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Laser Physics Letters

Femtosecond echo-processing in a dye-doped polymer film at room temperature

Georgy M. Safiullin, Victor G. Nikiforov, Vladimir S. Lobkov, В. В. Самарцев, A.V. Leontiev

Published Jun 16, 2009• 11 citations
Publisher

Abstract

The possibility to mechanize at room temperature a logical function of bit-to-bit parallel multiplication for optical echo-processor based on the third-order nonlinear optical response of a resonant medium is experimentally studied. The polyvinilbutural film doped with phthalocyanine dye was used as an operating medium in our experiments. The time needed to realize the logical operation, the result of which is presented in the spectrum of the nonlinear optical response of the medium after action of the two spectrally coded pumping pulses, is less than 1 ps. The values of a homogeneous broadening of S 0 – S 1 line Γ hom = 89 cm -1 and Γ hom = 44 cm -1 are established at T = 300 K and T = 77 K respectively. The laser excitation parameters needed for effective operating of optical processor are defined. The maximum word length achievable under current experimental conditions is estimated.

DOI
10.1002/lapl.200910060

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Bit-to-bit parallel multiplication based on the third-order nonlinear optical response in a dye-doped polymer film at room temperature

Georgy M. Safiullin, Victor G. Nikiforov, Vladimir S. Lobkov +2 more

We realized a logical function of bit-to-bit parallel multiplication for optical echo-processor based on the third-order nonlinear optical response of a resonant medium at room temperature. As an operating medium we used the polyvinilbutural film doped with phthalocyanine dye. The result of the logical operation is presented in the spectrum of the nonlinear optical response after action of the two spectrally coded pumping pulses. The time of the logical operation is about 500 fs. We obtained the values of a homogeneous broadening of S0 - S1 line: Γhom = 89 cm-1 at T = 300 K and Γhom = 44 cm-1 at T = 77 K. The laser excitation parameters needed for effective operating of optical processor are defined. The maximum word length achievable under current experimental conditions is estimated.

Proceedings of SPIE, the International Society for Optical Engineering/Proceedings of SPIE•Sep 10, 2010•0 citations

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It is reported about the first observation (in a solid-state sample) and detailed investigation of the stimulated femtosecond photon echo (SFPE) signals at room temperature in a polyvinylbutural film doped with molecules of phthalocyanine of HW 1009 type at the wavelength of 788 nm. A dependence of relative intensity of these echo-signals on time intervals between the second and the third exciting pulses was studied and the SFPE spectrum was investigated with respect to the spectra of both exciting pulses and signals of self-diffraction. It was found that the linear electron-phonon coupling is weak and the influence of the phonon-side band of the absorption line on the SFPE signals is less significantly than on the signals of primary photon echo.

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The first observation is reported of the primary and stimulated femtosecond photon echoes at liquid nitrogen and room temperatures in a dye-doped polymer film at a wavelength of 780 nm. Echo signals were generated by pulses with the duration of 65 fs. The primary echo signal decay at liquid nitrogen and room temperatures can not be described by a simple exponential function. The decay of primary echo signal at room temperature demonstrates complex behavior caused by the presence of the phonon-side band in the optical band of impurity centers. There were also detected signals of the self-diffraction of exciting pulses on a nonequilibrium population difference grating, induced in resonant medium by these pulses.

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Femtosecond photon echo in a dye-doped polymer film and the possibility of coherent optical cooling

Vladimir S. Lobkov, S. V. Petrushkin, К. М. Салихов +3 more

The signals of primary and stimulated femtosecond photon echoes are investigated in a dye-doped polymer film at room temperature. The homogeneous S 0 → S 1 spectral line width, which is due to the interaction between the impurity molecules and the quasi-local low-frequency modes, is estimated (≈5 × 1012 Hz). Special attention is paid to the study of spectra of femtosecond echo signals. The short-wave shifts of these spectra, with respect to the spectrum of femtosecond exciting pulses, are observed. These shifts indicate that the anti-Stokes regime of femtosecond pulse emission is realized. Therefore, the coherent regime of laser cooling of solids appears to be possible. The prospects of using of this new cooling regime in the function of a solid-state optical refrigerator are discussed.

Laser Physics•May 1, 2007•8 citations
The possibility to mechanize at room temperature a logical function of bit-to-bit parallel multiplication for optical echo-processor based on the third-order nonlinear optical response of a resonant medium is experimentally studied. The polyvinilbutural film doped with phthalocyanine dye was used as an operating medium in our experiments. The time needed to realize the logical operation, the result of which is presented in the spectrum of the nonlinear optical response of the medium after action of the two spectrally coded pumping pulses, is less than 1 ps. The values of a homogeneous broadening of S 0 – S 1 line Γ hom = 89 cm -1 and Γ hom = 44 cm -1 are established at T = 300 K and T = 77 K respectively. The laser excitation parameters needed for effective operating of optical processor are defined. The maximum word length achievable under current experimental conditions is estimated.
We realized a logical function of bit-to-bit parallel multiplication for optical echo-processor based on the third-order nonlinear optical response of a resonant medium at room temperature. As an operating medium we used the polyvinilbutural film doped with phthalocyanine dye. The result of the logical operation is presented in the spectrum of the nonlinear optical response after action of the two spectrally coded pumping pulses. The time of the logical operation is about 500 fs. We obtained the values of a homogeneous broadening of S0 - S1 line: Γhom = 89 cm-1 at T = 300 K and Γhom = 44 cm-1 at T = 77 K. The laser excitation parameters needed for effective operating of optical processor are defined. The maximum word length achievable under current experimental conditions is estimated.
The signals of primary and stimulated femtosecond photon echo in polymer films doped with dye (phthalocyanine) molecules have been experimentally investigated at room temperature. A femtosecond echo spectrometer for these echo experiments is described. The decay curves of echo signals with increasing time intervals between excitation femtosecond pulses are obtained and blue shifts of the spectra of femtosecond echo signals with respect to the spectrum of excitation pulses are revealed. The possibilities of using the studied doped polymer films as recording media for high-temperature echo processors and coolants in optical refrigerators are analyzed.
It is reported about the first observation (in a solid-state sample) and detailed investigation of the stimulated femtosecond photon echo (SFPE) signals at room temperature in a polyvinylbutural film doped with molecules of phthalocyanine of HW 1009 type at the wavelength of 788 nm. A dependence of relative intensity of these echo-signals on time intervals between the second and the third exciting pulses was studied and the SFPE spectrum was investigated with respect to the spectra of both exciting pulses and signals of self-diffraction. It was found that the linear electron-phonon coupling is weak and the influence of the phonon-side band of the absorption line on the SFPE signals is less significantly than on the signals of primary photon echo.
The first observation is reported of the primary and stimulated femtosecond photon echoes at liquid nitrogen and room temperatures in a dye-doped polymer film at a wavelength of 780 nm. Echo signals were generated by pulses with the duration of 65 fs. The primary echo signal decay at liquid nitrogen and room temperatures can not be described by a simple exponential function. The decay of primary echo signal at room temperature demonstrates complex behavior caused by the presence of the phonon-side band in the optical band of impurity centers. There were also detected signals of the self-diffraction of exciting pulses on a nonequilibrium population difference grating, induced in resonant medium by these pulses.
The signals of primary and stimulated femtosecond photon echoes are investigated in a dye-doped polymer film at room temperature. The homogeneous S 0 → S 1 spectral line width, which is due to the interaction between the impurity molecules and the quasi-local low-frequency modes, is estimated (≈5 × 1012 Hz). Special attention is paid to the study of spectra of femtosecond echo signals. The short-wave shifts of these spectra, with respect to the spectrum of femtosecond exciting pulses, are observed. These shifts indicate that the anti-Stokes regime of femtosecond pulse emission is realized. Therefore, the coherent regime of laser cooling of solids appears to be possible. The prospects of using of this new cooling regime in the function of a solid-state optical refrigerator are discussed.