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Conference on Lasers and Electro-Optics Europe & European Quantum Electronics Conference (CLEO/Europe-EQEC)

Excitation of a single atom with a temporally shaped light pulses

Syed Abdullah Aljunid, Victor Leong, Dao Hoang Lan, Yimin Wang, Gleb Maslennikov, Valerio Scarani, Christian Kurtsiefer

Published May 1, 2013• 0 citations
Publisher

Abstract

We investigate the interaction between a single87Rb atom and optical pulses with a controlled temporal envelope. In our experiment an atom is coupled to the light field by high numerical aperture aspheric lens that focuses a Gaussian beam to an atom and fixes the spatial overlap with a field. The frequency/temporal overlap can be changed by shaping the temporal envelope of an attenuated coherent pulse with fast modulators [3]. The excitation probability Peis measured by detecting atomic fluorescence with high temporal resolution and normalizing the acquired rates by optical losses (Fig. 1).

DOI
10.1109/cleoe-iqec.2013.6801626

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QUANTUM INFORMATION EXCHANGE BETWEEN PHOTONS AND ATOMS

Wang Yi-min

Quantum information processing tasks have been implemented in various physical platforms. In this thesis, we consider two specific implementations: Part I presents a detailed study of the interaction of a single atom with a light pulse. Part II examines the case of a quantum controlled-phase gate in circuit quantum electrodynamics in the ultrastrong coupling regime. They are both actively pursued by many research groups. In Part I, we first present the framework for a single two-level atom interacting with the quantized electromagnetic field. The effect of temporal and spectral properties of the pulses on atomic excitation is studied for both Fock state and coherent state pulse. The detailed analysis of atomic excited state population is provided for single photon pulse with various temporal shapes. The work is then extended to a more general case with two spatial-modes and multi-photon pulses. The difference between Fock state and coherent state pulse on atomic excitation is further investigated. We find that at few photon levels, the maximum atomic excitation probability is a monotonic function of photon number for the coherent state pulse, but not for the Fock state pulse. Furthermore, we show that the atomic dynamics can be controlled by the initial relative phase between the two counter-propagating coherent state pulses incident on the atom, which is not the case with two Fock state pulses. The theoretical prediction is then compared with an experiment, where a single trapped 87Rb atom interacts with coherent state pulses engineered in temporal shape of rising exponential and rectangular form. Next, we propose a quantum memory setup based on a single two-level atom in a half cavity with a moving mirror. The efficiency of the quantum storage process is studied analytically and

•Jan 1, 2013•0 citations
We investigate the interaction between a single87Rb atom and optical pulses with a controlled temporal envelope. In our experiment an atom is coupled to the light field by high numerical aperture aspheric lens that focuses a Gaussian beam to an atom and fixes the spatial overlap with a field. The frequency/temporal overlap can be changed by shaping the temporal envelope of an attenuated coherent pulse with fast modulators [3]. The excitation probability Peis measured by detecting atomic fluorescence with high temporal resolution and normalizing the acquired rates by optical losses (Fig. 1).
We investigate the interaction between a single atom and optical pulses in a coherent state with a controlled temporal envelope. In a comparison between a rising exponential and a square envelope, we show that the rising exponential envelope leads to a higher excitation probability for fixed low average photon numbers, in accordance with a time-reversed Weisskopf-Wigner model. We characterize the atomic transition dynamics for a wide range of the average photon numbers and are able to saturate the optical transition of a single atom with ≈50 photons in a pulse by a strong focusing technique.
We report on a simple method to prepare optical pulses with exponentially rising envelope on the time scale of a few ns. The scheme is based on the exponential transfer function of a fast transistor, which generates an exponentially rising envelope that is transferred first on a radio frequency carrier, and then on a coherent cw laser beam with an electro-optical phase modulator. The temporally shaped sideband is then extracted with an optical resonator and can be used to efficiently excite a single (87)Rb atom.
State mapping between atoms and photons, and photon-photon interactions play an important role in scalable quantum information processing. We consider the interaction of a two-level atom with a quantized propagating pulse in free space and study the probability Pe(t){P}_{e}(t)Pe​(t) of finding the atom in the excited state at any time ttt. This probability is expected to depend on (i) the quantum state of the pulse field and (ii) the overlap between the pulse and the dipole pattern of the atomic spontaneous emission. We show that the second effect is captured by a single parameter $\ensuremath{\Lambda}\ensuremath{\in}[0,8\ensuremath{\pi}/3]$, obtained by weighting the dipole pattern with the numerical aperture. Then, Pe(t){P}_{e}(t)Pe​(t) can be obtained by solving time-dependent Heisenberg-Langevin equations. We provide detailed solutions for both single-photon Fock state and coherent states and for various temporal shapes of the pulses.
We demonstrate the generation of an optical dipole wave suitable for the process of efficiently coupling single quanta of light and matter in free space. We employ a parabolic mirror for the conversion of a transverse beam mode to a focused dipole wave and show the required spatial and temporal shaping of the mode incident onto the mirror. The results include a proof of principle correction of the parabolic mirror's aberrations. For the application of exciting an atom with a single photon pulse, we demonstrate the creation of a suitable temporal pulse envelope. We infer coupling strengths of 89% and success probabilities of up to 87% for the application of exciting a single atom for the current experimental parameters.
The ability to control the temporal shape of single-photon pulses is highly desirable in quantum information processing. For instance, it has been shown that Gaussian pulses are best suited for linear optics quantum computing1. By mimicking the time-reversal of a spontaneous emission event, it also allows to optimize the absorption of the prepared photons by a quantum emitter. In this work we investigate the potential of using fast modifications of the detuning between an atomic system and a cavity mode during photon emission to reach this goal. We compare two approaches consisting of varying the emitter or cavity frequency. The latter, achievable by a fast modification of the refractive index of a solid state cavity, will be shown to have negligible influence on the photon spectrum. It allows to create Gaussian pulses interacting with a fidelity to the target photons of 99%, as well as time-reversed photons absorbed by an atom in a cavity with a probability of 93%.
Quantum information processing tasks have been implemented in various physical platforms. In this thesis, we consider two specific implementations: Part I presents a detailed study of the interaction of a single atom with a light pulse. Part II examines the case of a quantum controlled-phase gate in circuit quantum electrodynamics in the ultrastrong coupling regime. They are both actively pursued by many research groups. In Part I, we first present the framework for a single two-level atom interacting with the quantized electromagnetic field. The effect of temporal and spectral properties of the pulses on atomic excitation is studied for both Fock state and coherent state pulse. The detailed analysis of atomic excited state population is provided for single photon pulse with various temporal shapes. The work is then extended to a more general case with two spatial-modes and multi-photon pulses. The difference between Fock state and coherent state pulse on atomic excitation is further investigated. We find that at few photon levels, the maximum atomic excitation probability is a monotonic function of photon number for the coherent state pulse, but not for the Fock state pulse. Furthermore, we show that the atomic dynamics can be controlled by the initial relative phase between the two counter-propagating coherent state pulses incident on the atom, which is not the case with two Fock state pulses. The theoretical prediction is then compared with an experiment, where a single trapped 87Rb atom interacts with coherent state pulses engineered in temporal shape of rising exponential and rectangular form. Next, we propose a quantum memory setup based on a single two-level atom in a half cavity with a moving mirror. The efficiency of the quantum storage process is studied analytically and