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Quantum Electronics and Laser Science Conference

Alignment of neutral molecules by a strong laser field

Hirofumi Sakai, C. P. Safvan, Jakob Juul Larsen, K.M. Hilligsøe, Kathrine Hald, Henrik Stapelfeldt

Published Jan 20, 2003• 2 citations
Publisher

Abstract

Summary form only given. The use of cw lasers to manipulate the external degrees of freedom of atoms is a central subject of atomic physics. Here, we report experimental evidence that a strong, nonresonant, linearly polarized, laser pulse can align a sample of neutral molecules without causing ionization or dissociation.
DOI
10.1109/qels.1999.807468

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Reflection of neutral atoms and molecules by a pulsed standing wave with a duration on the order of nanoseconds is studied. It is shown that, with a suitable choice of the laser parameter values, each period of the standing-wave pattern functions as an independent mirror, thus providing a novel way to manipulate large samples of neutral gas-phase particles even with a single laser pulse. At moderate field intensities, the pulsed standing-wave mirror would be directly applicable, e.g., for the manipulation of buffer-gas cooled molecules.
The forces felt by atoms when illuminated with resonant radiation can reduce their velocity dispersion and confine them in a region of space for further probing and experimentation. The forces can be dissipative or conservative and allow manipulations of the external degrees of freedom of atoms and small neutral particles. Laser cooling and trapping is now an important tool for many spectroscopic studies. It enhances the density of atoms in phase space by many orders of magnitude reducing the need of large samples. These lecture notes review the fundamental principles of the field and show some of the applications to the study of the spectroscopy of radioactive atoms. 1
We measure the role of field-induced alignment on the dipole force for molecules using a single focused nonresonant laser beam. We show that through the alignment process we can modify the effective polarizability by field polarization and thus control the center-of-mass motion of the molecule. We observe a maximum change of 2020%20 in the dipole force on CS2{}_{2}2​ molecules when changing from linearly to circularly polarized light. Additionally, the effect of the dipole force on different vibrational states is also studied.
Summary form only given. Optical manipulation of atoms is a well-developed and established field. Its successful use of resonant processes is difficult to mimic for molecules due to the complexity of the molecular energy spectra. However, intense non-resonant fields can provide forces similar to or even stronger than the resonant weak fields used in atom optics. These forces, long utilized in the manipulation of microscopic particles, were recently demonstrated for molecules in optical deflection and trapping experiments. We propose to use strong infrared laser field to create an "optical twister" a field that would exert very large optical torques on anisotropic molecules, leading to a controlled molecular rotation induced with a simple pulse. Molecular dissociation via rotations is used to demonstrate our method. The scheme distinguishes molecules with different moments of inertia, and thus acts as an optical centrifuge.
We report on the ability to tailor the optical dipole force for molecules by tuning their effective polarizability with strong field alignment using polarized fields. We have measured a difference of 20% in the dipole force on cold CS2 molecules when changing from linear to near-circular polarization using peak field intensities of 5.7x10(11) W cm(-2). A variation in the focal length with laser polarization of a molecular-optical lens formed by a single focused laser beam was also measured. This provides a new way of modifying this force for many molecules.
A strong inhomogeneous static electric field is used to spatially disperse a supersonic beam of polar molecules, according to their quantum state. We show that the molecules residing in the lowest-lying rotational states can be selected and used as targets for further experiments. As an illustration, we demonstrate an unprecedented degree of laser-induced one-dimensional alignment (cos;(2)theta_(2D)=0.97) and strong orientation of state-selected iodobenzene molecules. This method should enable experiments on pure samples of polar molecules in their rotational ground state, offering new opportunities in molecular science.