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Physical Review A

Suppression of spontaneous emission and superradiance over macroscopic distances in media with negative refraction

Jürgen Kästel, Michael Fleischhauer

Published Jan 31, 2005• 75 citations
Publisher

Abstract

The possibility of negative optical path length in left-handed media (LHM) is shown to lead to complete suppression of spontaneous emission of an atom in front of a mirror with a layer of LHM. For the same reason two atoms put at the foci of a perfect lens formed by a parallel LHM slab [J. B. Pendry, Phys. Rev. Lett. 85, 3966 (2000)] exhibit perfect subradiance and superradiance. It is shown that these effects occur over distances that can be orders of magnitude larger than the transition wavelength and are only limited by the propagation length within the free-space decay time of the atoms. Single- and two-atom decay rates are calculated from the Greens function of the electric field in the presence of a LHM and limitations as well as potential applications are discussed.

DOI
10.1103/physreva.71.011804

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Physical Review A•Apr 14, 2009•33 citations
The possibility of negative optical path length in left-handed media (LHM) is shown to lead to complete suppression of spontaneous emission of an atom in front of a mirror with a layer of LHM. For the same reason two atoms put at the foci of a perfect lens formed by a parallel LHM slab [J. B. Pendry, Phys. Rev. Lett. 85, 3966 (2000)] exhibit perfect subradiance and superradiance. It is shown that these effects occur over distances that can be orders of magnitude larger than the transition wavelength and are only limited by the propagation length within the free-space decay time of the atoms. Single- and two-atom decay rates are calculated from the Greens function of the electric field in the presence of a LHM and limitations as well as potential applications are discussed.
We consider the interaction of atoms with the quantized electromagnetic field in the presence of materials with negative index of refraction. Spontaneous emission of an atom embedded in a negative index material is discussed. It is shown furthermore that the possibility of a vanishing optical path length between two spatially separated points provided by these materials can lead to complete suppression of spontaneous emission of an atom in front of a perfect mirror even if the distance between atom and mirror is large compared to the transition wavelength. Two atoms put in the focal points of a lens formed by a parallel slab of ideal negative index material are shown to exhibit perfect sub- and superradiance. The maximum length scale in both cases is limited only by the propagation distance within the free-space radiative decay time. Limitations of the predicted effects arising from absorption, finite transversal extension and dispersion of the material are analyzed.
Two atoms put at the foci of a perfect lens [J.B. Pendry, Phys. Ref. Lett. 85, 3966 (2000)] are shown to exhibit perfect sub- and super-radiance even over macroscopic distances limited only by the propagation length in the free-space decay time. If the left-handed material forming the perfect lens has nearly constant negative refraction and vanishing absorption over a spectral range larger than the natural linewidth, the imaginary part of the retarded Greens-function between the two focal points is identical to the one at the same spatial position and the atoms undergo a Markovian dynamics. Collective decay rates and level shifts are calculated from the Greens-function of the Veselago-Pendry lens and limitation as well as potential applications are discussed.
The spontaneous decay process of a two-level atom embedded in a one-dimensional structure containing left-handed material (LHM) is investigated. We first consider the case of the atom being in front of a LHM layer mounted on a mirror, where it has been claimed that the atomic decay would be inhibited completely. Here we introduce dispersion and dissipation in the LHM, and find that there are two factors that weaken the inhibition of spontaneous decay. One is atomic nonradiative decay at shorter distances and the other is the instantaneous radiative decay process for larger distances. Then we discuss the decay process of an atom embedded in a one-dimensional photonic crystal composed of alternate LHM and ordinary material [right-handed material (RHM)] layers (LHM-RHM PC). Because of two special characteristics of the LHM, phase compensation and the fact that a frequency with negative index is usual near the material resonance frequency, both the radiative and nonradiative decay processes in the LHM-RHM PC are much different from those in a RHM PC. Under appropriate condition, the population evolution of atoms in a LHM-RHM PC displays oscillatory behavior.
We present a quantization scheme for the electromagnetic field interacting with atomic systems in the presence of dispersing and absorbing magnetodielectric media, including left-handed material having negative real part of the refractive index. The theory is applied to the spontaneous decay of a two-level atom at the center of a spherical free-space cavity surrounded by magnetodielectric matter of overlapping band-gap zones. Results for both big and small cavities are presented, and the problem of local-field corrections within the real-cavity model is addressed.
We investigate the spontaneous emission of a two-level atom in one dimensional photonic crystals composed of left-hand material (LHM) and right-hand material (RHM). A complete set of mode functions is constructed for the quantization of the radiation field. It is found that the mode functions for the frequency with in the band gap decreases exponentially from the surface to the interior of the photonic crystal which results in a much weaker field than the vacuum in the free space. The depression of the field leads to weak interaction with the atom, which leads to the suppressed spontaneous emission. Due to the strong reflection, the field in the LHM-RHM structure is much weaker than that in the RHM-RHM structure, thus the spontaneous emission is more strongly suppressed.
Spontaneous decay of a two-level atom near the left-handed material (LHM) slab is investigated. The contributions of the guided modes and the surface-plasmon polariton (SPP) modes supported by the LHM slab to the spontaneous decay are studied at length. We find that the atomic decay near a LHM slab is much different from that near a dielectric slab or metal slab. The first---the dielectric slab with arbitrary thickness---supports at least two guided modes (one for TE polarized and one for TM polarized), but LHM slab may support none of the guided mode for certain thickness. The second---the atom near the LHM slab---may decay through both TE- and TM-polarized SPP, but the atom near the metal slab can decay only through TM-polarized SPP. The third, when the LHM slab supports only TE-polarized SPP modes, the atom near such slab cannot couple to the SPP mode when its dipole moment is perpendicular to the interface. Even if LHM contains weak loss, above analysis is also valid, and the decay rate directly related to material's losses (defined by the decay through dissipation here) can be distinguished from the total decay rate. Most interesting, we find that the decay through SPP will be larger than the decay through dissipation when the atom is placed at an appropriate position. Our results will give constructive reference to the design and fabrication of the quantum device made of LHM.