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Journal of the Optical Society of America B

Induced-frequency modulation in a nonzero-relaxation-time medium

Jamal T. Manassah

Published Jun 1, 1989• 2 citations
Publisher

Abstract

Induced-frequency modulation in the presence of pump–probe walk-off in a nonzero-relaxation-time nonlinear medium is investigated. The probe shape, phase, and frequency shift that are due to both effects are calculated in the weak-probe limit.
DOI
10.1364/josab.6.001253

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I show that a probe pulse that is copropagating in an enhanced induced-phase-modulation nonlinear two-dimensional medium in the presence of a pump may be transformed into an induced superspike in time and space. The conditions of this induced collapse are that the ratio of the probe and pump initial transverse dimension to the duration be equal to 1/[beta((2))k(probe)]((1/2)), that their group velocities be equal, that the pump energy be larger than a waveguiding critical value, and that the probe central frequency be in the group-velocity dispersion anomalous region.
The analytic solutions of equations, which describe the time behavior of density-matrix elements of a two-level medium driven by weak-probe tunable and strong fields, namely, scrE(t)=E(t)cos[\ensuremath{\omega}t+\ensuremath{\varphi}(t)]+\ensuremath{\varepsilon} cos[(\ensuremath{\omega}+\ensuremath{\delta})t], the amplitude E(t) and phase \ensuremath{\varphi}(t) of which are any arbitrary functions of time, are obtained. We obtain explicit expressions of the medium polarizability in two cases of the strong-field parameters modulation: first, E(t)=E0{\mathit{E}}_{0}E0​cos(\ensuremath{\xi} cos\ensuremath{\Omega}t), where E0{\mathit{E}}_{0}E0​, \ensuremath{\Omega}, and \ensuremath{\xi} are constants, and \ensuremath{\varphi}=0; and second, both the amplitude E(t) and the phase \ensuremath{\varphi}(t) are periodic functions of time, and E(t)=C\ensuremath{\varphi}\ifmmode \dot{}\else \.{}\fi{}, where C is an arbitrary constant. These cases of modulation are generalizations of cases that were considered earlier. The first case of modulation causes a shift of the well-known Rabi resonances in the weak-probe absorption and dispersion spectra by the factor J0{\mathit{J}}_{0}J0​(\ensuremath{\xi}) (J0{\mathit{J}}_{0}J0​ is the zero-order Bessel function of the first kind) in comparison with a nonmodulated exciting field. In the second case of the modulation, the Rabi resonances are present but the effect of such a modulation results in an attenuation of the amplitude-modulation effect. The values of the parameters E0{\mathit{E}}_{0}E0​, \ensuremath{\Omega}, C, and \ensuremath{\xi} and the frequency ranges in which the weak-probe gain, caused by resonant Rayleigh scattering and by three-photon scattering, takes place are determined for these two cases of the modulation.
We discuss experimental observations of an induced phase shift of the rf signal produced in frequency-modulated saturated-absorption measurements under the conditions of large probe-beam intensities. This phase shift can be understood in terms of the phase difference between the phase modulation of the optical driving field and the steady-state macroscopic polarization of the medium. We also present theoretically calculated spectra that are based on the optical Bloch equations and that are in excellent agreement with the experimental results.