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International Journal of Modern Physics B

EVOLUTION AND DESTRUCTION OF THE KONDO EFFECT IN A CAPACITIVELY COUPLED DOUBLE DOT SYSTEM

David E. Logan, Martin R. Galpin

Published May 30, 2007• 0 citations
Publisher

Abstract

We consider the simplest example of a double quantum dot system: two equivalent, capacitively coupled single-level dots, each coupled to its own lead. Focussing on a regime of two electrons on the double dot, a rich range of behaviour is found on increasing the interdot coupling: first a crossover from spin- to charge-Kondo physics, via an intermediate SU(4) state with entangled spin and charge degrees of freedom; followed by a quantum phase transition of Kosterlitz-Thouless type to a non-Fermi liquid 'charge-ordered' phase with finite residual entropy and anomalous transport properties. The numerical renormalization group method, coupled with simple physical arguments, is employed to obtain a detailed understanding of the problem.

DOI
10.1142/s0217979207043580

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We consider the simplest example of a double quantum dot system: two equivalent, capacitively coupled single-level dots, each coupled to its own lead. Focussing on a regime of two electrons on the double dot, a rich range of behaviour is found on increasing the interdot coupling: first a crossover from spin- to charge-Kondo physics, via an intermediate SU(4) state with entangled spin and charge degrees of freedom; followed by a quantum phase transition of Kosterlitz-Thouless type to a non-Fermi liquid 'charge-ordered' phase with finite residual entropy and anomalous transport properties. The numerical renormalization group method, coupled with simple physical arguments, is employed to obtain a detailed understanding of the problem.
We investigate two equivalent, capacitively coupled semiconducting quantum dots, each coupled to its own lead, in a regime where there are two electrons on the double dot. With increasing interdot coupling, a rich range of behavior is uncovered: first a crossover from spin- to charge-Kondo physics, via an intermediate SU(4) state with entangled spin and charge degrees of freedom, followed by a quantum phase transition of Kosterlitz-Thouless type to a non-Fermi-liquid "charge-ordered" phase with finite residual entropy and anomalous transport properties. Physical arguments and numerical renormalization group methods are employed to obtain a detailed understanding of the problem.
The numerical renormalization group is employed to study a double quantum (DQD) dot system consisting of two equivalent single-level dots, each coupled to its own lead and with a mutual capacitive coupling embodied in an interdot interaction U', in addition to the intradot Coulomb interaction U. We focus on the regime with two electrons on the DQD, and the evolution of the system on increasing U'/U. The spin-Kondo effect arising for U'=0 (SU(2) x SU(2)) is found to persist robustly with increasing U'/U, before a rapid but continuous crossover to (a) the SU(4) point U'=U where charge and spin degrees of freedom are entangled and the Kondo scale strongly enhanced; and then (b) a charge-Kondo state, in which a charge-pseudospin is quenched on coupling to the leads/conduction channels. A quantum phase transition of Kosterlitz-Thouless type then occurs from this Fermi liquid, strong coupling (SC) phase, to a broken symmetry, non-Fermi liquid charge ordered (CO) phase at a critical U'_c. Our emphasis in this paper is on the structure, stability and flows between the underlying RG fixed points, on the overall phase diagram in the (U,U')-plane and evolution of the characteristic low-energy Kondo scale inherent to the SC phase; and on static physical properties such as spin- and charge-susceptibilities (staggered and uniform), including universality and scaling behaviour in the strongly correlated regime. Some exact results for associated Wilson ratios are also obtained.
Abstract. The numerical renormalization group is employed to study a double quantum (DQD) dot system consisting of two equivalent single-level dots, each coupled to its own lead and with a mutual capacitive coupling embodied in an interdot interaction U ′, in addition to the intradot Coulomb interaction U. We focus on the regime with two electrons on the DQD, and the evolution of the system on increasing U ′/U. The spin-Kondo effect arising for U ′ = 0 (SU(2) × SU(2)) is found to persist robustly with increasing U ′/U, before a rapid but continuous crossover to (a) the SU(4) point U ′ = U where charge and spin degrees of freedom are entangled and the Kondo scale strongly enhanced; and then (b) a charge-Kondo state, in which a charge-pseudospin is quenched on coupling to the leads/conduction channels. A quantum phase transition of Kosterlitz-Thouless type then occurs from this Fermi liquid, strong coupling (SC) phase, to a broken symmetry, non-Fermi liquid charge ordered (CO) phase at a critical U ′ c. Our emphasis in this paper is on the structure, stability and flows between the underlying RG fixed points, on the overall phase diagram in the (U, U ′)-plane and evolution of the characteristic low-energy Kondo scale inherent to the SC phase; and on static physical properties such as spin- and charge-susceptibilities (staggered and uniform), including universality and scaling behaviour in the strongly correlated regime. Some exact results for associated Wilson ratios are also obtained.
Abstract. We consider a double dot system of equivalent, capacitively coupled semiconducting quantum dots, each coupled to its own lead, in a regime where there are two electrons on the double dot. Employing the numerical renormalization group, we focus here on single-particle dynamics and the zerobias conductance, considering in particular the rich range of behaviour arising as the interdot coupling is progressively increased through the strong coupling (SC) phase, from the spin-Kondo regime, across the SU(4) point to the charge-Kondo regime; and then towards and through the quantum phase transition to a charge-ordered (CO) phase. We first consider the two-self-energy description required to describe the broken symmetry CO phase, and implications thereof for the non-Fermi liquid nature of this phase. Numerical results for single-particle dynamics on all frequency scales are then considered, with particular emphasis on universality and scaling of low-energy dynamics throughout the SC phase. The role of symmetry breaking perturbations is also briefly discussed.
We consider a double dot system of equivalent, capacitively coupled semiconducting quantum dots, each coupled to its own lead, in a regime where there are two electrons on the double dot. Employing the numerical renormalization group, we focus here on single-particle dynamics and the zero-bias conductance, considering in particular the rich range of behaviour arising as the interdot coupling is progressively increased through the strong coupling (SC) phase, from the spin-Kondo regime, across the SU(4) point to the charge-Kondo regime; and then towards and through the quantum phase transition to a charge-ordered (CO) phase. We first consider the two-self-energy description required to describe the broken symmetry CO phase, and implications thereof for the non-Fermi liquid nature of this phase. Numerical results for single-particle dynamics on all frequency scales are then considered, with particular emphasis on universality and scaling of low-energy dynamics throughout the SC phase. The role of symmetry breaking perturbations is also briefly discussed.
We investigate the Kondo effect in a double quantum dot which is capacitively coupled to a charge qubit. It is shown that due to this capacitive coupling, the bare interdot repulsive interaction in the double quantum dot is effectively reduced and eventually changed to an attractive interaction for strong couplings between the double quantum dot and the qubit. By deriving the low-energy effective Hamiltonian of the system, we find that the low-energy dynamics of the system corresponding to these two positive or negative effective interaction regimes can be described, respectively, by an isotropic orbital-Kondo or an anisotropic charge-Kondo Hamiltonian. Moreover, we study various thermodynamic and electronic transport properties of the system by using the numerical renormalization group method.