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Journal of Physics A Mathematical and General

Analytic continuation of generalized susceptibility and system-reservoir correlation effects

Horacio M. Cataldo

Published Mar 7, 1995• 2 citations
Publisher

Abstract

A fully non-Markovian calculation of the generalized susceptibility of a quantum system weakly coupled to a heat bath is presented. In contrast to most of the treatments we provide a complete solution in the sense that it includes the analytic continuation to the lower half-plane. Various applications are discussed including the consideration of boson and fermion heat baths. It is shown that our result takes into account system-reservoir correlations which are neglected in the Markovian approximation.

DOI
10.1088/0305-4470/28/5/009

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A fully non-Markovian calculation of the generalized susceptibility of a quantum system weakly coupled to a heat bath is presented. In contrast to most of the treatments we provide a complete solution in the sense that it includes the analytic continuation to the lower half-plane. Various applications are discussed including the consideration of boson and fermion heat baths. It is shown that our result takes into account system-reservoir correlations which are neglected in the Markovian approximation.
We propose a formulation to obtain the exact susceptibility for system arbitrary operators to the external fields by means of the whole-system Hamiltonian (system plus reservoir) diagonalization methods, where the dissipative effects directly reflect the nature of the structured non-Markovian reservoir. This treatment does not make the Born-Markovian approximation in structured non-Markovian reservoir. The relations between linear response function and bound-states for the system as well as structured reservoir are found, which shows the photon bound-states and continuous energy spectrum can be readout from the susceptibility, respectively. These results are then used to examine the validity of second-order Born-Markovian approximation, where we find interesting features (e.g., bound-states) are lost in the approximate treatments for open systems. We study the dependence of the response function on the type (spectrum density) of interaction between the system and structured reservoir. We also give the physical reasons behind the disappearance of the bound-states in the approximation method. Finally, these results are also extended to a more general quantum network involving an arbitrary number of coupled-bosonic system without rotating-wave approximation. The presented results might open a new door to understand the linear response and the energy spectrum for non-Markovian open systems with structured reservoirs.
The heat flow between a quantum system and its reservoir is analyzed when initially both are in a separable thermal state and asymptotically approach a correlated equilibrium. General findings are illustrated for specific systems and various classes of non-Markovian reservoirs. System-bath correlations are shown to be substantial at low temperatures even in the weak coupling regime. As a consequence, predictions of work and heat for actual experiments obtained within conventional perturbative approaches may often be questionable. Correlations induce characteristic imprints in heat capacities which opens a proposal to measure them in solid state devices.
A method is proposed to describe Fermi or Bose systems coupled to one or several heat baths composed of fermions and/or bosons. The method, called the coupled equations of motion method, properly includes non-Markovian effects. The approach is exact in the full-coupling approximation when only bosonic particles are present in the system and baths. The approach provides an approximate treatment when fermions are present either in the system and/or in one or several environments. Our approach has the advantage of properly respecting the Pauli exclusion principle for fermions during the evolution. We illustrate the approach for the single fermionic or bosonic oscillator coupled to one or two heat baths assuming different types of quantum statistics (fermion or boson) for them. The cases of a Fermi system coupled to fermion or boson heat baths or a mixture of both are analyzed in detail. With the future goal of treating Fermi systems formed of an increasing number of two-level systems (qubits), we discuss possible simplifications that could be made in the equations of motion and their limits of validity in terms of the system-bath coupling or of the initial heat bath temperatures.
A close examination of the validity of the Markovian approximation in the context of relaxation theory is presented. In particular, we examine the question of positivity of various approximations to the reduced dynamics of an open system in interaction with a heat reservoir. It is shown that the Markovian equations of motion obtained in the weak coupling limit (Redfield equations) are a consistent approximation to the actual reduced dynamics only if supplemented by a slippage in the initial conditions. This slippage captures the effects of the non-Markovian evolution that takes place in a short transient time, of the order of the relaxation time of the isolated bath.
The reduced dynamics of a quantum system interacting with a linear heat bath finds an exact representation in terms of a stochastic Schrödinger equation. All memory effects of the reservoir are transformed into noise correlations and mean-field friction. The classical limit of the resulting stochastic dynamics is shown to be a generalized Langevin equation, and conventional quantum state diffusion is recovered in the Born-Markov approximation. The non-Markovian exact dynamics, valid at arbitrary temperature and damping strength, is exemplified by an application to the dissipative two-state system.