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Optics and Spectroscopy

Superradiant decay of localized excitations in a linear atomic chain

E. A. Gavrilenko, А. И. Зайцев

Published Mar 1, 2009• 0 citations
Publisher

Abstract

The superradiant decay of localized excitations in a linear chain of two-level atoms has been investigated. It is shown that the excitation energy is not completely emitted in the cooperative stage of the process. The residual excitation forms waves propagating from the regions of initial localization to the chain edges.
DOI
10.1134/s0030400x09030035

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We introduce a straightforward quantum-electrodynamic approach to the problem of superradiant spontaneous emission from a system of two-level atoms, and also discuss two classical superradiant systems. The same physical concepts underlie our treatment of both the quantum and classical cases. Explicit expressions are found which describe the time evolution and directional character of the radiated power. Our approach applies to an arbitrary number of atoms which are confined to a region with linear dimensions which may be large compared with the mean wavelength of the emitted radiation. The radiative decay half-life of a large many-atom system is found to be much shorter than the natural lifetime of a single atom, but not as short as the half-life of a small atomic system with the same number of atoms. The far-field radiation pattern appropriate to the case of a circular cylinder of emitters which have been excited by a plane-wave pulse is considered in detail. Polar plots are presented of the radiation patterns produced when the atoms are excited by a plane-wave pulse. Exciting pulses traveling in directions both parallel and at an angle of 10\ifmmode^\circ\else\textdegree\fi{} to the axis of the cylinder are considered. A discussion and generalization of Dicke's "coherence-brightening" criterion is given.
Dicke's superradiance from a gas system of atoms and molecules was described in terms of two-level atoms, i.e., as an assembly of half-spin operators. In this system the magnitude of the total spin, which is called a cooperation number, is conserved at the maximum for the whole radiative process. We will answer in this paper how this superradiance is modified in the crystal in which an excitation can propagate from atom to atom through dipolar interactions. As a prototype of a crystal, we choose a linear chain of two-level atoms. The superradiance master equation of this system can be solved in terms of the exact solution of Lieb, Shultz, and Mattis for the spin system. The first effect is that the emitted frequency shows opposite shifts red and blue, respectively, for the first and second halves of the superradiance pulse, or vice versa, depending upon the sign of the transfer-matrix element of the excitation. The second effect is the appearance of a slow component in the emission tail, which originates from mixture of the states with smaller cooperation numbers or smaller oscillator strength under the transfer of the excitations. These results are demonstrated for a mesoscopic system of linear chains.
We discuss the cooperative decay of initial atomic excitation for a pencil-shaped active volume filled with two-level atoms. As long as the length of the sample is much smaller than a certain maximal cooperation length, the atom-field interaction producing the superradiant pulse can be treated in terms of the simplest possible laser model (single mode). The basic laser master equation turns out to be exactly solvable if specified for the superradiance limit which is characterized by two conditions: (i) The photons escape from the low-QQQ cavity so fast that they cannot feed themselves back into atomic excitation to any appreciable amount (this no-feedback condition is equivalent to the above-mentioned requirement for the length of the sample). (ii) The incoherent atomic decay due to natural relaxation is so slow that the individual atomic dipoles do not dephase before engaging themselves cooperatively in the interaction with the electromagnetic field. The present paper presents the derivation and general discussion of the equations describing the statistical properties of atoms and field in a superradiant pulse. Analytical and numerical solutions will be presented in a subsequent paper.
We describe collective spontaneous emission of NNN two-level atoms placed within a photonic band-gap material. When the atomic resonance frequency lies at the band edge, superradiant emission remains localized in the vicinity of the atoms. This leads to a steady state with spontaneously broken symmetry in which the atomic system acquires a macroscopic polarization. The superradiant decay rate is proportional to N2/3{N}^{2/3}N2/3 and N2{N}^{2}N2 for isotropic and anisotropic 3D band gaps, respectively. The corresponding peak intensity of superradiance is proportional to N5/3{N}^{5/3}N5/3 and N3{N}^{3}N3, respectively.
The radiation pattern of light scattered from a chain of atoms having J=0J=0J=0 ground states and J=1J=1J=1 excited states is calculated in the weak driving field approximation. It is shown that, in general, for arbitrary orientation of the driving field to the chain axis, it is not possible to treat the atoms in a two-level approximation owing to cooperative effects. In the limit of large detuning, however, all cooperative decay effects can be neglected in calculating the scattered spectrum. Nevertheless, even in this limit, in order to ensure conservation of energy, it is still necessary to include cooperative decay when calculating the energy lost by the driving field. For arbitrary detunings, conservation of energy can be expressed in the form of a generalized optical theorem.