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Cambridge University Press eBooks

Quantum theory of the laser – density operator approach

Marlan O. Scully, Muhammad Suhail Zubairy

Published Sep 4, 1997• 2 citations
Publisher

Abstract

In Chapters 5 and 7 we presented a treatment of laser physics in which the light is described as a classical Maxwell field while the lasing medium is described as a collection of atoms whose dynamic evolution is governed by the Schrödinger equation. This semi-classical theory of laser behavior is sufficient to describe a rich variety of phenomena. However, there are many questions which require a fully quantized theory of the radiation. For example, the photon statistics and linewidth of the laser can be properly understood only via the full quantum theory of a laser. The laser linewidth is an important quantity. For example, it determines the fundamental limit of operation of an active ring laser gyroscope. The first fully quantized derivation of the laser linewidth general enough to include even the semiconductor laser linewidth problem utilized a quantum noise operator approach, and is presented in chapter 12. The photon statistical distribution for the laser is of interest for several reasons. Historically, it was initially thought by some that the statistical photon distribution should be a Bose–Einstein distribution. A little reflection shows that this can not be, since the laser is operating far from thermodynamic equilibrium. However, a different paradigm recognizes many atoms oscillating in phase produce what is essentially a classical current, and this would generate a coherent state; the statistics of which is Possionian. But, for example, the photon statistics of a typical Helium–Neon laser is substantially different from a Possionian distribution.

DOI
10.1017/cbo9780511813993.013

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In Chapters 5 and 7 we presented a treatment of laser physics in which the light is described as a classical Maxwell field while the lasing medium is described as a collection of atoms whose dynamic evolution is governed by the Schrödinger equation. This semi-classical theory of laser behavior is sufficient to describe a rich variety of phenomena. However, there are many questions which require a fully quantized theory of the radiation. For example, the photon statistics and linewidth of the laser can be properly understood only via the full quantum theory of a laser. The laser linewidth is an important quantity. For example, it determines the fundamental limit of operation of an active ring laser gyroscope. The first fully quantized derivation of the laser linewidth general enough to include even the semiconductor laser linewidth problem utilized a quantum noise operator approach, and is presented in chapter 12. The photon statistical distribution for the laser is of interest for several reasons. Historically, it was initially thought by some that the statistical photon distribution should be a Bose–Einstein distribution. A little reflection shows that this can not be, since the laser is operating far from thermodynamic equilibrium. However, a different paradigm recognizes many atoms oscillating in phase produce what is essentially a classical current, and this would generate a coherent state; the statistics of which is Possionian. But, for example, the photon statistics of a typical Helium–Neon laser is substantially different from a Possionian distribution.
In this chapter, we present a theory of the laser based on the Heisenberg–Langevin approach. This is a different, but completely equivalent approach to the density operator approach discussed in the previous chapter. In general, the density operator approach is better suited to study the photon statistics of the radiation field whereas the Heisenberg–Langevin approach has certain calculational advantages in the determination of phase diffusion coefficients, and consequently laser linewidth. In Section 12.1, a simple approach to determine laser linewidth based on a linear theory is presented. This analysis is especially interesting and useful in that it includes atomic memory effects, something that is difficult to do within a density matrix theory. In Sections 12.2–12.4, we consider the complete nonlinear theory of the laser and rederive all the important quantities related to the quantum statistical properties of the radiation field. A simple Langevin treatment of the laser linewidth including atomic memory effects† The full nonlinear quantum theory of the laser discussed in the previous chapter yields most of the interesting quantum statistical properties of the radiation field. In many problems of interest, however, we do not need such an elaborate treatment. For example, as we saw in the previous chapter, the natural linewidth of the laser can be determined from a linearized theory of the laser. That is, the full nonlinear theory serves to determine the amplitude of the field but the phase fluctuations about this operating point are described by a linear theory.
In Chap. 17 we developed the quantum theory of the laser obtaining in particular expressions for the laser photon statistics and linewidth. In this chapter we discuss and amplify those results in terms of measurement theory. Section 18-1 provides an overview of measurement theory as it applies to the quantum electric field. The discussion leads naturally into a specific discussion of the measurement of photon statistics and the laser linewidth. In Sec. 18-2 a heuristic model of a photodetector is presented with reveals how the photo­ electron statistics resulting from incident radiation is related to the photon statistics of that radiation, t In Sec. 18-3 we discuss the laser linewidth with the use of a simple two level atom beam much like that of Sec. 16-1. Our present discussion utilizes the density matrix technique throughout rather than the density matrix-state vector combination of Sec. 16-1. The laser spectrum “seen” by the atomic beam has, in fact, the same Lorentzian profile given in Sec. 17-3. In Sec. 18-4 the laser linewidth is discussed in terms of a quantum version of the classical correlation function <£(* -f t )E(t)y. In spite of the fact that two time correlations are apparently required, we show that a single time and solutions to the density operator equation of motion are sufficient. This reduction is an example of the so-called Onsager regression hypothesis, which shows how to proceed from single-time to multitime correlation functions.
Our treatment of the quantum theory of radiation so far has predominantly involved entire systems, such as the electromagnetic field in a cavity. In most areas of quantum optics, however, we are interested in only part of the entire system. For example, in the laser problem, we want to know the field but are not particularly interested in what happens to the atoms. We find it convenient to separate the system of primary interest from that (or those) of secondary interest and to call the former simply the “system” and the latter the “res­ ervoir.” We can eliminate the reservoir by using the reduced density operator method in the Schrodinger (or interaction) picture or the noise operator method in the Heisenberg picture. In this chapter we discuss the density operator method, which provides computational convenience while stressing the statistical aspects of the problem. In Chap. 19 we use the noise operator approach, which often requires more calculation but offers a direct physical appeal in its resemblance to the classical Brownian motion problem.
This chapter is devoted to coherent states. Generally speaking, a wave function of a system of identical particles does not have to have a certain number of particles. It can be a superposition of states with different numbers of particles. We have already encountered this in Chapters 5 and 6 when we studied superconductivity and superfluidity. Another important example of states with no well-defined number of particles is given by coherent states . In a way, these states are those which most resemble classical ones: the uncertainty in conjugated variables (such as position and momentum) is minimal for both variables, and their time-evolution is as close to classical trajectories as one can get. Coherent states of radiation are relatively easy to achieve. They arise if we excite the electromagnetic field with classical currents. We look in detail at the coherent state of a single-mode oscillator and all its properties. The coherent state turns out to be an eigenfunction of the annihilation operator, the distribution of photon numbers is Poissonian, and it provides an optimal wave function describing a classical electromagnetic wave. We come back to our simple model of the laser and critically revise it with our knowledge of coherent states, and estimate the time at which the laser retains its optical coherence. We then derive Maxwell–Bloch equations that combine the master equation approach to the lasing (as outlined in Chapter 9) with the concept of coherence.
A quantum statistical analysis of an optical maser is presented in generalization of the recent semiclassical theory of Lamb. Equations of motion for the density matrix of the quantized electromagnetic field are derived. These equations describe the irreversible dynamics of the laser radiation in all regions of operation (above, below, and at threshold). Nonlinearities play an essential role in this problem. The diagonal equations of motion for the radiation are found to have an apparent physical interpretation. At steady state, these equations may be solved via detailed-balance considerations to yield the photon statistical distribution ${\ensuremath{\rho}}_{n,n}$. The resulting distribution has a variance which is significantly larger than that for coherent light. The off-diagonal elements of the radiation density matrix describe the effects of phase diffusion in general and provide the spectral profile ${| E(\ensuremath{\omega}) |}^{2}$ as a special case. A detailed discussion of the physics involved in this paper is given in the concluding sections. The theory of the laser adds another example to the short list of solved problems in irreversible quantum statistical mechanics.
Chapter 6 begins by transforming the optical wave itself into a quantized form, and the full implications of the wave‐particle duality of Chapter 2 become clear. The electric field may be pictured as an infinite ladder of discrete states and this structure allows optical interactions to be described photon by photon. The origin of spontaneous emission emerges from this treatment as a transition process that is stimulated by electric field fluctuations of the vacuum, and Weisskopf–Wigner theory explains why it is irreversible. The subject of coherent states is introduced and intriguing possibilities outlined regarding the noise properties of components of these states that form different quadratures in terms of the optical phase. Next, statistical analysis of light fields is considered to serve as a basis for more quantitative comparisons of fields and their noise properties. Methods of calculating the first and second degrees of coherence are presented, and the ranges of values corresponding to “classical” versus “quantum” light sources are discussed. The reduced density matrix is developed to justify analysis that focuses on only certain aspects of optical dynamics while ignoring others, as an important tool for simplifying complex problems. Finally, in view of its historical importance, the problem of calculating the fluorescence spectrum of resonantly excited two‐level atoms is considered using both a method of moments and dressed atom theory.