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Journal of Physics Conference Series

Fluorescence of surface adsorbed dyes: investigation of a new detector for molecule interferometry

Fabienne Goldfarb, Sarayut Deachapunya, André Stefanov, Alexander Stibor, Elisabeth Reiger, Markus Arndt

Published Jan 1, 2005• 0 citations
Publisher

Abstract

Matter-wave interferometry with large molecules is partially limited by the inefficiency of the commonly used ionization detection schemes. Here we discuss the possibility of employing a surface imaging method in which molecular interferograms with periods in the micron range are adsorbed on a surface and subsequently read using fluorescence microscopy. Our preliminary experiments show that the detection efficiency can be significantly increased compared to electron impact ionization and quadrupole mass spectrometry. However the interpretation of fluorescent molecular patterns requires a good understanding and control of the molecular mobility, the bleaching behavior, and the coverage dependence of the fluorescence intensity.

DOI
10.1088/1742-6596/19/1/021

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Imaging of surface adsorbed molecules is investigated as a novel detection method for matter wave interferometry with fluorescent particles. Mechanically magnified fluorescence imaging turns out to be an excellent tool for recording quantum interference patterns. It has a good sensitivity and yields patterns of high visibility. The spatial resolution of this technique is only determined by the Talbot gratings and can exceed the optical resolution limit by an order of magnitude. A unique advantage of this approach is its scalability: for certain classes of nano-sized objects, the detection sensitivity will even increase significantly with increasing size of the particle.
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