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Physical Review

Quantum Theory of an Optical Maser. I. General Theory

Marlan O. Scully, Willis E. Lamb

Published Jul 10, 1967• 685 citations
Publisher

Abstract

A quantum statistical analysis of an optical maser is presented in generalization of the recent semiclassical theory of Lamb. Equations of motion for the density matrix of the quantized electromagnetic field are derived. These equations describe the irreversible dynamics of the laser radiation in all regions of operation (above, below, and at threshold). Nonlinearities play an essential role in this problem. The diagonal equations of motion for the radiation are found to have an apparent physical interpretation. At steady state, these equations may be solved via detailed-balance considerations to yield the photon statistical distribution ${\ensuremath{\rho}}_{n,n}$. The resulting distribution has a variance which is significantly larger than that for coherent light. The off-diagonal elements of the radiation density matrix describe the effects of phase diffusion in general and provide the spectral profile ${| E(\ensuremath{\omega}) |}^{2}$ as a special case. A detailed discussion of the physics involved in this paper is given in the concluding sections. The theory of the laser adds another example to the short list of solved problems in irreversible quantum statistical mechanics.

DOI
10.1103/physrev.159.208

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Cambridge University Press eBooks•Sep 4, 1997•2 citations
A quantum statistical analysis of an optical maser is presented in generalization of the recent semiclassical theory of Lamb. Equations of motion for the density matrix of the quantized electromagnetic field are derived. These equations describe the irreversible dynamics of the laser radiation in all regions of operation (above, below, and at threshold). Nonlinearities play an essential role in this problem. The diagonal equations of motion for the radiation are found to have an apparent physical interpretation. At steady state, these equations may be solved via detailed-balance considerations to yield the photon statistical distribution \ensuremathρn,n{\ensuremath{\rho}}_{n,n}\ensuremathρn,n​. The resulting distribution has a variance which is significantly larger than that for coherent light. The off-diagonal elements of the radiation density matrix describe the effects of phase diffusion in general and provide the spectral profile ∣E(\ensuremathω)∣2{| E(\ensuremath{\omega}) |}^{2}∣E(\ensuremathω)∣2 as a special case. A detailed discussion of the physics involved in this paper is given in the concluding sections. The theory of the laser adds another example to the short list of solved problems in irreversible quantum statistical mechanics.
In Paper I of this series, we derived equations of motion for a quantum-laser field interacting with atomic reservoirs. In the usual region of sustained oscillation, the off-diagonal elements of the radiation density matrix ${\ensuremath{\rho}}_{n,n+k}(t)$ were found to have an expontential decay associated with phase diffusion. In I we found the spectrum of the laser radiation by calculating the single time-ensemble average electric field implied by ${\ensuremath{\rho}}_{n,n+1}(t)$. This electric field was then treated as a classical variable whose Fourier analysis gave the spectrum. In the present paper, we establish the validity of this procedure by analyzing a simple model for a spectrometer. It is also shown that the same spectrum can be obtained from a two-time correlation function derived from the equations of motion.
We have solved a master equation to obtain the diagonal elements of the density matrix for laser light. The master equation represents a generalization of a master equation derived earlier for a single radiation mode interacting with NNN stationary two-level atoms. The generalization takes into account the pumping scheme which characterizes a three-level laser. For positive temperatures and a lossless cavity, the equilibrium solution of the master equation gives the correct statistical-mechanical description of the atoms and radiation. For negative temperatures, the distribution function for the number of photons in the mode is either exponential or peaked, depending on whether the laser is operating below or above threshold. The calculated intensity fluctuations are in good agreement with semiclassical results for lasers operating slightly above threshold.
We discuss the quantum theory of a simple model of a maser oscillator, consisting of one radiation-field mode interacting with a large number of stationary three-level atoms. The field and the atoms also interact with separate heat reservoirs which represent dissipation mechanisms and an incoherent pumping mechanism. The model is sufficiently simple that some analytical progress can be made with the nonlinear quantal equations before further approximation is necessary. We start from the quantal equation of motion of the field-atom density operator. We make immediate use of a diagonal coherent-state expansion for the field part of the density operator and a somewhat similar expansion for the atom part. This yields an exact equation of the Fokker-Planck form for a ccc-number weight distribution, which retains all the significance of the original operator equation, and which has the semiclassical equation for the same model as a first, fluctuation-free approximation. We make use of our basic Fokker-Planck equation in a variety of ways. We discuss the reduction of the equation under conditions that the atomic decay constants are large (large atomic linewidth), arriving finally at an equation of motion for a field-only weight function which serves to demonstrate the basic coherence properties of a maser. We derive and discuss the equation of motion of the generalized Wigner density for the maser model. The generalized Wigner density is a smoothed version (a convolution) of our basic weight distribution, and from it we derive an equivalent classical model including noise sources. Finally, we discuss other useful weight distributions and the number representation for the field. The equations we derive in these discussions make contact with the rate equations of Shimoda, Takahasi, and Townes, as well as with the more recent work of Lax and Louisell, Lax, and of Scully and Lamb.
We have solved a master equation to obtain the diagonal elements of the density matrix for laser light. The master equation represents a generalization of a master equation derived earlier for a single radiation mode interacting with NNN stationary two-level atoms. The generalization takes into account the pumping scheme which characterizes a three-level laser. For positive temperatures and a lossless cavity, the equilibrium solution of the master equation gives the correct statistical-mechanical description of the atoms and radiation. For negative temperatures, the distribution function for the number of photons in the mode is either exponential or peaked, depending on whether the laser is operating below or above threshold. The calculated intensity fluctuations are in good agreement with semiclassical results for lasers operating slightly above threshold.
The transient behavior of a laser is discussed using the quantum theory as did Scully and Lamb. The formal solution of the density-matrix equation is expressed in terms of exponentially decaying eigenmodes. Some of the lower decay constants are obtained numerically. The equations for the moments of the density matrix are then derived and solved by a truncation method. The equations of motion are integrated numerically for the case where the average number of photons in a laser cavity has the realistically large value 1.3 \ifmmode\times\else\texttimes\fi{} 105{10}^{5}105. An alternative Fokker-Planck-equation approach is discussed.
In Chapters 5 and 7 we presented a treatment of laser physics in which the light is described as a classical Maxwell field while the lasing medium is described as a collection of atoms whose dynamic evolution is governed by the Schrödinger equation. This semi-classical theory of laser behavior is sufficient to describe a rich variety of phenomena. However, there are many questions which require a fully quantized theory of the radiation. For example, the photon statistics and linewidth of the laser can be properly understood only via the full quantum theory of a laser. The laser linewidth is an important quantity. For example, it determines the fundamental limit of operation of an active ring laser gyroscope. The first fully quantized derivation of the laser linewidth general enough to include even the semiconductor laser linewidth problem utilized a quantum noise operator approach, and is presented in chapter 12. The photon statistical distribution for the laser is of interest for several reasons. Historically, it was initially thought by some that the statistical photon distribution should be a Bose–Einstein distribution. A little reflection shows that this can not be, since the laser is operating far from thermodynamic equilibrium. However, a different paradigm recognizes many atoms oscillating in phase produce what is essentially a classical current, and this would generate a coherent state; the statistics of which is Possionian. But, for example, the photon statistics of a typical Helium–Neon laser is substantially different from a Possionian distribution.