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Journal of Physics A Mathematical and Theoretical

Exactly solvable three-level quantum dissipative systems via bosonization of fermion gas-impurity models

Sol H. Jacobsen, Peter Jarvis

Published May 28, 2010• 4 citations
Publisher

Abstract

We study the relationship between one-dimensional fermion gas-impurity models and quantum dissipative systems, via the method of constructive bosonization and unitary transformation. Starting from an anisotropic Coqblin–Schrieffer model, a new, exactly solvable, three-level quantum dissipative system is derived as a generalization of the standard spin- spin-boson model. The new system has two environmental oscillator baths with ohmic coupling, and admits arbitrary detuning between the three levels. All tunnelling matrix elements are equal, up to one complex phase which is itself a function of the longitudinal and transverse couplings in the integrable limit. Our work underlines the importance of re-examining the detailed structure of fermion-gas impurity models and spin chains, in the light of connections to models for quantum dissipative systems.

DOI
10.1088/1751-8113/43/25/255305

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We study the relationship between one-dimensional fermion gas-impurity models and quantum dissipative systems, via the method of constructive bosonization and unitary transformation. Starting from an anisotropic Coqblin–Schrieffer model, a new, exactly solvable, three-level quantum dissipative system is derived as a generalization of the standard spin- spin-boson model. The new system has two environmental oscillator baths with ohmic coupling, and admits arbitrary detuning between the three levels. All tunnelling matrix elements are equal, up to one complex phase which is itself a function of the longitudinal and transverse couplings in the integrable limit. Our work underlines the importance of re-examining the detailed structure of fermion-gas impurity models and spin chains, in the light of connections to models for quantum dissipative systems.
We study the relationship between one-dimensional fermion gas-impurity models and quantum dissipative systems, via the method of constructive bosonisation and unitary transformation. Starting from an anisotropic Coqblin-Schrieffer model, a new, exactly solvable, three-level quantum dissipative system is derived as a generalisation of the standard spin-half spin-boson model. The new system has two environmental oscillator baths with ohmic coupling, and admits arbitrary detuning between the three levels. All tunnelling matrix elements are equal, up to one complex phase which is itself a function of the longitudinal and transverse couplings in the integrable limit. Our work underlines the importance of re-examining the detailed structure of fermion-gas impurity models and spin chains, in the light of connections to models for quantum dissipative systems.
We summarize in this work the relations of the spin-boson Hamiltonian, which was recently studied in connection with the phenomenon of quantum coherence in the presence of dissipation, to three different fermionic Hamiltonians. These relations were obtained through well-known equivalences between Fermi and Bose operators in one dimension. The fermionic Hamiltonians correspond to (a) a two-level system coupled linearly with a fermionic bath, (b) the resonant-level model, and (c) the anisotropic Kondo model. For the first Hamiltonian we reobtain and discuss the relationship between the dimensionless dissipation coefficient \ensuremath{\alpha} and the phase shift of the fermions. The resonant-level model allows us to study the properties of the two-level system for values of \ensuremath{\alpha} around (1/2). At \ensuremath{\alpha}=(1/2) the model reduces to the Toulouse limit, where the Hamiltonian is exactly soluble. A pure exponential decay is obtained for the relaxation of P(t)=〈${\ensuremath{\sigma}}_{z}$(t)〉 for t>0, given that for t<0 the system is known to be localized in one of the two states. The comparison with the Kondo model gives the long-time-limit behavior of the system for (1/2)1 and provides a connection between universal numbers obtained previously for the spin-boson Hamiltonian and the Kondo model.
We study the elliptic spin-1/2 Kondo model (spin-1/2 fermions in one dimension with fully anisotropic contact interactions with a magnetic impurity) in the light of mappings to bosonic systems using the fermion-boson correspondence and associated unitary transformations. We show that for fixed fermion number, the bosonic system describes a two-level quantum dissipative system with two noninteracting copies of infinitely-degenerate upper and lower levels. In addition to the standard tunnelling transitions, and the transitions driven by the dissipative coupling, there are also bath-mediated transitions between the upper and lower states which simultaneously effect shifts in the horizontal degeneracy label. We speculate that these systems could provide new examples of continuous time quantum random walks, which are exactly solvable.
Dissipative processes in nonequilibrium many-body systems are fundamentally different than their equilibrium counterparts. Such processes are of great importance for the understanding of relaxation in single-molecule devices. As a detailed case study, we investigate here a generic spin-fermion model, where a two-level system couples to two metallic leads with different chemical potentials. We present results for the spin relaxation rate in the nonadiabatic limit for an arbitrary coupling to the leads using both analytical and exact numerical methods. The nonequilibrium dynamics is reflected by an exponential relaxation at long times and via complex phase shifts, leading in some cases to an ``antiorthogonality'' effect. In the limit of strong system-lead coupling at zero temperature we demonstrate the onset of a Marcus-like Gaussian decay with voltage difference activation. This is analogous to the equilibrium spin-boson model, where at strong coupling and high temperatures, the spin excitation rate manifests temperature activated Gaussian behavior. We find that there is no simple linear relationship between the role of the temperature in the bosonic system and a voltage drop in a nonequilibrium electronic case. The two models also differ by the orthogonality-catastrophe factor existing in a fermionic system, which modifies the resulting line shapes. Implications for current characteristics are discussed. We demonstrate the violation of pairwise Coulomb gas behavior for strong coupling to the leads. The results presented in this paper form the basis of an exact, nonperturbative description of steady-state quantum dissipative systems.
We extend a standard stochastic theory to study open quantum systems coupled to a generic quantum environment. We exemplify the general framework by studying a two-level quantum system coupled bilinearly to the three fundamental classes of non-interacting particles: bosons, fermions, and spins. In this unified stochastic approach, the generalized stochastic Liouville equation (SLE) formally captures the exact quantum dissipations when noise variables with appropriate statistics for different bath models are applied. Anharmonic effects of a non-Gaussian bath are precisely encoded in the bath multi-time correlation functions that noise variables have to satisfy. Starting from the SLE, we devise a family of generalized hierarchical equations by averaging out the noise variables and expand bath multi-time correlation functions in a complete basis of orthonormal functions. The general hierarchical equations constitute systems of linear equations that provide numerically exact simulations of quantum dynamics. For bosonic bath models, our general hierarchical equation of motion reduces exactly to an extended version of hierarchical equation of motion which allows efficient simulation for arbitrary spectral densities and temperature regimes. Similar efficiency and flexibility can be achieved for the fermionic bath models within our formalism. The spin bath models can be simulated with two complementary approaches in the present formalism. (I) They can be viewed as an example of non-Gaussian bath models and be directly handled with the general hierarchical equation approach given their multi-time correlation functions. (II) Alternatively, each bath spin can be first mapped onto a pair of fermions and be treated as fermionic environments within the present formalism.
Recent work is reviewed on continuous quantum phase transitions in impurity models, both with fermionic and bosonic baths – these transitions are interesting realizations of boundary critical phenomena at zero temperature. The models with fermion bath are generalizations of the standard Kondo model, with the common feature that Kondo screening of the localized spin can be suppressed due to competing processes. The models with boson bath are related to the spin–boson model of dissipative two-level systems, where the interplay between tunneling and friction results in multiple phases. The competition inherent to all models can generate unstable fixed points associated with quantum phase transitions, where the impurity properties undergo qualitative changes. Interestingly, certain impurity transitions feature both lower-critical and upper-critical “dimensions” and allow for epsilon-type expansions. Results are presented for a number of observables, obtained by both analytical and numerical renormalization group techniques, and connections made to experiments.