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Journal of Physics A Mathematical and General

Collective radiation and the near-zone field

Maciej Lewenstein, Kazimierz Rza̧żewski

Published Feb 1, 1980• 15 citations
Publisher

Abstract

Collective radiation of several atoms represented by harmonic oscillators is analysed. When taking into account the near-zone field, the authors show that the existence of the super-radiant mode in the small-system limit is a rare phenomenon. Explicit calculations for four oscillators placed on the vertices of a tetrahedron are presented. Analogous results are obtained for two-level atoms in the case of small total excitation.

DOI
10.1088/0305-4470/13/2/035

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Physical Review A•Jun 1, 1977•51 citations
Collective radiation of several atoms represented by harmonic oscillators is analysed. When taking into account the near-zone field, the authors show that the existence of the super-radiant mode in the small-system limit is a rare phenomenon. Explicit calculations for four oscillators placed on the vertices of a tetrahedron are presented. Analogous results are obtained for two-level atoms in the case of small total excitation.
The evolution of a small spherical system of many harmonic oscillators, initially in a coherent superradiant state, is considered. The dipole oscillators interact via their mutual fields, both longitudinal and transverse, including both radiation- and near-zone contributions. In principle, this interaction can dephase the vibration of oscillators and thereby decrease or eliminate the coherent superradiant contribution to the emitted radiation. It is shown, however, that if the system is sufficiently small, this dephasing makes only small corrections to the decay of the initial state. Thus the emission of a superradiant pulse and cooperative radiative decay are major processes in the system.
In a previous investigation, a general theory for spontaneous emission from a system of NNN identical atoms or molecules was developed. This theory was based on the master equation recently derived in another paper. In that paper, the master equation relating to spontaneous emission from a system of harmonic oscillators was also derived. In the present investigation, the normally ordered correlation functions for the oscillator system are calculated and these are then used to calculate the radiation-field correlation functions in the far zone. These correlation functions are compared for two different modes of excitation, viz., (i) when each of the oscillators is excited initially to a Fock state, and (ii) when each of the oscillators is excited to some coherent state. It is found that the even-order (2n2n2n) correlation functions for the second mode of excitation (superradiant excitation) are of order N2n{N}^{2n}N2n higher than those for the first mode of excitation. It is also shown that the photoelectron counting distribution for the superradiant excitation is Poissonian. Finally, the non-Markoffian effects in the spontaneous emission are studied in detail and their connection with exact results is described.
The paper discusses three different modes of electromagnetic field generation by an ensemble of oscillators placed at the radiation wavelength in the one-dimensional case. The excitation of the resonator field is considered, which, as a rule, is determined by the geometry of the system, with and without taking into account the eigenfields of the emitters. The superradiance regime of the same ensemble of oscillators is also analyzed. In fact, superradiance is formed due to the emitters' own fields even in the absence of a resonator. It is noted that the maximum achievable amplitudes of induced fields both in the superradiance regime and in the regime of excitation of the resonator field are comparable. This makes us think about the role of the self-fields of emitters in electronic devices. It is shown that in describing the resonator excitation mode, in addition to the resonator field, it is also necessary to take into account the sum of the natural fields of the emitters in the active zone. Synchronization of emitters leads not only to an increase in the resonator field, but also, as in the superradiance regime, it significantly increases the amplitude of the sum of the oscillator fields. It is shown that in the practically interesting case of open systems (dissipative generation modes), taking into account the eigenfields of the emitters significantly reduces the characteristic time for the development of the generation process and increases the maximum achievable oscillation amplitude. This account also changes the conditions for achieving the maximum energy flow from the system. This can change the operating point of the generation process, which is determined by the requirement for the maximum rate of energy output from the system.
The problem of the evolution in time of a system of two-level atoms that are coupled through their electromagnetic fields, is studied and solved in the framework of semiclassical radiation theory. The atoms may be in any initial states and the radiation reaction is fully taken into account. Both superradiance and time-dependent frequency shift or chirping effects are found. The assumption that all the atoms see the same field is shown to place severe constraints on the evolution of the system, in the form of constants of the motion. These constraints are most easily pictured in terms of the Bloch-vector representation of the atomic system, and they lead to explicit solutions for the time development of each atom. It is shown that the evolution of the complex system is describable by means of a collective super Bloch vector, whose behavior is similar to the behavior of the Bloch vector for a single isolated atom. The constraints on the motion also imply that the system cannot radiate all its energy coherently; some of it remains trapped, to be dissipated ultimately by incoherent processes. Some curves are presented to illustrate the behavior of the system in special cases.
In order to study the cooperative emission of radiation from an extended system of NNN two-level atoms, we use the master-equation approach within the Born and Markov approximations. All the properties of the emission of radiation can be deduced from the diagonalization of the coupling matrix $\ensuremath{\Gamma}$, where an element ${\ensuremath{\Gamma}}_{\mathrm{jk}}$ gives the coupling between the atoms labeled jjj and kkk via the electromagnetic field. We choose a pencil-shaped volume and study analytically the coupling matrix in the limit for small and large Fresnel numbers. For Fresnel numbers of order unity numerical methods are used. Thus we prove that, for the pencil-shaped geometry, any elaborated model must take into account the interaction of the atoms with the infinity of electromagnetic field modes lying inside two small solid angles about the axis of the largest linear dimension, which we label the zzz axis. In other words, the intensity of radiation emitted by any atom of the system depends on its position with respect to the others and this "propagation effect" cannot be neglected when interpreting superradiance experiments. For small Fresnel numbers the zzz dependence predominates, in the opposite case the (x,yx, yx,y) dependence does, while for Fresnel numbers of order unity the dependence of all three components must be taken into account. Preliminary calculations are given for which only the zzz dependence is considered; for Fresnel numbers of magnitude of order unity or smaller, the effect of propagation along the zzz axis displays large delays for the appearance of superradiance with respect to the time at which the superradiant pulse is maximum when the "propagation effects" are neglected (one-mode model).