At low temperatures, the thermodynamic properties of a many-body system are determined by the low energy excursions from the ground state. In quantum degenerate rubidium, the low energy excitations are phonons—phase and density modes—and magnons—spin modes. This thesis reports on the construction of an ultracold rubidium apparatus and techniques to create and image phonons and magnons. We propose and study matter wave interferometry of phonons in a ring trap as a potential rotation sensor in a compact sensor. Precision measurements of coherent magnons allow us to determine the magnon dispersion relation, including a gap induced by magnetic dipole-dipole interactions.
At low temperatures, the thermodynamic properties of a many-body system are determined by the low energy excursions from the ground state. In quantum degenerate rubidium, the low energy excitations are phonons—phase and density modes—and magnons—spin modes. This thesis reports on the construction of an ultracold rubidium apparatus and techniques to create and image phonons and magnons. We propose and study matter wave interferometry of phonons in a ring trap as a potential rotation sensor in a compact sensor. Precision measurements of coherent magnons allow us to determine the magnon dispersion relation, including a gap induced by magnetic dipole-dipole interactions.
Ultracold atomic gas systems provide a remarkably versatile platform for studying a wide range of physical phenomena, from analogue particle physics and gravity, to the emergence of subtle and profound order in many body and condensed matter systems. In addition, ultracold atomic gas systems can be used to perform a range of precision measurements, from time keeping to variations in the fine structure constant. In this dissertation, I describe our efforts to build a new apparatus capable testing a range of techniques for performing precision measurements in a magnetic storage ring for cold, possibly Bose-condensed, lithium and rubidium atoms. Next, I briefly touch upon our explorations of spin vortices in a ferromagnetic rubidium Bose-Einstein condensate before presenting an exhaustive account of our work using free-particle-like magnon excitations of the ferromagnetic gas to cool it and measure its temperature in a never-before-seen regime of low entropy. Using magnons as a thermometer, we measure temperatures as low as one nanokelvin in gases with an entropy per particle of about one thousandth of the Boltzmann constant, 0.001 k_B. I conclude by presenting the details of our procedure for calculating the entropy of our coldest, lowest entropy gases in the regime where the local density approximation does not apply.
We measure the dispersion relation, gap, and magnetic moment of a magnon in the ferromagnetic F = 1 spinor Bose-Einstein condensate of (87)Rb. From the dispersion relation we measure an average effective mass 1.033(2)(stat)(10)(sys) times the atomic mass, as determined by interfering standing and running coherent magnon waves within the dense and trapped condensed gas. The measured mass is higher than theoretical predictions of mean-field and beyond-mean-field Beliaev theory for a bulk spinor Bose gas with s-wave contact interactions. We observe a magnon energy gap of h × 2.5(1)(stat)(2)(sys) Hz, which is consistent with the predicted effect of magnetic dipole-dipole interactions. These dipolar interactions may also account for the high magnon mass. The effective magnetic moment of -1.04(2)(stat)(8)(sys) times the atomic magnetic moment is consistent with mean-field theory.
Bose-Einstein condensation (BEC) is a phenomenon in which identical bosons occupy the same quantum state below a certain critical temperature. A hallmark of BEC is the coherence between particles every particle shares the same quantum wavefunction and phase. This coherence has been demonstrated for the external (motional) degrees of freedom of the atomic condensates by interfering two condensates. In this thesis, the coherence is shown to extend to the internal spin degrees of freedom of a spin-1 Bose gas evidenced by the observed coherent and reversible spin-changing collisions. The observed coherent dynamics are analogous to Josephson oscillations in weakly connected superconductors and represent a type of matter-wave four-wave mixing. Control of the coherent evolution of the system using magnetic fields is also demonstrated. The studies on spinor condensates begin by creating spinor condensates directly using all-optical approaches that were first developed in our laboratory. All-optical formation of Bose-Einstein condensates (BEC) in 1D optical lattice and single focus trap geometries are developed and presented. These techniques offer considerable flexibility and speed compared to magnetic trap approaches, and the trapping potential can be essentially spin-independent and are ideally suited for studying spinor condensates. Using condensates with well-defined initial non-equilibrium spin configuration, spin mixing of F = 1 and F = 2 spinor condensates of rubidium-87 atoms confined in an optical trap is observed. The equilibrium spin configuration in the F = 1 manifold confirms that 87Rb is ferromagnetic. The coherent spinor dynamics are demonstrated by initiating spin mixing deterministically with a non-stationary spin population configuration. Finally, the interplay between the coherent spin mixing and spatial dynamics in spin-1 condensates with ferromagnetic interactions is investigated.
This thesis contains theoretical studies of weakly interacting, trapped Bose-Einstein condensed gases. The main emphasis is on the rotational properties of these systems. A typical Bose-Einstein condensate reacts to external rotation by forming singly quantized vortices. By the word ”typical” we refer to a condensate with repulsive interparticle interactions and with a frozen spin degree of freedom. However, there are some atomic species for which the low-energy interactions are attractive. Moreover, the tuning of different condensate properties is relatively easy. For example, there are ways to experimentally change the effective interaction from repulsive to attractive. For an attractively interacting condensate the vortex is not the only possible rotational state but the sample may also experience rotation through its center of mass. In the first part of the thesis, we analyze some properties of a rotating attractive Bose gas at the zero temperature limit. First, we note that in order to maintain energetical stability, the gas has to be rotated in an external trap which is steeper than a harmonic trap. We study the system in an anharmonic quadratic + quartic potential. The rotating ground state phase-space is determined with analytical and numerical methods. If the interactions are strong enough, the rotating ground state appears to be a state with the rotating center of mass. On the other hand, at the limit of weak interactions the system experiences rotation by forming a multiply quantized vortex. We also determine the spectrum of elementary excitations for these quantum many-particle states. We find that the broken symmetry of the center of mass rotating state induces an additional zero-energy (Goldstone) mode and that the small oscillations of the ground state exhibit the decoupling between the center of mass and relative motions. If the spin of the atoms is allowed to change freely, a rich variety of topological excitations in condensates can be studied. External rotation is one of the tools for examining the excitations in spinor condensates. In a spinless scalar condensate the appearance of a quantized vortex is manifested by the vortex line in which the condensate density vanishes. In the plane perpendicular to the vortex line, one speaks of the vortex core for the density minimum. We study the properties of slowly rotated F = 1 spinor condensates and show that for ferromagnetic interactions the ground state is a coreless vortex. While the individual spin components may carry ordinary vortices the overall density of the system is coreless. We also study a method to create a point-like monopole structure in a ferromagnetic condensate by suitably imprinting vortices and solitons for different spin components of the condensate.
Spinor Bose-Einstein condensates (BECs) are multi-component superfluids with magnetic interactions, formed from dilute gases of atoms in the Zeeman sublevels mF of a single hyperfine ground state F. Spinor BECs are inherently magnetic quantum objects, and exhibit a multitude of features such as spin domains, magnon excitations, and distinct magnetic phases. At the heart of the magnetic nature of a spinor BEC is the spin-dependent collisional interaction c, which determines the overall magnetic behaviour of the superfluid. In conjunction with the quadratic Zeeman shift q, the magnitude and sign of c give rise to an intricate magnetic phase diagram. The magnetic phase of a spinor BEC is tunable, and c and q are the knobs. In addition to realising quantum simulators of magnetism, spinor BECs are also precise magnetic sensors. Atomic magnetometry measures the Larmor precession frequency of atoms, which is proportional to the magnetic field strength. The sensitivity of an atomic magnetometer is principally dependent on the duration of the measurement (interrogation time) and number of atoms participating in the measurement. BECs are highly suitable as atomic magnetometers, allowing for long interrogation times and high atomic density, with microscopic sensor volumes. The latter is an important consideration, as measurement of small magnetic sources demand equally microscopic sensors. Established forms of magnetometry (such as warm vapour magnetometers) use large sensing volumes and are not trivially miniaturised. The exquisite sensitivity of a spinor BEC to magnetic fields becomes a liability when one studies low energy (~ 1 Hz) spinor physics over long evolution times (100 ms) in a typical laboratory environment. To first order, the spin-collisional interaction is independent of the magnetic field. However, spatially inhomogeneous magnetic fields are problematic, exerting mechanical forces on the magnetically sensitive spin components, suppressing spin collisions and possibly introducing relaxation mechanisms that confound the observation of intrinsic equilibration. Precise characterisation of magnetic field gradients and their cancellation is thus of paramount importance. In this thesis, the interaction of a spinor BEC with its environment is studied. The construction, operation and optimisation of a BEC machine is described in detail, as well as the quantum state preparation and control techniques used. Spin-mixing collisions were studied by observing population oscillations, the characteristic hallmark of such coherent phenomena. The observed population dynamics showed strong evidence of the deleterious effects of magnetic field gradients. A series of experiments were performed using spin-echo pulse sequences to decouple the evolving spinor condensate from the inhomogeneous magnetic environment with encouraging results, but which posed further questions. The fidelity of spin-echo pulses in the strong radiative coupling regime was also studied. Spinor condensates were then employed as sensitive magnetometers to characterise the magnetic landscape they inhabit. A new method of measuring magnetic field gradients was developed, using a pair of spinor BECs separated in space that are simultaneously addressed by a Ramsey interferometry sequence. Combined with a re-orientable magnetic bias field, the resulting gradiometer was used to measure the magnetic field gradient tensor in vacuo. This scheme can be extended to realise a high-precision vector co-magnetometer, with spatiotemporal sensitivity comparable to established forms of magnetometry. Vector light shifts (VLSs) are optically-induced energy shifts that result in effective magnetic fields, which in our case originate from the laser beams used to trap the atoms. The VLS vanishes for purely linearly polarised light, which is experimentally difficult to obtain in vacuo. Small elliptical polarisation imperfections originating from birefringent optics and the glass vacuum cell result in a non-zero shift that contaminates magnetometry measurements. The VLS is spatially varying due to the intensity gradient of the trapping light. Due to gravitational sag of the trapping potential, the spatial variation of the VLS is accentuated, resulting in an effective magnetic field gradient that contributes to dephasing and component separation. The simultaneous Ramsey interferometry experiments are then adapted to measure the VLS-induced Zeeman shift and diagnose its elimination. Up to 99.96% of the VLS is eliminated using this method, and extensions to the technique are described.
Long-lived coherent spin precession of 3He-B at low temperatures around 0.2 Tc is a manifestation of Bose-Einstein condensation of spin-wave excitations or magnons in a magnetic trap which is formed by the order-parameter texture and can be manipulated experimentally. When the number of magnons increases, the orbital texture reorients under the influence of the spin-orbit interaction and the profile of the trap gradually changes from harmonic to a square well, with walls almost impenetrable to magnons. This is the first experimental example of Bose condensation in a box. By selective rf pumping the trap can be populated with a ground-state condensate or one at any of the excited energy levels. In the latter case the ground state is simultaneously populated by relaxation from the exited level, forming a system of two coexisting condensates.