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Physical Review Letters

Pulsed Standing-Wave Mirror for Neutral Atoms and Molecules

Pasi Ryytty, M. Kaivola

Published May 29, 2000• 14 citations
Publisher

Abstract

Reflection of neutral atoms and molecules by a pulsed standing wave with a duration on the order of nanoseconds is studied. It is shown that, with a suitable choice of the laser parameter values, each period of the standing-wave pattern functions as an independent mirror, thus providing a novel way to manipulate large samples of neutral gas-phase particles even with a single laser pulse. At moderate field intensities, the pulsed standing-wave mirror would be directly applicable, e.g., for the manipulation of buffer-gas cooled molecules.

DOI
10.1103/physrevlett.84.5074

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Quantum Electronics•Apr 30, 1994•1 citation
Reflection of neutral atoms and molecules by a pulsed standing wave with a duration on the order of nanoseconds is studied. It is shown that, with a suitable choice of the laser parameter values, each period of the standing-wave pattern functions as an independent mirror, thus providing a novel way to manipulate large samples of neutral gas-phase particles even with a single laser pulse. At moderate field intensities, the pulsed standing-wave mirror would be directly applicable, e.g., for the manipulation of buffer-gas cooled molecules.
In this thesis, the use of pulsed laser fields to control the center-of-mass motion of neutral atoms and molecules is studied both numerically and experimentally. In particular, we consider the use of a pulsed standing wave for the deflection of atomic beams, and develop novel types of mirrors for applications in atom and molecule optics. The research work shows that pulsed laser fields can be applied to form efficient mirrors for neutral particles regardless of the details of their internal energy-level structure. Moreover, it is shown that pulsed standing waves can also be utilized to efficiently deflect atomic beams. In the first part of the thesis, we study the effects of phase fluctuations of the laser field on the momentum distribution of atoms after interaction with a standing wave. Our numerical simulations show that the coherence properties of the laser field play a major role in diffraction of atoms, especially when using pulsed lasers. It turns out that the effects caused by the limited coherence time of the optical field are clearly observable as a transfer of atoms in momentum space to the region around zero momentum rather than to high momentum states. The numerical analysis of the pulsed standing-wave diffraction was complemented by experimental measurements of the deflection profiles of a beam of thermal sodium atoms. The experimental distributions were measured for a value of the coherence time intermediate between the Rabi period and the interaction time. A comparison of the results with an expected distribution calculated for a fully coherent interaction shows that the phase fluctuations of the light field drastically affect the achievable transverse momentum values. Based on our theoretical and experimental analysis of the diffraction profiles, we conclude that large deflection angles can be reached only when laser pulses with a Fourier-limited bandwidth are applied. The second part of the thesis concentrates on the development of pulsed mirrors for neutral atoms and molecules. In particular, we consider the use of an evanescent wave, formed in total internal reflection of light on a vacuum-dielectric interface, and of a standing wave as possible mirror configurations. Our numerical simulations of the pulsed evanescent-wave mirror show that atoms with initial velocities up to several tens of meters per second can be reflected already at the moderate field intensities of a few tens of MW/cm2. This allows pulsed evanescent waves to be applied in a compact setup to control the motion of thermal atomic beams, for which the traditional atom mirrors are suited only at grazing incidence. However, since the effective interaction volume of the atomic beam and the laser field is limited by the short decay length of the evanescent wave, only a relatively small number of atoms can be reflected with a single laser pulse. Furthermore, the reflection is always inelastic, since the force exerted on the atoms varies as a function of the initial position of the particles. To solve the above problem we consider the use of a standing wave as a pulsed mirror for atoms. Our numerical simulations show that with a proper choice of the pulse duration and field intensity, each period of the standing-wave pattern functions as an elastic mirror for particles with an initial kinetic energy below the depth of the standing-wave potential. Hence, the standing-wave pattern acts as a long row of independent atom mirrors, which provides a novel route to controlling large volumes of fast atoms even with a single laser pulse. As a second application for the pulsed standing-wave mirror we consider the reflection of slow molecules, for which no efficient mirror configuration previously has been available. It is shown that pulsed standing waves of nonresonant frequencies can be used to efficiently manipulate large volumes of rotationally cold molecules. With a suitable choice of the parameter values, the molecules can be reflected nearly elastically, or with a tailored momentum distribution. This opens up a possibility to use the pulsed standing-wave mirror to control the motion of particles in various applications of atomic and molecular physics. Such a mirror could be applied, for example, to steer and image molecular beams, separate molecular species, and to form pulsed molecular beams.
A matter wave mirror using a single, pulsed, super-Gaussian (SG) optical beam for specular reflection of neutral ground-state molecules is studied. The mirror has a high reflectivity close to 100% and nearly perfect specular reflection over a large incident angle. This mirror avoids the usual problems due to surface roughness and the van der Waals interactions that occur in conventional atomic mirrors. Further, it is capable of reflectance and transmittance with applications to velocity filtering and deceleration of cold molecules.
In this paper we present some new results concerning the observed anomalous frequency properties of the process of the neutral atom scattering in the standing light wave field near the reflecting mirror. The investigations were carried out using the method of scattering of the sodium atomic strip beam, intersecting at right angle the region of the standing light wave field. The standing light wave field was formed by two counterpropagating waves of resonant laser radiation -- incident and reflected from the mirror, mounted at a distance of about 1 cm from the atomic beam. The coherence length of the laser radiation was about 10 cm, that's why the interaction of atoms with the field of two counterpropagating light waves was coherent. The width of the strip atomic beam (a equals 0.02 cm) was much less than the distance to the mirror. The specific feature of the given setup is the use of pulsed laser radiation with the duration (tau) less than 1/(gamma) ((gamma) -1- the time of resonant level spontaneous decay), so the atoms are scattered only due to the induced light pressure force. In this paper the detailed investigation of the distance R influence on the scattering process was carried out. With this purpose the mirror was mounted at different distances from the atomic beam. (truncated)
Laser induced strong-field phenomena in atoms and molecules on the femtosecond (fs) time scale have been almost exclusively investigated with traveling wave fields. In almost all cases, approximation of the strong electromagnetic field by an electric field purely oscillating in time suffices to describe experimental observations. Spatially dependent electromagnetic fields, as they occur in a standing light wave, allow for strong energy and momentum transfer and are expected to extend strong-field dynamics profoundly. Here we report a strong-field version of the Kapitza-Dirac effect for neutral atoms where we scatter neutral He atoms in an intense short pulse standing light wave with fs duration and intensities well in the strong-field tunneling regime. We observe substantial longitudinal momentum transfer concomitant with an unprecedented atomic photon scattering rate greater than 10(16)s(-1).
The scattering of neutral sodium atoms by a strong field of two counterpropagating (incident on and reflected from a mirror) short laser pulses was used in an experimental investigation of a stimulated radiation pressure. The reasons for the anomalous frequency structure in the scattering of atoms were identified. The oscillatory nature of the dependence of the scattering on the detuning from resonance was found to be significant in strong laser radiation fields. The oscillation period depended on the distance between the reflecting mirror and the atomic beam.