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Physical Review Letters

Intrinsic Decoherence Mechanisms in the Microcavity Polariton Condensate

A. P. D. Love, Dmitry N. Krizhanovskii, David M. Whittaker, R. Bouchekioua, D. Sanvitto, S. Al Rizeiqi, R. A. Bradley, Maurice S. Skolnick, P. R. Eastham, R. André, Le Si Dang

Published Aug 7, 2008• 216 citations
Publisher

Abstract

The fundamental mechanisms which control the phase coherence of the polariton Bose-Einstein condensate (BEC) are determined. It is shown that the combination of number fluctuations and interactions leads to decoherence with a characteristic Gaussian decay of the first-order correlation function. This line shape, and the long decay times ( approximately 150 ps) of both first- and second-order correlation functions, are explained quantitatively by a quantum-optical model which takes into account interactions, fluctuations, and gain and loss in the system. Interaction limited coherence times of this type have been predicted for atomic BECs, but are yet to be observed experimentally.

DOI
10.1103/physrevlett.101.067404

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The fundamental mechanisms which control the phase coherence of the polariton Bose-Einstein condensate (BEC) are determined. It is shown that the combination of number fluctuations and interactions leads to decoherence with a characteristic Gaussian decay of the first-order correlation function. This line shape, and the long decay times ( approximately 150 ps) of both first- and second-order correlation functions, are explained quantitatively by a quantum-optical model which takes into account interactions, fluctuations, and gain and loss in the system. Interaction limited coherence times of this type have been predicted for atomic BECs, but are yet to be observed experimentally.
A theoretical model is presented which explains the dominant decoherence process in a microcavity polariton condensate. The mechanism which is invoked is the effect of self-phase modulation, whereby interactions transform polariton number fluctuations into random energy variations. The model shows that the phase coherence decay, g (1) (τ), has a Kubo form, which can be Gaussian or exponential, depending on whether the number fluctuations are slow or fast. This fluctuation rate also determines the decay time of the intensity correlation function, g (2) (τ), so it can be directly determined experimentally. The model explains recent experimental measurements of a relatively fast Gaussian decay for g (1) (τ), but also predicts a regime, further above threshold, where the decay is much slower.
The demonstration of coherent polariton emission from a CdTe microcavity structure [1] has provided a new system for the study of condensate physics. Unlike atomic condensates, the microcavity system is not in equilibrium; the polariton life-time in the cavity is only ∼ 2ps, so the population has to be maintained by pumping. This raises interesting questions about how the properties of such a non-equilibrium condensate differ from those of an equilibrium system. Recent experimental measurements of the first (g(1)) and second (g(2)) order correlation functions of the emitted light have shown that the decay times of both are ∼ 100−200ps, much longer than the cavity life-time. In this work, we present a theroetical treatment which provides a quantitative explanation of these results, and shows that the ultimate cause of the coherence decay is interactions between polaritons in the condensate. The microcavity polariton condensate is a mesoscopic quantum system, consisting of N ∼ 102 po-laritons within the finite size excitation spot. As a result, number fluctuations of ∼ N 1 2 are expected. For a finite equilibrium condensate of interacting particles, it is straight forward to show that the decay
Second-order time correlation measurements with a temporal resolution better than 3 ps were performed on a CdTe microcavity where spontaneous Bose-Einstein condensation is observed. After the laser pulse, the nonresonantly excited thermal polariton population relaxes into a coherent polariton condensate. Photon statistics of the light emitted by the microcavity evidences a clear phase transition from the thermal state to a coherent state, which occurs within 3.2 ps after the onset of stimulated scattering. Following this very fast transition, we show that the emission possesses a very high coherence that persists for more than 100 ps after the build-up of the condensate.
Temporal coherence is a fundamental property of macroscopic quantum systems, such as lasers in optics and Bose-Einstein condensates in atomic gases and it is a crucial issue for interferometry applications with light or matter waves. Whereas the laser is an ``open'' quantum system, ultracold atomic gases are weakly coupled to the environment and may be considered as isolated. The coherence time of a condensate is then intrinsic to the system and its derivation is out of the frame of laser theory. Using quantum kinetic theory, we predict that the interaction with noncondensed modes gradually smears out the condensate phase, with a variance growing as At2+Bt+C\mathcal{A}{t}^{2}+\mathcal{B}t+\mathcal{C}At2+Bt+C at long times ttt, and we give a quantitative prediction for A\mathcal{A}A, B\mathcal{B}B, and C\mathcal{C}C. Whereas the coefficient A\mathcal{A}A vanishes for vanishing energy fluctuations in the initial state, the coefficients B\mathcal{B}B and C\mathcal{C}C are remarkably insensitive to these fluctuations. The coefficient B\mathcal{B}B describes a diffusive motion of the condensate phase that sets the ultimate limit to the condensate coherence time. We briefly discuss the possibility to observe the predicted phase spreading, also including the effect of particle losses.