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Physica B Condensed Matter

Spin squeezed states in two-dimensional antiferromagnet with a single impurity

Feng Peng

Published Mar 12, 2005• 2 citations
Publisher
DOI
10.1016/j.physb.2005.01.483

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Ground States of Quantum Antiferromagnets in Two Dimensions

Subir Sachdev A, Kwon Park

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We describe the spin distribution in the vicinity of a nonmagnetic impurity in a two-dimensional antiferromagnet undergoing a transition from a magnetically ordered N\'eel state to a paramagnet with a spin gap. The quantum critical ground state in a finite system has total spin S=1∕2S=1∕2S=1∕2 (if the system without the impurity had an even number of S=1∕2S=1∕2S=1∕2 spins), and recent numerical studies in a double layer antiferromagnet [K. H. H\"oglund et al., Phys. Rev. Lett. 98, 087203 (2007)] have shown that the spin has a universal spatial form delocalized across the entire sample. We present the field theory describing the uniform and staggered magnetizations in this spin texture for two classes of antiferromagnets: (i) the transition from a N\'eel state to a paramagnet with local spin singlets, in models with an even number of S=1∕2S=1∕2S=1∕2 spins per unit cell, which are described by a O(3) Landau-Ginzburg-Wilson field theory; and (ii) the transition from a N\'eel state to a valence bond solid, in antiferromagnets with a single S=1∕2S=1∕2S=1∕2 spin per unit cell, which are described by a ``deconfined'' field theory of spinons.
Based on quantum Monte Carlo simulations, we study the local-order-parameter modulations induced by a magnetic impurity that couples to a single moment of a two-dimensional quantum antiferromagnet. A strong antiferromagnetic coupling of the impurity spin reduces the antiferromagnetic order in the host beyond the next-nearest-neighbor sites of the impurity spin, whereas on the next-nearest neighbors the order increases, similar as for an embedded vacancy. We show that for weak and intermediate couplings to the impurity spin, the local antiferromagnetic order is enhanced throughout the host magnet. We compare our numerical findings to analytical results from a recent perturbative approach based on spin-wave theory.
We consider a two-dimensional Heisenberg antiferromagnet on a square lattice with weakly coupled impurities, i.e., additional spins interacting with the host magnet by a small dimensionless coupling constant g⪡1g⪡1g⪡1. Using linear spin-wave theory, we find that the magnetization disturbance at distance rrr from a single impurity behaves as $\ensuremath{\delta}{S}^{z}\ensuremath{\propto}g∕r$ for 1⪡r⪡1∕g1⪡r⪡1∕g1⪡r⪡1∕g and as $\ensuremath{\delta}{S}^{z}\ensuremath{\propto}1∕(g{r}^{3})$ for r⪢1∕gr⪢1∕gr⪢1∕g. Surprisingly the magnetization disturbance is inversely proportional to the coupling constant. The interaction between two impurities separated by a distance rrr is $\ensuremath{\delta}ϵ\ensuremath{\propto}{g}^{2}∕r$ for 1⪡r⪡1∕g1⪡r⪡1∕g1⪡r⪡1∕g and $\ensuremath{\delta}ϵ\ensuremath{\propto}1∕{r}^{3}$ for r⪢1∕gr⪢1∕gr⪢1∕g. For large distances, the interaction is therefore universal and independent of the coupling constant. We have also found that the frequency of Rabi oscillations between two impurities is logarithmically enhanced compared to the decay width ${\ensuremath{\omega}}_{\mathrm{Rabi}}\ensuremath{\propto}{g}^{2}\phantom{\rule{0.2em}{0ex}}\mathrm{ln}(1∕\mathit{gr})$ at 1⪡r⪡1∕g1⪡r⪡1∕g1⪡r⪡1∕g. This leads to a logarithmic enhancement for NMR and EPR line broadening. All these astonishing results are due to the gapless spectrum of magnetic excitations in the quantum antiferromagnet.