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Conference on Lasers and Electro-Optics

Photon-photon correlations from a resonantly driven quantum dot in a microcavity

Edward B. Flagg, Andreas Müller, John W. Robertson, Thai Tran, DENNIS GLENN DEPPE, Jaiyu Zhang, Wenquan Ma, Gregory J. Salamo, Chih-Kang Ken Shih

Published May 1, 2008• 0 citations
Publisher

Abstract

We demonstrate strongly driven resonance fluorescence from a single InGaAs quantum dot in a planar microcavity by measuring the coherent oscillations in the second-order correlation function, g(2)(t), of the photoluminescence.
DOI
10.1109/cleo.2008.4551959

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We show that resonance fluorescence, i.e., the resonant emission of a coherently driven two-level system, can be realized with a semiconductor quantum dot. The dot is embedded in a planar optical microcavity and excited in a waveguide mode so as to discriminate its emission from residual laser scattering. The transition from the weak to the strong excitation regime is characterized by the emergence of oscillations in the first-order correlation function of the fluorescence, g(tau), as measured by interferometry. The measurements correspond to a Mollow triplet with a Rabi splitting of up to 13.3 microeV. Second-order correlation measurements further confirm nonclassical light emission.
The time dependence of correlations between the photons emitted from a microcavity with an embedded quantum dot under incoherent pumping is studied theoretically. Analytic expressions for the second-order correlation function g (2)(t) are presented in strong and weak coupling regimes. The qualitative difference between the incoherent and coherent pumping schemes in the strong coupling case is revealed: under incoherent pumping, the correlation function demonstrates pronounced Rabi oscillations, but in the resonant pumping case, these oscillations are suppressed. At high incoherent pumping, the correlations decay monoexponentially. The decay time nonmonotonically depends on the pumping value and has a maximum corresponding to the self-quenching transition.
Next-generation information technology is expected to rely on discrete two-state quantum systems that can deterministically emit single photons. Quantum dots are mesoscopic (~10,000 atoms large) semiconductor islands grown in a host crystal of larger band-gap that make well-defined two-level quantum systems and are very attractive due to stability, record coherence times, and the possibility of integrating them into larger structures, such as optical microcavities. This work presents experimental progress towards understanding the coherent optical processes that occur in single quantum dots, particularly such phenomena that might be one day utilized for quantum communication applications. High resolution low temperature optical spectroscopy is used in conjunction with first order (amplitude) and second-order (intensity) correlation measurements of the emitted field. A novel technique is introduced that is capable of harvesting the fluorescence of single dots at the same frequency as the laser, previously impossible due to insurmountable scattering. This technique enables the observation, for the first time, of single quantum dot resonance fluorescence, in both the weak and strong excitation regimes, which forms the basis for deterministic generation of single photons. Guided by the rich theoretical description available from quantum optics with atoms we obtain insight into the complex dynamics of this driven system. Quantum dots confined to novel optical microcavities were further investigated using micro photoluminescence. An optical microcavity properly coupled to a two-level system can profoundly modify its emission characteristics via quantum electrodynamical effects, which are highly attractive for single photon sources. The all-epitaxial structures we probe are distinguished by a bulk morphology that overcomes the fragility problems of existing approaches, and provides high quality factors as well as small mode volumes. Lasing is obtained with larger strucutres. Additionally, isolation of individual dots is further realized in smaller cavities and the Purcell effect observed in time-resolved photon counting experiments.
The time dependence of the correlations between the photons, emitted from the microcavity with embedded quantum dot under incoherent pumping, is studied theoretically. Analytical expressions for the second-order correlation function g2(t) are presented in strong and weak coupling regimes. At moderate pumping the correlation function demonstrates Rabi oscillations, while at larger pumping it shows monoexponential decay. The decay time of the correlations nonmonotonously depends on the pumping value and has a maximum corresponding to the self-quenching transition.
Photon correlations in the emission of a resonantly driven quantum dot are investigated, accounting for the influence of the solid-state phonon environment. An analytical expression is derived for the second-order fluorescence intensity correlation function, from which regimes of correlated and uncorrelated photon emissions are predicted as the driving field is varied. Experiments to investigate this effect would provide valuable insight into quantum dot carrier-phonon dynamics and are feasible with current technology.
The Jaynes-Cummings model, describing the interaction between a single two-level system and a photonic mode, has been used to describe a large variety of systems, ranging from cavity quantum electrodynamics, trapped ions, to superconducting qubits coupled to resonators. Recently there has been renewed interest in studying the quantum strong-coupling (QSC) regime, where states with photon number greater than one are excited. This regime has been recently achieved in semiconductor nanostructures, where a quantum dot is trapped in a planar microcavity. Here we study the quantum strong-coupling regime by calculating its photoluminescence (PL) properties under a pulsed excitation. We discuss the changes in the PL as the QSC regime is reached, which transitions between a peak around the cavity resonance to a doublet. We particularly examine the variations of the PL in the time domain, under regimes of short and long pulse times relative to the microcavity decay time.