In the framework of a general theory of open quantum systems, we obtain a quantum master equation for the two-level atom interacting with a single mode of the electromagnetic field. On this basis, we obtain new optical equations. In comparison with the conventional Bloch-Feynman optical equations which contain three phenomenological parameters, the new equations contain nine phenomenological parameters. New physical effects , due to the opening of the system, are predicted: 1) a resonance frequency shift, 2) an asymmetry of the spectral line, 3) a modification of the dependence of the absorbtion coefficient and of the nonlinear dephasing on the atomic detuning, and 4) an additional nonlinear dependence of the absorbtion coefficient on the electric field. For a rather small atom density when the fourth effect can be neglected,we found an analytical expression of the transmittivity characteristic of an optical bistable Fabry-Perot resonator and found a good agreement with the experiment.
In the framework of a general theory of open quantum systems, we obtain a quantum master equation for the two-level atom interacting with a single mode of the electromagnetic field. On this basis, we obtain new optical equations. In comparison with the conventional Bloch-Feynman optical equations which contain three phenomenological parameters, the new equations contain nine phenomenological parameters. New physical effects , due to the opening of the system, are predicted: 1) a resonance frequency shift, 2) an asymmetry of the spectral line, 3) a modification of the dependence of the absorbtion coefficient and of the nonlinear dephasing on the atomic detuning, and 4) an additional nonlinear dependence of the absorbtion coefficient on the electric field. For a rather small atom density when the fourth effect can be neglected,we found an analytical expression of the transmittivity characteristic of an optical bistable Fabry-Perot resonator and found a good agreement with the experiment.
We present a many-body theory of nonlinear atom optics, and discuss some of its physical implications in the coherent regime. Considering a system of N identical two-level atoms interacting with classical and quantum-mechanical electromagnetic fields, we derive a Fock-space many-particle master equation. Introducting a Bogoliubov-Born-Green-Kirkwood-Yvon hierarchy and a Hartree-Fock factorization to truncate this hierarchy, we obtain an effective nonlinear single-particle master equation that forms the basis of nonlinear atom optics. In the second part of the paper, we concentrate on the coherent part of that master equation, and derive an effective single-atom nonlinear Schr\"odinger equation. This equation leads to the prediction of a number of effects, and, in particular, several kinds of atomic solitons. We discuss and numerically study two such kinds of solitons, Thirring solitons and gap solitons. Finally, the axial containment of an atomic gap soliton is illustrated.
We have investigated nonlinear atom optical effects which arise from atom-atom collisional interactions in a single-mode atomic Fabry-Perot cavity driven by a coherent cw atom laser beam. When the nonlinear interaction energy per single atom is small, the exact numerical solution of the master equation is well reproduced by a mean-field treatment in which quantum fluctuations are included linearizing the stochastic equations of the Positive-P representation. On the other hand, when the damping of the cavity mode is very weak and its wave-function is tightly confined in space, a regime of strong nonlinearity can be achieved. For the specific case of an incident atom laser frequency at resonance with the empty cavity, the numerical calculations predict a sort of atom blockade effect, which is a sort of atom optical analog of the well-known Coulomb blockade effect of electronic transport through microscopic structures: only one atom can occupy the cavity mode at a time and the statistical properties of the transmitted beam, being very similar to the resonance fluorescence from a single two-level system, show definitely nonclassical behaviors such as antibunching. Only at very large incident intensities, more than one atom can be simultaneously forced inside the cavity mode: in this regime, the results of the numerical calculations can be successfully interpreted using a dressed cavity model. From the formal analogy between atomic matter waves and optical light waves in nonlinear media, it follows that the same results hold for photonic systems.
The nine (9) elements of the density matrix of a general three-level atom interacting with a classically described linearly polarized light are parameterized by eight (8) variables related to the populations of the atomic levels, and the coherences (interference effects) between the levels. The dynamical equations of these eight parameters (that is, the optical Bloch equations for a general three-level atom) are derived under the electric dipole as well as the rotating wave approximations, and under the assumption that the matrix elements of the atomic electric dipole are all real. The general optical Bloch equations so derived are shown to contain the well-known optical Bloch equations for three-level atoms in the , and cascade configurations as well as those for two-level atoms as special cases. Expressing the interaction of light with a three-level atom in all possible configurations as well as with a two-level atom by a single set of generalized optical Bloch equations is the main result of this work.
In this chapter, we treat the basic quantum process of electromagnetic field propagation through an atomic system in a resonant Fabry-Perot cavity. We obtain the transmission characteristic of such a cavity, which is a basic element for a quantum heat converter. When the system is opened only by a population decay and a polarization dephasing, we get only an optical bistability characteristic. By openness according to the Lindblad- Sandulescu-Scutaru theory, we get also a coupling through environment between population and polarization, which, in some conditions, leads to an energy transfer from the disordered environment to the coherent electromagnetic field. We find that this phenomenon, which has experimental evidence, is an effect of an atom-atom coupling.
An open quantum system is a quantum system that interacts with some environment whose degrees of freedom have been coarse grained away. This model describes non-equilibrium processes more general than scattering-matrix formulations. Furthermore, the microscopically-derived environment provides a model of noise, dissipation and decoherence far more general than Markovian (white noise) models. The latter are fully characterized by Lindblad equations and can be motivated phenomenologically. Non-Markovian processes consistently account for backreaction with the environment and can incorporate effects such as finite temperature and spatial correlations. We consider linear systems with bilinear coupling to the environment, or quantum Brownian motion, and nonlinear systems with weak coupling to the environment. For linear systems we provide exact solutions with analytical results for a variety of spectral densities. Furthermore, we point out an important mathematical subtlety which led to incorrect master-equation coefficients in earlier derivations, given nonlocal dissipation. For nonlinear systems we provide perturbative solutions by translating the formalism of canonical perturbation theory into the context of master equations. It is shown that unavoidable degeneracy causes an unfortunate reduction in accuracy between perturbative master equations and their solutions. We also extend the famous theorem of Lindblad, Gorini, Kossakowski and Sudarshan on completely positivity to non-Markovian master equations. Our application is primarily to model atoms interacting via a common electromagnetic field. The electromagnetic field contains correlations in both space and time, which are related to its relativistic (photon-mediated) nature. As such, atoms residing in the same field experience different environmental effects depending upon their relative position and orientation. Our more accurate solutions were necessary to assess sudden death of entanglement at zero temperature. In contrast to previous claims, we found that all initial states of two-level atoms undergo finite-time disentanglement. We were also able to access regimes which cannot be described by Lindblad equations and other simpler methods, such as near resonance. Finally we revisit the infamous Abraham-Lorentz force, wherein a single particle in motion experiences backreaction from the electromagnetic field. This leads to a number of well-known problems including pre-acceleration and runaway solutions. We found a more a more-suitable open-system treatment of the nonrelativistic particle to be perfectly causal and dissipative without any extraneous requirements for finite size of the particle, weak coupling to the field, etc..
We study interactions of light with a sample of two-level atoms. Quantum statistical effects of degenerate boson and fermion gases are described by using the quantum field theory of atom-photon interactions, fully including the angular momentum degeneracies. Coupled propagation equations are given for light and matter fields, and plausible general simplifications are enumerated.^ In the limit of large atom-field detuning, multiple scattering of light and QED linewidths and line shifts may be ignored, and the propagation equations of light and matter fields may be decoupled. A general expression for the spectrum of the scattered light is derived, complete with the dependence on atomic level scheme, on various light polarizations, and on the geometry of the experiment. With these simplifications we are able to find distinct qualitative features in the spectrum of the scattered light in the case of both fermions and bosons that depend on the statistics of atoms. This is because for bosons (fermions), those scattering events in which an atom recoils to an already occupied state are enhanced (inhibited).^ As the driving light gets closer to the atomic resonance, multiple scattering and vacuum fluctuations of the electromagnetic fields should also be taken into account. We write the equations of motion for the excited state field operators by eliminating the vacuum electromagnetic field. It is always assumed that the driving external laser field is in the coherent state. We find in the limit of low light intensity, a hierarchy of equations of motion for correlation functions that contain one excited-atom field and one, two, three, etc., ground state atom fields. It is conjectured that the entire linear hierarchy may be solved by solving numerically the classical equations for the coupled system of electromagnetic fields and charged harmonic oscillators. We discuss the emergence of resonant dipole-dipole interactions and collective linewidths, and delineate the limits of validity of the column density approach in terms of non-cooperative atoms by presenting a mathematical example in which this approach is exact. ^