness and purity in terms of clear anti-bunching as well as high two-photon interference visibilities of the emitted photons, making them promising candidates for different quantum information applications such as quantum computing, quantum communication and quantum teleportation. However, as most single-photon sources also quantum dots typically emit light at wavelengths of electronic transitions within the visible or the near infrared range. In order to establish quantum networks with remote building blocks, low-loss single photons at telecom wavelengths are preferable, though. Despite recent progress on emitters of telecom-photons, the most efficient single-photon sources still work at shorter wavelengths. On that matter, quantum frequency down-conversion, being a nonlinear optical process, has been used in recent years to alter the wavelength of single photons to the telecom wavelength range while conserving their nonclassical properties. Characteristics such as lifetime, first-order coherence, anti-bunching and entanglement have been shown to be conserved or even improved due to background suppression during the conversion process, while the conservation of indistinguishability was yet to be shown. Here we present our experimental results on quantum frequency down-conversion of single photons emitted by an InAs/GaAs quantum dot at 903.6 nm following a pulsed excitation of a p-shell exciton at 884 nm. The emitted fluorescence photons are mixed with a strong pump-field at 2155 nm inside a periodically poled lithium niobate ridge waveguide and converted to 1557 nm. Common issues of a large background due to Raman-scattered pump-light photons spectrally overlapping with the converted single photons could largely be avoided, as the pump-wavelength was chosen to be fairly longer than the target wavelength. Additional narrowband spectral filtering at the telecom regime as a result of the small conversion bandwidth and using a high-performance fiber-Bragg-grating solely left the detector dark counts as the only noise source in our setup. Therefore, we could achieve conversion efficiencies of more than 20 %. In order to test the indistinguishability, sequentially emitted photons were fed into a Mach-Zehnder interferometer and spatially as well as temporally overlapped at the output beam splitter. Cross-correlation measurements between both output-ports of the beam splitter exhibit two-photon interference contrasts of more than 40 % prior to and after the down-conversion step. Accordingly, we demonstrate that the process of quantum frequency conversion preserves photon indistinguishability and can be used to establish a versatile source of indistinguishable single photons at the telecom C-Band. Furthermore our scheme allows for converting photons in a wavelength band from 900 nm to 910 nm to the same telecom target wavelength. This enables us to test indistinguishability of frequency-converted photons, originally stemming from different sources with dinstinguishable wavelengths.
We propose a method of single photon detection of infrared (IR) photons at potentially higher efficiencies and lower noise than allowed by traditional IR band Avalanche Photodiodes (APD). By up-converting the photon from IR, e.g., 1550 nm, to a visible wavelength in a nonlinear crystal, we can utilize the much higher efficiency of visible wavelength APDs. We have used a nonlinear crystal -- Periodically Poled Lithium Niobate (PPLN) -- and a pulsed 1064-nm Nd:YAG laser to perform the up-conversion to a 631-nm photon. When properly quasi-phase-matched, PPLN provides a large enough second order nonlinear susceptibility that near unit conversion efficiency of the IR photon into the visible should be possible. We have been able to observe peak conversion efficiencies as high as 80%, and have demonstrated scaling down to the single photon level while maintaining a background of 3 x 10-4 dark counts/count. Since the PPLN only acts on one polarization of the single photon, we also propose a 2-crystal extension of this scheme whereby orthogonal polarizations may be up-converted coherently, thereby enabling complete quantum state transduction.