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Physical review. B, Condensed matter

Bosonization of a two-level system with dissipation

F. Guinea, Vincent Hakim, A. Muramatsu

Published Oct 1, 1985• 173 citations
Publisher

Abstract

We summarize in this work the relations of the spin-boson Hamiltonian, which was recently studied in connection with the phenomenon of quantum coherence in the presence of dissipation, to three different fermionic Hamiltonians. These relations were obtained through well-known equivalences between Fermi and Bose operators in one dimension. The fermionic Hamiltonians correspond to (a) a two-level system coupled linearly with a fermionic bath, (b) the resonant-level model, and (c) the anisotropic Kondo model. For the first Hamiltonian we reobtain and discuss the relationship between the dimensionless dissipation coefficient \ensuremath{\alpha} and the phase shift of the fermions. The resonant-level model allows us to study the properties of the two-level system for values of \ensuremath{\alpha} around (1/2). At \ensuremath{\alpha}=(1/2) the model reduces to the Toulouse limit, where the Hamiltonian is exactly soluble. A pure exponential decay is obtained for the relaxation of P(t)=〈${\ensuremath{\sigma}}_{z}$(t)〉 for t>0, given that for t<0 the system is known to be localized in one of the two states. The comparison with the Kondo model gives the long-time-limit behavior of the system for (1/2)1 and provides a connection between universal numbers obtained previously for the spin-boson Hamiltonian and the Kondo model.

DOI
10.1103/physrevb.32.4410

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We summarize in this work the relations of the spin-boson Hamiltonian, which was recently studied in connection with the phenomenon of quantum coherence in the presence of dissipation, to three different fermionic Hamiltonians. These relations were obtained through well-known equivalences between Fermi and Bose operators in one dimension. The fermionic Hamiltonians correspond to (a) a two-level system coupled linearly with a fermionic bath, (b) the resonant-level model, and (c) the anisotropic Kondo model. For the first Hamiltonian we reobtain and discuss the relationship between the dimensionless dissipation coefficient \ensuremath{\alpha} and the phase shift of the fermions. The resonant-level model allows us to study the properties of the two-level system for values of \ensuremath{\alpha} around (1/2). At \ensuremath{\alpha}=(1/2) the model reduces to the Toulouse limit, where the Hamiltonian is exactly soluble. A pure exponential decay is obtained for the relaxation of P(t)=〈\ensuremathσz{\ensuremath{\sigma}}_{z}\ensuremathσz​(t)〉 for t>0, given that for t<0 the system is known to be localized in one of the two states. The comparison with the Kondo model gives the long-time-limit behavior of the system for (1/2)1 and provides a connection between universal numbers obtained previously for the spin-boson Hamiltonian and the Kondo model.
We study the elliptic spin-1/2 Kondo model (spin-1/2 fermions in one dimension with fully anisotropic contact interactions with a magnetic impurity) in the light of mappings to bosonic systems using the fermion-boson correspondence and associated unitary transformations. We show that for fixed fermion number, the bosonic system describes a two-level quantum dissipative system with two noninteracting copies of infinitely-degenerate upper and lower levels. In addition to the standard tunnelling transitions, and the transitions driven by the dissipative coupling, there are also bath-mediated transitions between the upper and lower states which simultaneously effect shifts in the horizontal degeneracy label. We speculate that these systems could provide new examples of continuous time quantum random walks, which are exactly solvable.
We study the relationship between one-dimensional fermion gas-impurity models and quantum dissipative systems, via the method of constructive bosonization and unitary transformation. Starting from an anisotropic Coqblin–Schrieffer model, a new, exactly solvable, three-level quantum dissipative system is derived as a generalization of the standard spin- spin-boson model. The new system has two environmental oscillator baths with ohmic coupling, and admits arbitrary detuning between the three levels. All tunnelling matrix elements are equal, up to one complex phase which is itself a function of the longitudinal and transverse couplings in the integrable limit. Our work underlines the importance of re-examining the detailed structure of fermion-gas impurity models and spin chains, in the light of connections to models for quantum dissipative systems.
We study a spinless level that hybridizes with a fermionic band and is also coupled via its charge to a dissipative bosonic bath. We consider the general case of a power-law hybridization function $\ensuremath{\Gamma}(\ensuremath{\omega})\ensuremath{\propto}{\ensuremath{\mid}\ensuremath{\omega}\ensuremath{\mid}}^{r}$, with $r\ensuremath{\geqslant}0$, and a bosonic-bath spectral function $B(\ensuremath{\omega})\ensuremath{\propto}{\ensuremath{\omega}}^{s}$, with $s\ensuremath{\geqslant}\ensuremath{-}1$. For r<1r<1r<1 and $\mathrm{max}(0,2r\ensuremath{-}1)<s<1$, this Bose-Fermi quantum impurity model features a continuous zero-temperature transition between a delocalized phase, with tunneling between the impurity level and the band, and a localized phase, in which dissipation suppresses tunneling in the low-energy limit. The phase diagram and the critical behavior of the model are elucidated using perturbative and numerical renormalization-group techniques, between which there is excellent agreement in the appropriate regimes. For r=0r=0r=0, this model's critical properties coincide with those of the spin-boson and Ising Bose-Fermi Kondo models, as expected from bosonization.
Dissipative processes in nonequilibrium many-body systems are fundamentally different than their equilibrium counterparts. Such processes are of great importance for the understanding of relaxation in single-molecule devices. As a detailed case study, we investigate here a generic spin-fermion model, where a two-level system couples to two metallic leads with different chemical potentials. We present results for the spin relaxation rate in the nonadiabatic limit for an arbitrary coupling to the leads using both analytical and exact numerical methods. The nonequilibrium dynamics is reflected by an exponential relaxation at long times and via complex phase shifts, leading in some cases to an ``antiorthogonality'' effect. In the limit of strong system-lead coupling at zero temperature we demonstrate the onset of a Marcus-like Gaussian decay with voltage difference activation. This is analogous to the equilibrium spin-boson model, where at strong coupling and high temperatures, the spin excitation rate manifests temperature activated Gaussian behavior. We find that there is no simple linear relationship between the role of the temperature in the bosonic system and a voltage drop in a nonequilibrium electronic case. The two models also differ by the orthogonality-catastrophe factor existing in a fermionic system, which modifies the resulting line shapes. Implications for current characteristics are discussed. We demonstrate the violation of pairwise Coulomb gas behavior for strong coupling to the leads. The results presented in this paper form the basis of an exact, nonperturbative description of steady-state quantum dissipative systems.
We study the relationship between one-dimensional fermion gas-impurity models and quantum dissipative systems, via the method of constructive bosonisation and unitary transformation. Starting from an anisotropic Coqblin-Schrieffer model, a new, exactly solvable, three-level quantum dissipative system is derived as a generalisation of the standard spin-half spin-boson model. The new system has two environmental oscillator baths with ohmic coupling, and admits arbitrary detuning between the three levels. All tunnelling matrix elements are equal, up to one complex phase which is itself a function of the longitudinal and transverse couplings in the integrable limit. Our work underlines the importance of re-examining the detailed structure of fermion-gas impurity models and spin chains, in the light of connections to models for quantum dissipative systems.
Based on the recent paper [Phys. Rev. Lett. 102, 216803 (2009)], we study the nonequilibrium occupation number nd{n}_{d}nd​ and charge susceptibility $\ensuremath{\chi}$ of a resonance level close to dissipative quantum phase transition of the Kosterlitz-Thouless (KT) type between a delocalized phase for weak dissipation and a localized phase for strong dissipation. The resonance level is coupled to two spinless fermionic baths with a finite bias voltage and an Ohmic bosonic bath representing the dissipative environment. The system is equivalent to an effective anisotropic Kondo model out of equilibrium. Within the nonequilibrium renormalization-group approach, we calculate nonequilibrium magnetization MMM and spin susceptibility $\ensuremath{\chi}$ in the effective Kondo model, corresponding to $2{n}_{d}\ensuremath{-}1$ and $\ensuremath{\chi}$ of a resonance level, respectively. We demonstrate the smearing of the KT transition in the nonequilibrium magnetization MMM as a function of the effective anisotropic Kondo couplings, in contrast to a perfect jump in MMM at the transition in equilibrium. In the limit of large bias voltages, we find MMM and $\ensuremath{\chi}$ at the KT transition and in the localized phase show deviations from the equilibrium Curie-law behavior. As the system gets deeper in the localized phase, both ${n}_{d}\ensuremath{-}1/2$ and $\ensuremath{\chi}$ decrease more rapidly to zero with increasing bias voltages.