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Physical Review B

Collective spontaneous emission in coupled quantum dots: Physical mechanism of quantum nanoantenna

Salman Mokhlespour, Jos E. M. Haverkort, Gregory Ya. Slepyan, С. А. Максименко, A. Hoffmann

Published Dec 27, 2012• 34 citations
Publisher

Abstract

We investigate the collective spontaneous emission in a system of two identical quantum dots (QDs) strongly coupled through the dipole-dipole ($d\ensuremath{-}d$) interaction. The QDs are modeled as two-level quantum objects, while the $d\ensuremath{-}d$ interaction is described as the exchange of a virtual photon through the photonic reservoir. The master equation approach is used in the analysis. The main attention is focused on antenna characteristics of the two-QD system---the radiation intensity dependence on the meridian and azimuthal angles of observation. We show that the radiation pattern of such a system is nonstationary and its temporal behavior depends on the initial quantum state. In particular, for entangled initial states the radiative pattern exhibits oscillations on the frequency which corresponds to the $d\ensuremath{-}d$ interaction energy. We also analyze spectral properties of the directional diagram. The comparison of radiation patterns is carried out for two QDs and two classical dipoles. The concept of quantum nanoantenna is proposed based on collective spontaneous emission in QD ensembles.

DOI
10.1103/physrevb.86.245322

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We investigate the collective spontaneous emission in a system of two identical quantum dots (QDs) strongly coupled through the dipole-dipole (d\ensuremath−dd\ensuremath{-}dd\ensuremath−d) interaction. The QDs are modeled as two-level quantum objects, while the d\ensuremath−dd\ensuremath{-}dd\ensuremath−d interaction is described as the exchange of a virtual photon through the photonic reservoir. The master equation approach is used in the analysis. The main attention is focused on antenna characteristics of the two-QD system---the radiation intensity dependence on the meridian and azimuthal angles of observation. We show that the radiation pattern of such a system is nonstationary and its temporal behavior depends on the initial quantum state. In particular, for entangled initial states the radiative pattern exhibits oscillations on the frequency which corresponds to the d\ensuremath−dd\ensuremath{-}dd\ensuremath−d interaction energy. We also analyze spectral properties of the directional diagram. The comparison of radiation patterns is carried out for two QDs and two classical dipoles. The concept of quantum nanoantenna is proposed based on collective spontaneous emission in QD ensembles.
The spontaneous emission spectrum from two quantum dots (QDs) that are strongly coupled with a single-mode nanocavity is investigated using rigorous numerical calculations and simple analytical solutions of quantum dynamics. The emission spectra both from the side and along the axis of the cavity are considered. Modification of two parameters, the coupling strength and the detuning between the transition frequencies of the two quantum dots, allows us to efficiently control the shape of the spontaneous emission spectrum. Different profiles and their physical origins can be well understood in the dressed-state picture for the light—QD interaction in the on-resonance and off-resonance situations. In the on-resonance situation, the emission spectra exhibit symmetric features, and they are not altered by the asymmetry in the coupling parameters. The axis spectra show two emission peaks while the side spectra have three emission peaks. In the off-resonance situation, the emission spectra always show an asymmetrical three-peak feature. When the two QDs have different decay parameters, singular features (a peak or a dip) can take place at the frequency of the cavity mode, and this is attributed to the unbalanced process of the emission and absorption of a single photon.
Using the electromagnetic response function of an electric dipole located within a dielectric geometry, we derive the mathematical equivalence between the classical response and quantum mechanical resonant dipole–dipole interaction between two quantum objects (atoms, quantum dots, etc). Cooperative spontaneous emission likewise emerges from this equivalence. We introduce a practical numerical technique using finite difference time domain for calculating both dipole–dipole interaction and collective spontaneous emission in confined dielectric structures, where strong light–matter coupling might arise. This method is capable of obtaining resonant dipole–dipole interaction over a wide range of frequencies in a single run. Our method recaptures the results of quantum mechanical second order perturbation theory for weak light–matter coupling. In strong coupling situations such as near a photonic band edge, second order Rayleigh–Schrödinger perturbation theory leads to divergences, and instead Brillouin–Wigner perturbation theory is required. This is equivalent to the use of a variational wavefunction to describe the exciton transfer between initial and final states. We introduce a system of coupled classical oscillators, that describes resonant dipole–dipole interaction and vacuum Rabi splitting in the strong-coupling regime, and that provides an effective numerical scheme based on the finite difference time domain method. This includes the effects of quantum entanglement and the correlation of quantum fluctuations. We discuss the crossover to Forster energy transfer when quantum correlations between the dipoles are damped by strong environmental interactions.
This paper describes a novel model for the dynamics of the dipole coherence in two-level quantum dots (QDs) interacting with localized photons. The model is based on the fact that the coupling on a nanometer scale between QDs via optical near fields represented by localized photons is much stronger than that via propagating far fields. The model predicts that an intriguing phenomenon such as a collective dipole oscillation occurs if the initial quantum states are locally manipulated. The origin of this kind of collective behaviour is discussed in view of Dicke's superradiance.
Spontaneous emission from two two-level atoms within an anisotropic photonic crystal is investigated when direct dipole-dipole interaction is taken into account. The radiation properties of the present two atoms system are similar to that of a V-type three-level atom embedded in an anisotropic photonic crystal. The direct dipole-dipole interaction can enhance or depress the spontaneous emission depending on the relative position of the upper levels from the band edge of the photonic crystals. Owing to quantum interference and the dipole-dipole interaction, the spontaneous emission spectra are complicated non-Lorentzian shapes and depend strongly on the relative position of the upper levels from the bandgap and the initial state of the system.
The role of local fields in quantum electrodynamics of isolated quantum dot (QD) has been analyzed. The system is modeled as a strongly confined in space two-level quantum oscillator illuminated by quantum light. Relation between local and acting fields in QD has been derived in the dipole approximation from the integral Maxwell equations for electromagnetic field operators. A formalism of the electromagnetic field quantization in electrically small scatterers has been developed. As a result, Hamiltonian of the system has been formulated in terms of the acting field with a separate term responsible for the effect of depolarization. Schr\"odinger equation with that Hamiltonian has been solved in linear approximation. Interaction of QD with different quantum states of light, such as Fock states, coherent states, Fock qubits, entangled states, has been analyzed. It has been shown that the local-fields induce a fine structure of the QD absorption (emission) spectrum: instead of a single line with the frequency corresponding to the exciton transition, a doublet appears with one component shifted to the blue (red). The value of the shift depends only on the geometrical and electronic properties of QD while the intensities of components are completely determined by the quantum light statistics. It has been demonstrated that in the limiting cases of classical light and single-photon state the doublet is reduced to a singlet shifted in the former case and unshifted in the latter one. A physical interpretation of the predicted effect has been proposed. Possible ways of experimental observation of the effect has been discussed together with the potentiality of its utilization in the quantum information processing.