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Physics Letters A

Effect of Doppler broadening on resonance fluorescence

Dezhong Wang, Jin-Yue Gao

Published Mar 1, 1997• 3 citations
Publisher
DOI
10.1016/s0375-9601(97)00085-6

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In a vapor cell, [Formula: see text] is the average velocity of the moving atoms. When [Formula: see text], the in-homogeneous broadening of the atomic spectral lines is important when taking into account thermal Doppler broadening. We also discover that the narrowing mechanism for inter-atomic with different components has more influence on the Doppler line-shape. Thus, the spectral line broadening of two-level and three-level multi-mer [Formula: see text] atom is not only influenced by the in-homogeneous Doppler broadening, but also affected by the Dicke narrowing effect. The fluorescence spectrum affords a good possibility for a detailed study of Dicke narrowing effect and thermal Doppler broadening effect. We analyze the influence of multi-mer [Formula: see text] atomic system component on resonance fluorescence spectrum (RFS). Based on the quantum regression theorem, we develop a method and derive a general analytical expression for the two-dimensional (2D) fluorescence correlation spectrum of three-level [Formula: see text] atomic system.
Calculations are presented for the degrees of first- and second-order coherence and the spectral distribution of the light emitted in resonance fluorescence by a two-level atom driven by monochromatic incident light. The theory includes the effects of both homogeneous and inhomogeneous broadening, but is restricted to ranges of the parameters for which analytic solutions can be obtained. There is a further restriction to forward scattering in the case where the inhomogeneous broadening is caused by the Doppler effect. The results show marked differences between the effects of the homogeneous and inhomogeneous broadening mechanisms.