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Physical Review A

Positron annihilation in the positron-helium ion e+[He(2S3)]

Alexei M. Frolov

Published Mar 21, 2005• 15 citations
Publisher

Abstract

The $({e}^{\ensuremath{-}},{e}^{+})$-pair annihilation is considered in the positron-helium ${e}^{+}[\mathrm{He}(2\phantom{\rule{0.2em}{0ex}}^{3}S)]$ four-body ion, in which the positron forms a bound state with the helium atom in its lowest triplet state [i.e., in the $2\phantom{\rule{0.2em}{0ex}}^{3}S\phantom{\rule{0.3em}{0ex}}(L=0)$ state]. A number of bound-state properties of this system have been determined for the ${e}^{+}[\mathrm{He}(2\phantom{\rule{0.2em}{0ex}}^{3}S)]$ ions, where the $^{\ensuremath{\infty}}\mathrm{He}$, $^{4}\mathrm{He}$, and $^{3}\mathrm{He}$ helium nuclei are considered. Some applications related to the positron annihilation in the ${e}^{+}[\mathrm{He}(2\phantom{\rule{0.2em}{0ex}}^{3}S)]$ ion are also discussed.

DOI
10.1103/physreva.71.032506

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The (e\ensuremath−,e+)({e}^{\ensuremath{-}},{e}^{+})(e\ensuremath−,e+)-pair annihilation is considered in the positron-helium e+[He(23S)]{e}^{+}[\mathrm{He}(2\phantom{\rule{0.2em}{0ex}}^{3}S)]e+[He(23S)] four-body ion, in which the positron forms a bound state with the helium atom in its lowest triplet state [i.e., in the 23S(L=0)2\phantom{\rule{0.2em}{0ex}}^{3}S\phantom{\rule{0.3em}{0ex}}(L=0)23S(L=0) state]. A number of bound-state properties of this system have been determined for the e+[He(23S)]{e}^{+}[\mathrm{He}(2\phantom{\rule{0.2em}{0ex}}^{3}S)]e+[He(23S)] ions, where the \ensuremath∞He^{\ensuremath{\infty}}\mathrm{He}\ensuremath∞He, 4He^{4}\mathrm{He}4He, and 3He^{3}\mathrm{He}3He helium nuclei are considered. Some applications related to the positron annihilation in the e+[He(23S)]{e}^{+}[\mathrm{He}(2\phantom{\rule{0.2em}{0ex}}^{3}S)]e+[He(23S)] ion are also discussed.
Bound state properties, positron annihilation and hyperfine structure splittings in the four-body positron-helium e+[3e^{+} [^{3}e+[3He(23Se2^{3}S_e23Se​)] and e+[4e^{+} [^{4}e+[4He(23Se2^{3}S_e23Se​)] ions
Hyperfine structure splitting of the positron-helium ions e+[e^{+}[e+[He(23S)](2^3S)](23S)]
The hyperfine structure splittings are determined for the lowest bound state in the positron-helium ion e+[3e^{+}[^3e+[3He(23S)](2^3S)](23S)] and e+[4e^{+}[^4e+[4He(23S)](2^3S)](23S)]. In particular, we have fond that for the e+[3e^{+}[{}^3e+[3He(23S)](2^3S)](23S)] ion one can observe the three following hyperfine structure splittinings: 5824.3986 MHzMHzMHz, 76466.5308 MHzMHzMHz and 5824.4019 MHzMHzMHz. In the e+[4e^{+}[{}^4e+[4He(23S)](2^3S)](23S)] ion only one hyperfine structure splitting 82963.0427 MHzMHzMHz can be observed. All these values can be measured in modern experiments.
Electron-positron annihilation rates calculated directly from the electron and positron densities are known to underestimate the true annihilation rate. A correction factor, known as the enhancement factor, allows for the local increase of the electron density around the positron caused by the attractive electron-positron interaction. Enhancement factors are given for positrons annihilating with the 1s1s1s electron in H, He+{\mathrm{He}}^{+}He+, He, Li2+{\mathrm{Li}}^{2+}Li2+, and Li+{\mathrm{Li}}^{+}Li+. The enhancement factor for a free positron annihilating with He+{\mathrm{He}}^{+}He+ and He is found to be close to that of ortho-positronium (i.e., Ps in its triplet state) annihilating with these atoms. The enhancement factor for Ps-He scattering is used in conjunction with the known annihilation rate for pickoff annihilation to derive a scattering length of 1.47a01.47{a}_{0}1.47a0​ for Ps-He scattering. Further, enhancement factors for e+{e}^{+}e+-Ne and e+{e}^{+}e+-Ar annihilation are used in conjunction with the pickoff annihilation rate to estimate scattering lengths of 1.46a01.46{a}_{0}1.46a0​ for Ps-Ne scattering and 1.75a01.75{a}_{0}1.75a0​ for Ps-Ar scattering.
Various geometrical and energetical (bound-state) properties of the positronium negative ion $({\mathrm{Ps}}^{\ensuremath{-}}$ or ${e}^{\ensuremath{-}}{e}^{+}{e}^{\ensuremath{-}})$ are determined by using highly accurate variational wave functions. These wave functions have been constructed by applying the advanced two-stage strategy proposed by Frolov [Phys. Rev. A 57, 2436 (1998)]. The determined total energy of the ground state $E=\ensuremath{-}0.2620050702329757\mathrm{a}.\mathrm{u}.$ is the lowest and most accurate value obtained for this system to date (the corresponding binding energy equals $\ensuremath{-}0.326674721317821\mathrm{eV}).$ The computation of the second-order relativistic corrections $(\ensuremath{\simeq}{\ensuremath{\alpha}}^{2})$ to the total energy is discussed also. The general form of the Breit-Pauli Hamiltonian in the relative coordinates for the ${\mathrm{Ps}}^{\ensuremath{-}}$ ion is presented.