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Experimentally-friendly methods of generation and detection of quantum correlations

Monika Bartkowiak

Published Jan 1, 2012• 0 citations
OpenAlex

Abstract

One of the most relevant problems in the quantum theory is the question whether the appropriate state of the system can be described within a classical theory. The famous examples of nonclassical states are Schrodinger-cats states or entanglement states. In spite of many practical applications of entanglement as a special kind of nonclassicality (like quantum teleportation [1], dense coding [2], or implementation of super-fast [3] and fast algorithms [4]), we still have difficulties with describing and specifying it. One cannot find such an operational optimal method, which would allow us to maximally use the technological and scientific potential arising from the adaptation properties of quantum correlations. Thus, my thesis is focused on giving a proposal of a theoretical recipe for constructing experimentally achievable procedures for the study of quantum correlations. In my thesis I have focused on quantum correlations described in terms of nonclassicality (quantumness) and specific kind of it,i.e., entanglement. The nonclassicality definition, used by me in the thesis, is based on the Glauber-Sudarshan function (P -function). One can assume, that a state is nonclassical, if its P -function is negative or more singular than Dirac’s delta [5]. As follows, the state is nonclassical, when its P -function cannot be treated as a “real” probabilistic distribution. Based on specific properties of the P -function, Agarwal and Tara [6], as well as, Shchukin, Richter and Vogel [7, 8] proposed nonclassicality and entanglement [9] criteria based on matrices of moments of annihilation and creation operators. The operational procedures for analyzing nonclassicality and an efficient method for measuring such moments developed by Shchukin and Vogel [10] creates basis for my thesis. It can be seen that the nonclassicality criteria based on matrices of moments offer an effective way of deriving specific inequalities, which might be useful in the verification of nonclassicality of particular states generated in experiments. Therefore, criteria constructed based on the above definition of nonclassicality can be used to find practical and effective methods of generating and testing nonclassicality and, therefore, also quantum entanglement of optical fields. The results presented in my thesis can be divided into three main groups: 1. Finding operational and practical criteria to classify states in terms of nonclassicality and entanglement based on fundamental classical inequalities like Cauchy-Schwarz inequality. It was also shown how some known entanglement inequalities can be derived as nonclassicality inequalities or as sums of more than one inequality [Bartkowiak2010a]. 2. Describing properties and behaviour of quantum correlations for different optical fields (e.g. for multiand single-mode systems, for interacting and noninteracting modes). In particular, general occurrence of sudden vanishing of nonclassicality, which can be observed not only for twoor multimode but also for single-mode fields, was proven [Bartkowiak2011]. 3. Finding the methods of generating and testing of quantum correlations, which would be practical and easy to implement with available resources in both linear and nonlinear optics.

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One of the most relevant problems in the quantum theory is the question whether the appropriate state of the system can be described within a classical theory. The famous examples of nonclassical states are Schrodinger-cats states or entanglement states. In spite of many practical applications of entanglement as a special kind of nonclassicality (like quantum teleportation [1], dense coding [2], or implementation of super-fast [3] and fast algorithms [4]), we still have difficulties with describing and specifying it. One cannot find such an operational optimal method, which would allow us to maximally use the technological and scientific potential arising from the adaptation properties of quantum correlations. Thus, my thesis is focused on giving a proposal of a theoretical recipe for constructing experimentally achievable procedures for the study of quantum correlations. In my thesis I have focused on quantum correlations described in terms of nonclassicality (quantumness) and specific kind of it,i.e., entanglement. The nonclassicality definition, used by me in the thesis, is based on the Glauber-Sudarshan function (P -function). One can assume, that a state is nonclassical, if its P -function is negative or more singular than Dirac’s delta [5]. As follows, the state is nonclassical, when its P -function cannot be treated as a “real” probabilistic distribution. Based on specific properties of the P -function, Agarwal and Tara [6], as well as, Shchukin, Richter and Vogel [7, 8] proposed nonclassicality and entanglement [9] criteria based on matrices of moments of annihilation and creation operators. The operational procedures for analyzing nonclassicality and an efficient method for measuring such moments developed by Shchukin and Vogel [10] creates basis for my thesis. It can be seen that the nonclassicality criteria based on matrices of moments offer an effective way of deriving specific inequalities, which might be useful in the verification of nonclassicality of particular states generated in experiments. Therefore, criteria constructed based on the above definition of nonclassicality can be used to find practical and effective methods of generating and testing nonclassicality and, therefore, also quantum entanglement of optical fields. The results presented in my thesis can be divided into three main groups: 1. Finding operational and practical criteria to classify states in terms of nonclassicality and entanglement based on fundamental classical inequalities like Cauchy-Schwarz inequality. It was also shown how some known entanglement inequalities can be derived as nonclassicality inequalities or as sums of more than one inequality [Bartkowiak2010a]. 2. Describing properties and behaviour of quantum correlations for different optical fields (e.g. for multiand single-mode systems, for interacting and noninteracting modes). In particular, general occurrence of sudden vanishing of nonclassicality, which can be observed not only for twoor multimode but also for single-mode fields, was proven [Bartkowiak2011]. 3. Finding the methods of generating and testing of quantum correlations, which would be practical and easy to implement with available resources in both linear and nonlinear optics.
Distinguishing quantum states that admit a classical counterpart from those that exhibit nonclassicality has long been a central issue in quantum optics. Finding an implementable criterion certifying optical nonclassicality (i.e., the incompatibility with a statistical mixture of coherent states) is of major importance as it often is a prerequisite to quantum information processes. A hierarchy of conditions for detecting whether a quantum state exhibits optical nonclassicality can be written based on matrices of moments of the optical field [E. V. Shchukin and W. Vogel, Phys. Rev. A 72, 043808 (2005)]. Here, we design optical nonclassicality observables that act on several replicas of a quantum state and whose expectation value coincides with the determinant of these matrices, hence providing witnesses of optical nonclassicality that overcome the need for state tomography. These multicopy observables are used to construct a family of physically implementable schemes involving linear optical operations and photon number detectors.
We consider a way to generate operational inequalities to test nonclassicality (or quantumness) of multimode bosonic fields (or multiparty bosonic systems) that unifies the derivation of many known inequalities and allows to propose new ones. The nonclassicality criteria are based on Vogel's criterion corresponding to analyzing the positivity of multimode PPP functions or, equivalently, the positivity of matrices of expectation values of, e.g., creation and annihilation operators. We analyze not only monomials but also polynomial functions of such moments, which can sometimes enable simpler derivations of physically relevant inequalities. As an example, we derive various classical inequalities which can be violated only by nonclassical fields. In particular, we show how the criteria introduced here easily reduce to the well-known inequalities describing (a) multimode quadrature squeezing and its generalizations, including sum, difference, and principal squeezing; (b) two-mode one-time photon-number correlations, including sub-Poisson photon-number correlations and effects corresponding to violations of the Cauchy-Schwarz and Muirhead inequalities; (c) two-time single-mode photon-number correlations, including photon antibunching and hyperbunching; and (d) two- and three-mode quantum entanglement. Other simple inequalities for testing nonclassicality are also proposed. We have found some general relations between the nonclassicality and entanglement criteria, in particular those resulting from the Cauchy-Schwarz inequality. It is shown that some known entanglement inequalities can be derived as nonclassicality inequalities within our formalism, while some other known entanglement inequalities can be seen as sums of more than one inequality derived from the nonclassicality criterion. This approach enables a deeper analysis of the entanglement for a given nonclassicality.
Quantum features of correlated optical modes define a major aspect of the nonclassicality in quantized radiation fields. However, the phase-sensitive detection of a two-mode light field is restricted to interferometric setups and local intensity measurements. Even the full reconstruction of the quantum state of a single radiation mode relies on such detection layouts and the preparation of a well-defined reference light field. In this work, we establish the notion of the essential quantum correlations of two-mode light fields. It refers to those quantum correlations which are measurable by a given device, i.e., the accessible part of a nonclassical Glauber-Sudarshan phase-space distribution, which does not depend on a global phase. Assuming a simple four-port interferometer and photon-number-resolving detectors, we derive the reconstruction method and nonclassicality criteria based on the Laplace-transformed moment-generating function of the essential quasiprobability. With this technique, we demonstrate that the essential quantum correlations of a polarization tomography scheme are observable even if the detectors are imperfect and cannot truly resolve the photon statistics.
Quantum features of correlated optical modes define a major aspect of the nonclassicality in quantized radiation fields. However, the phase-sensitive detection of a two-mode light field is restricted to interferometric setups and local intensity measurements. Even the full reconstruction of the quantum state of a single radiation mode relies on such detection layouts and the preparation of a well-defined reference light field. In this work, we establish the notion of the essential quantum correlations of two-mode light fields. It refers to those quantum correlations which are measurable by a given device, i.e., the accessible part of a nonclassical Glauber-Sudarshan phase-space distribution, which does not depend on a global phase. Assuming a simple four-port interferometer and photon-number-resolving detectors, we derive the reconstruction method and nonclassicality criteria based on the Laplace-transformed moment-generating function of the essential quasiprobability. With this technique, we demonstrate that the essential quantum correlations of a polarization tomography scheme are observable even if the detectors are imperfect and cannot truly resolve the photon statistics.
One of the main foci of modern applied quantum information theory\nis the production of large-scale quantum entanglement involving many\nparticles, to achieve the next-generation quantum technologies. Although a full-scale quantum computer is still far away in time, in the next\nfew years we can expect to have quantum devices composed of up to a\nhundred controllable qubits. The primary challenge in moving towards\nsuch devices lies in the development of reliable and resource-efficient\ndetection techniques to prove genuine quantum advantage. The main\nobjective of this thesis is to investigate novel methods to detect the presence of quantum correlations in such systems, in particular, quantum\nentanglement and quantum nonlocality.\nThe first part of this thesis is dedicated to entanglement detection\nin large-scale quantum systems. Our main goal is to develop a novel\nprobabilistic method in which entanglement is seen as an ability of a\nquantum system to accomplish certain information-processing tasks.\nWe show that for certain classes of large (e.g. few tens of qubits) quantum states, even a single copy of a quantum state suffices to detect\nentanglement with a high confidence. Compared to the standard detection methods, this makes our method exceptionally resource-efficient.\nThe developed probabilistic scheme applies to multiple classes of states, vital for quantum computation, such as cluster states or ground\nstates of local Hamiltonians.\nIn the second part of this thesis, we develop a generic framework\nfor translating any entanglement witness into a resource-efficient probabilistic scheme. We show that the confidence level of entanglement\ndetection grows exponentially fast with the number of detection events,\nwhich makes this ansatz very efficient and reliable. Furthermore, we\npresent the first experimental performance of our method by verifying\nthe presence of entanglement in a photonic six-qubit cluster state.\nThe third part of this thesis describes the extension of our entanglement verification method to quantum nonlocality. Concrete examples\nare presented where we convert Bell’s inequalities into the probabilistic\nprocedure and incorporate our method into self-testing schemes. We\nshow that the performance of our method significantly exceeds the ability of the existing methods for detection of quantum nonlocality and\nself-testing.\nThe last part of this thesis is a study of the weak-convergence properties of random variables generated by quantum measurements. Beginning with a sequence of random variables generated by repeated\nunsharp quantum measurements, we study the limit distribution of\nmeasured relative frequency. We provide the de Finetti-type of representation theorem for all separable states, showing that the measured\ndistribution can be well approximated by a mixture of normal distributions. Additionally, we investigate the convergence rates and show\nthat the relative frequency converges to some constant at the rate of\norder 1=pN for all separable inputs. Finally, we provide an example of\na strictly unsharp quantum measurement where we obtain better scaling by using entangled inputs. We find such behaviour of entangled\nstates relevant for quantum information processing.
Abstract Recently, experimental demonstrations of the pair coherent state of microwave photons in superconducting cavities (PRX QUANTUM 4, 020319, 2023) and experimental results of photon addition and subtraction in multimode entangled optical fields (Physical Review Research 6, 013065, 2024) were reported. Motivated by these results, we study the nonclassical properties of non-Gaussian photon-added and subtracted pair coherent states. More specifically, we explore quantum polarization, quadrature squeezing, sum and difference squeezing, Shchukin-Vogel Entanglement, EPR entanglement correlation, two-mode higher-order antibunching, and quasiprobability distribution function (Q function). The effect of photon addition and subtraction is visible in this study with different parameters, as we compared our results with the original pair coherent state (PCS). This study provides a deeper understanding of the quantum behavior of modified pair coherent states, with potential implications for advancements in quantum optics and information processing.