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Canadian Journal of Physics

Local driving field and the existence of a coherent mode in a system of driven two-level atoms

Haider R. Zaidi

Published Jan 1, 1985• 0 citations
Publisher

Abstract

Using a diagram technique, the equations of motion for the density matrix and the field inside the medium are derived for a system of driven two-level atoms. It is pointed out that these equations do not necessarily imply that the local driving field is perfectly coherent even if the external field is. In fact, by calculating the emission spectrum, it is shown that the coherent-scattering component acquires a small nonzero width in the strong-field region. It is concluded that the local driving field is only quasi-coherent. The physical origin of this effect lies in the peculiar nature of resonant interaction between two atoms. The results are compared with the previously obtained results for the foreign gas broadening type of collisions. It is found that there are qualitative as well as quantitative differences between the two results.

DOI
10.1139/p85-019

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Using a diagram technique, the equations of motion for the density matrix and the field inside the medium are derived for a system of driven two-level atoms. It is pointed out that these equations do not necessarily imply that the local driving field is perfectly coherent even if the external field is. In fact, by calculating the emission spectrum, it is shown that the coherent-scattering component acquires a small nonzero width in the strong-field region. It is concluded that the local driving field is only quasi-coherent. The physical origin of this effect lies in the peculiar nature of resonant interaction between two atoms. The results are compared with the previously obtained results for the foreign gas broadening type of collisions. It is found that there are qualitative as well as quantitative differences between the two results.
A theory of resonant light scattering from two level atoms in a gas is developed for an arbitrarily strong pump field. The Doppler effect and two body foreign gas collisions are considered. Elastic, inelastic (upward and downward), and the velocity changing collisions are retained in the general formulation. The impact approximation is not made, and the expressions for all (field dependent) collision rates are generated internally. Particular attention is paid to the lower state interaction, and a more complete parameterization of the theory is achieved. The general theory is non-Markovian and the quantum regression theorem is not used; it reduces to existing theories in special cases. It is shown that the coherent scattering is not a general property of the system if the lower state interaction is present; the "coherent" component acquires a small, but nonzero, width in the strong field region. This width could provide information about some new collision parameters.
The response of a collision-broadened gas sample to driving coherent radiation is studied theoretically, taking into account effects of coherent excitations of two or more atoms (or molecules). In analogy to the Bloch-type master equation for one-atom coherences, describing the motion of a single atom "dressed" by the relevant (incident and detected) field modes, a master equation is derived for two-atom coherences, including an effective interaction of the Bethe-Salpeter---type, accounting for the mutual interaction of the coherently driven pair. The master equation includes also all symmetrization effects owing to resonance exchange between identical atoms, and is limited to nonreactive gas atoms (or molecules) undergoing binary collisions, including otherwise all (internal and translational) relaxation effects. The self-energy kernels are expressed in a nonperturbative fashion, in terms of binary-collision scattering amplitudes, and include renormalization effects due to coincidence of radiative couplings with the collisions (optical and radiative collisions). The concept of two-atom coherences is generalized to higher coherence ranks by constructing a hierarchy of master equations, including vertex operators that upgrade or downgrade the coherence rank, as a prelude to a diagrammatic method for calculating continuous-wave spectra. This hierarchy is compared with prevalent Agarwal-type master equations, based on the Dicke pseudospin method, and used in the study of two-level atoms.
We investigate the steady-state spontaneous emission spectrum of a three-level atom driven by two coherent fields and the absorption spectrum of a weak probe passing through a collection of such driven atoms. We find that the fluorescence spectrum is strongly affected by the decay rates of all the levels involved in the atomic evolution and not just by the decay parameters of the specific transition whose emission spectrum is being monitored. In particular, the spectral components can acquire very different widths and peak heights relative to the case of the standard resonance fluorescence in which a two-level system is driven by a single near-resonant field. An external probe signal passing through the gas of three-level atoms may be absorbed or amplified, as in the standard two-level case, but under specific operating conditions, amplification (or absorption) occurs over the entire range where the atomic response is appreciable. In this case the existence of amplification or absorption is controlled solely by the population difference between two dressed states of the system. We provide numerical results in support of our arguments for arbitrary values of the atomic and field parameters and also develop an analytic description in the limit of strong driving fields that leads to explicit line-shape and linewidth formulas.
Interplay between the effects of coherent radiation and localization of light is analysed. A system of two-level atoms is placed in a medium interacting with electromagnetic field. The matter-light interaction can result in the appearance of a band gap in the spectrum of polariton states. If an atom with a resonance frequency inside the gap is incorporated into such a medium, the atomic spontaneous emission is suppressed, which is termed the localization of light. However, a system of resonance atoms inside the gap can radiate due to their coherent interactions. The peculiarity of the coherent radiation by a system of atoms, under the localization of light for a single atom, is studied.
A previously developed theory of spontaneous emission from driven systems has been applied to the case of a Doppler broadened gas of two level atoms radiating into free space. The power spectrum of those photons radiated nearly parallel to the propagation vector of the driving field is predicted to differ from that of the undriven system. The case of zero attenuation coefficient (population equality in the two resonance levels) and the driving field tuned to the center of the Doppler line, is investigated in particular. When the saturation parameter is large there is strong suppression, in an interval about the central frequency comparable to the saturated width, of the spontaneous emission whose spectral components are phased for amplitude modulation relative to the driving field. An amount of power equal to that suppressed, but with spectral components phased for phase modulation relative to the driving field, is radiated in an interval about the central frequency comparable to the homogeneous width.