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arXiv:quant-ph/0306028 · Physical Review A

Electromagnetic-field quantization and spontaneous decay in left-handed media

Ho Trung Dung, Stefan Yoshi Buhmann, L. Knöll, Dirk‐Gunnar Welsch, Stefan Scheel, Jürgen Kästel

Published Oct 13, 2003• 178 citations
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Abstract

We present a quantization scheme for the electromagnetic field interacting with atomic systems in the presence of dispersing and absorbing magnetodielectric media, including left-handed material having negative real part of the refractive index. The theory is applied to the spontaneous decay of a two-level atom at the center of a spherical free-space cavity surrounded by magnetodielectric matter of overlapping band-gap zones. Results for both big and small cavities are presented, and the problem of local-field corrections within the real-cavity model is addressed.

DOI
10.1103/physreva.68.043816

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We present a quantization scheme for the electromagnetic field interacting with atomic systems in the presence of dispersing and absorbing magnetodielectric media, including left-handed material having negative real part of the refractive index. The theory is applied to the spontaneous decay of a two-level atom at the center of a spherical free-space cavity surrounded by magnetodielectric matter of overlapping band-gap zones. Results for both big and small cavities are presented, and the problem of local-field corrections within the real-cavity model is addressed.
After giving a summary of the basic-theoretical concept of quantization of the electromagnetic field in the presence of dispersing and absorbing (macroscopic) bodies, their effect on spontaneous decay of an excited atom is studied. Various configurations such as bulk material, planar half space media, spherical cavities, and microspheres are considered. In particular, the influence of material absorption on the local-field correction, the decay rate, the line shift, and the emission pattern are examined. Further, the interplay between radiative losses and losses due to material absorption is analyzed. Finally, the possibility of generating entangled states of two atoms coupled by a microsphere-assisted field is discussed.
Starting from the quantized version of Maxwell's equations for the electromagnetic field in an arbitrary linear Kramers-Kronig dielectric, the Heisenberg equations of motion for a two-level atom resonantly coupled to the radiation field in the presence of dispersive and absorbing dielectric bodies are derived. The theory is applied to the problem of spontaneous decay of excited atoms in absorbing media. The decay rate is calculated for the (Glauber-Lewenstein) real-cavity model, and a comparison with the recently studied (Clausius-Mosotti) virtual-cavity model [S. Scheel, L. Kn\"oll, D.-G. Welsch, and S. M. Barnett, Phys. Rev. A 60, 1590 (1999)] is given. It is shown that owing to nonradiative decay associated with absorption, the rate of spontaneous decay sensitively depends on the cavity radius, particularly when the atomic transition frequency approaches an absorption band of the medium. Only when the effect of absorption is fully disregarded, is the familiar local-field correction factor recovered.
After giving an outline of the quantization scheme based on the microscopic Hopfield model of a dielectric bulk material, we show how the classical phenomenological Maxwell equations of the electromagnetic field in the presence of dielectric matter of given space- and frequency-dependent complex permittivity can be transferred to quantum theory. Including in the theory the interaction of the medium-assisted field with atomic systems, we present both the minimal-coupling Hamiltonian and the multipolar-coupling Hamiltonian in the Coulomb gauge. To illustrate the concept, we discuss the input--output relations of radiation and the transformation of radiation-field quantum states at absorbing four-port devices, and the spontaneous decay of an excited atom near the surface of an absorbing body and in a spherical micro-cavity with intrinsic material losses. Finally, we give an extension of the quantization scheme to other media such as amplifying media, magnetic media, and nonlinear media.
A formalism for studying spontaneous decay of an excited two-level atom in the presence of dispersing and absorbing dielectric bodies is developed. An integral equation, which is suitable for numerical solution, is derived for the atomic upper-state-probability amplitude. The emission pattern and the power spectrum of the emitted light are expressed in terms of the Green tensor of the dielectric-matter formation, including absorption and dispersion. The theory is applied to the spontaneous decay of an excited atom at the center of a three-layered spherical cavity, with the cavity wall being modeled by a band-gap dielectric of Lorentz type. Both weak and strong coupling are studied, the latter with a special emphasis on cases where the atomic transition is (i) in the normal-dispersion zone near the medium resonance, and (ii) in the anomalous-dispersion zone associated with the band gap. In a single-resonance approximation, conditions of the appearance of Rabi oscillations and closed solutions to the evolution of the atomic state population are derived, which are in good agreement with the exact numerical results.
We consider the interaction of atoms with the quantized electromagnetic field in the presence of materials with negative index of refraction. Spontaneous emission of an atom embedded in a negative index material is discussed. It is shown furthermore that the possibility of a vanishing optical path length between two spatially separated points provided by these materials can lead to complete suppression of spontaneous emission of an atom in front of a perfect mirror even if the distance between atom and mirror is large compared to the transition wavelength. Two atoms put in the focal points of a lens formed by a parallel slab of ideal negative index material are shown to exhibit perfect sub- and superradiance. The maximum length scale in both cases is limited only by the propagation distance within the free-space radiative decay time. Limitations of the predicted effects arising from absorption, finite transversal extension and dispersion of the material are analyzed.
The electromagnetic field inside a cubic cavity filled with a linear magnetodielectric medium and in the presence of external charges is quantized by modeling the magnetodielectric medium with two independent quantum fields. The electric and magnetic polarization densities of the medium are defined in terms of the ladder operators of the medium and eigenmodes of the cavity. The Maxwell and constitutive equations of the medium together with the equation of motion of the charged particles have been obtained from the Heisenberg equations using a minimal coupling scheme. The spontaneous emission of a two-level atom embedded in a magnetodielectric medium is calculated in terms of the electric and magnetic susceptibilities of the medium and the Green function of the cubic cavity, as an application of the model.