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Journal of the Optical Society of America B

Electromagnetically induced transparency over spectral hole-burning temperature in a rare-earth–doped solid

Byoung Seung HAM, M. S. Shahriar, Philip Hemmer

Published May 1, 1999• 24 citations
Publisher

Abstract

We have observed electromagnetically induced transparency (EIT) in rare-earth Pr3+-doped Y2SiO5 over the spectral hole-burning temperature. The transmission of the probe laser beam is increased by a factor of exp(1.4) at 12 K when a coupling laser of 1.2 kW/cm2 is applied to the system. The observation of EIT over the spectral hole-burning temperature in a rare-earth–doped solid represents important progress toward high-density echo-based optical memories at higher temperatures.

DOI
10.1364/josab.16.000801

Related papers

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We report on the observation of electromagnetically induced transparency using the hyperfine levels of Er 3+ :Y2SiO5 crystal and on hole burning spectroscopy in order to identify the

•Jan 1, 2006•0 citations
We have observed electromagnetically induced transparency (EIT) in rare-earth Pr3+-doped Y2SiO5 over the spectral hole-burning temperature. The transmission of the probe laser beam is increased by a factor of exp(1.4) at 12 K when a coupling laser of 1.2 kW/cm2 is applied to the system. The observation of EIT over the spectral hole-burning temperature in a rare-earth–doped solid represents important progress toward high-density echo-based optical memories at higher temperatures.
Summary form only given. When a resonant Raman laser field interacts with a three-level energy system, the system can undergo changes of linear and nonlinear optical properties. Especially in an optically thick medium, a strong resonant electromagnetic field can dress the energy states so that another resonant probe field may not be absorbed. This is due to destructive quantum interference between two absorption paths from the ground state to the dressed states. This phenomenon is called electromagnetically induced transparency. Our recently demonstrated Raman excited spin echo technique uses optically induced spin coherence. In general, the spin coherence decay time is much longer and more temperature insensitive than the optical coherence, so that the temperature limitation of the photon echoes can be overcome. The spin echoes are read by another optical field via enhanced four-wave mixing. Here, the nonlinearity in the optical transition is enhanced by EIT. In this paper we report the EIT observation at temperatures higher than that needed for the (optical) spectral hole-burning.
We study Lambda-type electromagnetically induced transparency (EIT) in cryogenically-cooled, europium and praseodymium doped yttrium orthosilicate (Eu:YSO and Pr:YSO). We use spectral hole burning techniques to vary the optical inhomogeneous width of the sub-ensemble of atoms participating in the EIT. The effect of inhomogeneous broadening has been studied in the context of Doppler broadened gases, but less so in solids where motional effects are absent and the coherence is not limited by the transit of atoms through the optical field. Rare earth doped crystals, like many solid-state systems, exhibit spectral hole burning in which a narrowband laser field optically pumps atoms to states in the ground manifold that are dark with respect to the applied field, opening up a transparency window that persists after the pumping laser is shuttered. More complex sequences of fields at multiple frequencies can create arbitrary spectral profiles, within bounds set by the particular energy level structure of the atoms. For both Eu:YSO and Pr:YSO, there are three hyperfine ground states and three hyperfine excited states (at zero magnetic field) and all nine transitions are dipole-allowed with varying transition strengths. We use spectral hole-burning techniques to prepare a sub-ensemble of atoms in a particular frequency class and a particular ground spin state, while also pumping atoms out of another ground state to create a Lambda system. We observe the same functional dependence of the EIT width on the optical inhomogeneous width and independently calibrated control field Rabi frequency in both systems.