Distinguishing quantum states that admit a classical counterpart from those that exhibit nonclassicality has long been a central issue in quantum optics. Finding an implementable criterion certifying optical nonclassicality (i.e., the incompatibility with a statistical mixture of coherent states) is of major importance as it often is a prerequisite to quantum information processes. A hierarchy of conditions for detecting whether a quantum state exhibits optical nonclassicality can be written based on matrices of moments of the optical field [E. V. Shchukin and W. Vogel, Phys. Rev. A 72, 043808 (2005)]. Here, we design optical nonclassicality observables that act on several replicas of a quantum state and whose expectation value coincides with the determinant of these matrices, hence providing witnesses of optical nonclassicality that overcome the need for state tomography. These multicopy observables are used to construct a family of physically implementable schemes involving linear optical operations and photon number detectors.
Distinguishing quantum states that admit a classical counterpart from those that exhibit nonclassicality has long been a central issue in quantum optics. Finding an implementable criterion certifying optical nonclassicality (i.e., the incompatibility with a statistical mixture of coherent states) is of major importance as it often is a prerequisite to quantum information processes. A hierarchy of conditions for detecting whether a quantum state exhibits optical nonclassicality can be written based on matrices of moments of the optical field [E. V. Shchukin and W. Vogel, Phys. Rev. A 72, 043808 (2005)]. Here, we design optical nonclassicality observables that act on several replicas of a quantum state and whose expectation value coincides with the determinant of these matrices, hence providing witnesses of optical nonclassicality that overcome the need for state tomography. These multicopy observables are used to construct a family of physically implementable schemes involving linear optical operations and photon number detectors.
One of the most relevant problems in the quantum theory is the question whether the appropriate state of the system can be described within a classical theory. The famous examples of nonclassical states are Schrodinger-cats states or entanglement states. In spite of many practical applications of entanglement as a special kind of nonclassicality (like quantum teleportation [1], dense coding [2], or implementation of super-fast [3] and fast algorithms [4]), we still have difficulties with describing and specifying it. One cannot find such an operational optimal method, which would allow us to maximally use the technological and scientific potential arising from the adaptation properties of quantum correlations. Thus, my thesis is focused on giving a proposal of a theoretical recipe for constructing experimentally achievable procedures for the study of quantum correlations. In my thesis I have focused on quantum correlations described in terms of nonclassicality (quantumness) and specific kind of it,i.e., entanglement. The nonclassicality definition, used by me in the thesis, is based on the Glauber-Sudarshan function (P -function). One can assume, that a state is nonclassical, if its P -function is negative or more singular than Dirac’s delta [5]. As follows, the state is nonclassical, when its P -function cannot be treated as a “real” probabilistic distribution. Based on specific properties of the P -function, Agarwal and Tara [6], as well as, Shchukin, Richter and Vogel [7, 8] proposed nonclassicality and entanglement [9] criteria based on matrices of moments of annihilation and creation operators. The operational procedures for analyzing nonclassicality and an efficient method for measuring such moments developed by Shchukin and Vogel [10] creates basis for my thesis. It can be seen that the nonclassicality criteria based on matrices of moments offer an effective way of deriving specific inequalities, which might be useful in the verification of nonclassicality of particular states generated in experiments. Therefore, criteria constructed based on the above definition of nonclassicality can be used to find practical and effective methods of generating and testing nonclassicality and, therefore, also quantum entanglement of optical fields. The results presented in my thesis can be divided into three main groups: 1. Finding operational and practical criteria to classify states in terms of nonclassicality and entanglement based on fundamental classical inequalities like Cauchy-Schwarz inequality. It was also shown how some known entanglement inequalities can be derived as nonclassicality inequalities or as sums of more than one inequality [Bartkowiak2010a]. 2. Describing properties and behaviour of quantum correlations for different optical fields (e.g. for multiand single-mode systems, for interacting and noninteracting modes). In particular, general occurrence of sudden vanishing of nonclassicality, which can be observed not only for twoor multimode but also for single-mode fields, was proven [Bartkowiak2011]. 3. Finding the methods of generating and testing of quantum correlations, which would be practical and easy to implement with available resources in both linear and nonlinear optics.
Nonclassicality, defined in the quantum optical sense, serves as a resource for photon-based quantum technologies. Therefore, certifying the nonclassicality of a quantum state is crucial for gauging its potential for quantum advantage. However, traditional nonclassicality witnesses that assume perfect knowledge of the witness observables often fail in realistic scenarios with limited statistics and finite-resolution photon detectors. Furthermore, these witnesses do not exploit the fact that certain states are unlikely to be observed in a given experiment. Here, we train a variational model to distinguish classical from nonclassical states using finitely many measurement samples of multimode quantum states that are probed with different photon-number-resolving detection schemes. The learned decision rule is then an indicator of nonclassicality, tailored to a given set of physically relevant states. Our approach is both data-driven and interpretable in the sense that the learned analytical decision rule can be extracted. Training the model on experimental data measured with (i) a superconducting nanowire single-photon detector and (ii) a time-bin multiplexing detection scheme demonstrates the versatility of the approach, paving the way for efficient nonclassicality detection.
Efficiently certifying non-Gaussian entanglement in continuous-variable quantum systems is a central challenge for advancing quantum information processing, photonic quantum computing, and metrology. Here, we put forward continuous-variable counterparts to the recently introduced entanglement criteria based on moments of the partially transposed state, together with simple readout schemes that require only a few replicas of the state, passive linear optics, and particle-number measurements. We develop a multicopy method that enables the detection of strongly non-Gaussian entanglement for various relevant state families overlooked by standard approaches, which include the entire class of NOON states. Further, it is robust against realistic experimental constraints (losses, noise, and finite statistics), which we demonstrate by extensive numerical simulations.
Quantum features of correlated optical modes define a major aspect of the nonclassicality in quantized radiation fields. However, the phase-sensitive detection of a two-mode light field is restricted to interferometric setups and local intensity measurements. Even the full reconstruction of the quantum state of a single radiation mode relies on such detection layouts and the preparation of a well-defined reference light field. In this work, we establish the notion of the essential quantum correlations of two-mode light fields. It refers to those quantum correlations which are measurable by a given device, i.e., the accessible part of a nonclassical Glauber-Sudarshan phase-space distribution, which does not depend on a global phase. Assuming a simple four-port interferometer and photon-number-resolving detectors, we derive the reconstruction method and nonclassicality criteria based on the Laplace-transformed moment-generating function of the essential quasiprobability. With this technique, we demonstrate that the essential quantum correlations of a polarization tomography scheme are observable even if the detectors are imperfect and cannot truly resolve the photon statistics.
We address the problem of constructing witnesses for nonclassical light that are applicable in state-of-the-art photon-counting devices. The key ingredient for the criteria we derive are generalized and directly measurable counting statistics and matrices of counting moments. Beyond common criteria, we find classes of witnesses that are based on half-integer powers of click moments and counts. Remarkably, this leads to an exponential increase of the number of nonclassicality criteria one can construct and apply. With this finding, special attention is payed to probing even and odd parity states, requiring such distinct witnesses. Our method is applicable to spatial and time-bin multiplexing in optical systems, where each spatial and temporal mode can be measured with both on-off detectors and detectors with partial internal quasi-photon-number resolution. Generalizations to multimode scenarios are provided, allowing for the direct measurement of nonclassical correlations and coincidence counts between an arbitrary number of modes.
Non-Gaussian quantum states of light are essential resources for quantum information processing and precision metrology. Among them, generalized coherent states (GCS), which naturally arise from the evolution of a coherent state with a nonlinear medium, exhibit useful quantum features such as Wigner negativity and metrological advantages [Phys. Rev. Res. 5, 013165 (2023)]. Because these states remain coherent to all orders, their nonclassical character cannot be revealed through standard intensity-intensity correlation measurements. Here, we demonstrate that the intensity-field correlation function alone provides a simple and experimentally accessible witness of nonclassicality. For GCSs, any deviation of this normalized correlation from unity signals nonclassical behavior. We derive analytical results for Kerr-generated states and extend the analysis to statistical mixtures of GCSs. The proposed approach enables real-time, low-complexity detection of quantum signatures in non-Gaussian states, offering a practical tool for experiments across a broad range of nonlinear regimes.