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Proceedings of SPIE, the International Society for Optical Engineering/Proceedings of SPIE

Self-induced coherence and conductivity of glow discharge

L. Petrov, Dimitar G. Slavov, Vladimir R. Arsov, А. П. Горбенко, Vasilka Steflekova, Vladimir A. Polischuk, Dimo Zhechev, G. Todorov

Published Mar 2, 2007• 0 citations
Publisher

Abstract

Comparative studies of MO resonances and MG responses with and without resonant laser irradiation were carried out to establish the interconnection of the effects and the influence of the self-alignment destruction on the MO signal in positive column discharge. These studies aim to clarify the possible formation mechanisms of the neon 1 si (2p53s) states coherences and to examine the possibility to use the galvanic resonances for estimation of the relaxation constants of the neon 1 s5 state.

DOI
10.1117/12.726890

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Physical Review•Aug 30, 1965•44 citations
Comparative studies of MO resonances and MG responses with and without resonant laser irradiation were carried out to establish the interconnection of the effects and the influence of the self-alignment destruction on the MO signal in positive column discharge. These studies aim to clarify the possible formation mechanisms of the neon 1 si (2p53s) states coherences and to examine the possibility to use the galvanic resonances for estimation of the relaxation constants of the neon 1 s5 state.
Comparative studies of magneto-optical (MO) resonances and magneto-galvanic (MG) responses with and without resonant laser irradiation are earned out to establish the interconnection of the effects and the influence of the selfalignment destruction on the MO signal in positive column discharge. These studies aim to clarify the possible formation mechanisms of the neon Is, (2p 53s) states coherences and to examine the possibility to use the galvanic resonances for estimation of the relaxation constants of the neon lr state.
The degenerate Zeeman sublevels were found to contribute to the ionization in a gas discharge in accordance with their coherent state. The voltage across the discharge was monitored while the same ensemble of excited atoms was alternately self-aligned ↔ nonaligned or oriented ↔ aligned. In the latter case, the coherence was optically induced; the corresponding opto-galvanic signals, i.e. amplitude- and time-resolved ones, were compared. Each state of the ensemble of degenerate Zeeman sublevels, i.e. (self-) aligned, oriented or disordered was characterized by its own rate of ionization. Various hollow cathode discharge (HCD) media were studied, namely, Ne/As, Ne/Cu, Ne/Ni, Ne/Cd, Ne/Li and Ne/Si in the corresponding commercial HCD spectral lamps.
In a positive column of a glow discharge, a linearly polarized laser pulse produces aligned neon atoms in the 2p 2 (Paschen notation) level, and the subsequent fluorescence is observed with its polarized components resolved. The relaxation rate of the alignment, or the disalignment rate, is thus determined. The populations of the 1s 2 – 1s 5 levels are found to be strongly dependent on the discharge current, and so are the degrees of radiation re-absorption of the transition lines from 2p 2 to these levels. A Monte Carlo simulation is performed by which the disalignment rate by radiation re-absorption for these transitions is determined, where the isotope splitting of the transition lines is taken into account. This rate is subtracted from the observed disalignment rate, resulting in the rate being independent of the degree of radiation re-absorption. Thus, disalignment due to atom collisions and that due to radiation re-absorption are separated. For the latter disalignment the disalignment rate deduced by the simulation, treating the four transitions simultaneously, is found to be virtually equal to the sum of the disalignment rates for each of the transitions. The approximate expression for the disalignment rate given by D’Yakonov and Perel’ (1965 Sov. Phys.–JETP 20 997) is quantified, so that it can be applied to estimating the disalignment rate of an upper level having several transition lines with finite optical thickness.
Alignment cascade phenomena have been studied in the neon 2p levels (Paschen notation) Hanle effect and double resonance techniques in a mild discharge. The levels are aligned directly by an optical excitation mechanism. Most 2p levels show evidence of alignment cascade from the 2s 4 , 3s 1 or 3d levels below 0.1 Torr; addition of argon impurities greatly enhances the cascade signal relative to the direct alignment signal. Data used previously in pressure broadening studies are shown to be free of cascade errors and are used to establish upper limits for the 2p level life times. A correction for coherence narrowing is estimated; this gives natural life times systematically less than those obtained by methods in which cascade effects are not carefully eliminated. In common with other Hanle effect measurements for these levels the values are marginally smaller than the threshold life times of Bennett and Kindlmann (1966).
The interaction of an intense optical-maser field with excited atoms in a gas discharge leads to a considerable change in the population of those levels which are resonant at the maser frequency. This will cause a change in the population of other levels that are connected to the maser levels through collision-induced nonradiative as well as radiative transitions. Using the 1.15-\ensuremath{\mu} optical maser, these effects have been studied in detail for the 2s2s2s levels of neon where the changes are completely due to collisions. By analyzing the intensity changes in spontaneous emission originating from a gas-discharge cell placed within the maser resonator, we have observed the approach to a partial thermalization of two closely spaced levels. In this way we have been able to obtain the atomic-collision cross section for excitation transfer between the 2s22{s}_{2}2s2​ and 2s32{s}_{3}2s3​ levels. In pure neon this has been found to be ${\ensuremath{\sigma}}_{23}=(2.3\ifmmode\pm\else\textpm\fi{}0.3)\ifmmode\times\else\texttimes\fi{}{10}^{\ensuremath{-}16}$ cm2{\mathrm{cm}}^{2}cm2. For a helium-neon mixture the measured cross section is ${\ensuremath{\sigma}}_{23}=(1.8\ifmmode\pm\else\textpm\fi{}0.3)\ifmmode\times\else\texttimes\fi{}{10}^{\ensuremath{-}16}$ cm2{\mathrm{cm}}^{2}cm2. The experimental method used to determine these cross sections eliminates the uncertainties caused by the effects of electron-atom collisions and radiative cascade. These techniques also yield the ratio of the Einstein coefficients for the transitions $2{s}_{2}\ensuremath{\rightarrow}2{p}_{10}$ and $2{s}_{3}\ensuremath{\rightarrow}2{p}_{10}$. The measured ratio is $\frac{{A}_{2}}{{A}_{3}}=3.0\ifmmode\pm\else\textpm\fi{}0.4$.