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Physical Review A

Master equations for a damped nonlinear oscillator and the validity of the Markovian approximation

Robert Alicki

Published Oct 1, 1989• 75 citations
Publisher

Abstract

The different conditions that could be imposed on a Markovian master equation for a nonlinear oscillator weakly coupled to a thermal reservoir are formulated. They concern preservation of trace and positivity of a density matrix, return to a proper equilibrium state, and the detailed balance condition. It is shown that only one of the known master equations satisfies all of these conditions. Then the validity of the Markovian approximation is reanalyzed using certain non-Markovian weak-coupling approximations, and the existence of different stages of evolution associated with different time scales of the Hamiltonian dynamics is predicted. The consequences of these facts for the description of a damped nonlinear oscillator are discussed.

DOI
10.1103/physreva.40.4077

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The different conditions that could be imposed on a Markovian master equation for a nonlinear oscillator weakly coupled to a thermal reservoir are formulated. They concern preservation of trace and positivity of a density matrix, return to a proper equilibrium state, and the detailed balance condition. It is shown that only one of the known master equations satisfies all of these conditions. Then the validity of the Markovian approximation is reanalyzed using certain non-Markovian weak-coupling approximations, and the existence of different stages of evolution associated with different time scales of the Hamiltonian dynamics is predicted. The consequences of these facts for the description of a damped nonlinear oscillator are discussed.
Markovian quantum master equations are generally thought to satisfy the following three conditions: (i) they describe the dynamics of time scales that are larger than the reservoir correlation time scale, (ii) these stationary solutions give the thermal equilibrium states with a reservoir, and (iii) they can be written in the Lindblad form. In fact, for single systems such as a single harmonic oscillator and a single two-level system, Markovian quantum master equations satisfying all these conditions can be obtained. However, for composite systems, which consist of more than one subsystem coupled with each other, such equations have not been obtained thus far. In this study, we found that we cannot use the Born–Markov approximation for obtaining quantum master equations for composite systems in the strong-coupling regime, no matter how short the reservoir correlation time is.
The quantum master equation obtained from two different thermodynamic arguments is seriously nonlinear. We argue that, for quantum systems, nonlinearity occurs naturally in the step from reversible to irreversible equations and we analyze the nature and consequences of the nonlinear contribution. The thermodynamic nonlinearity naturally leads to canonical equilibrium solutions and extends the range of validity to lower temperatures. We discuss the Markovian character of the thermodynamic quantum master equation and introduce a solution strategy based on coupled evolution equations for the eigenstates and eigenvalues of the density matrix. The general ideas are illustrated for the two-level system and for the damped harmonic oscillator. Several conceptual implications of the nonlinearity of the thermodynamic quantum master equation are pointed out, including the absence of a Heisenberg picture and the resulting difficulties with defining multitime correlations.
We study a driven two-state system interacting with a generic structured environment. We outline the derivation of the time-local microscopic non-Markovian master equation, in the limit of weak coupling between the system and the reservoir, and we derive its analytic solution for general reservoir spectra in the regime of validity of the secular approximation. We also consider the non-Markovian master equation without the secular approximation and study the effect of nonsecular terms on the system dynamics for two classes of reservoir spectra: the Ohmic and the Lorentzian reservoir. Finally, we derive the analytic conditions for complete positivity of the dynamical map, with and without the secular approximation. Interestingly, the complete positivity conditions have a transparent physical interpretation in terms of the characteristic time scales of phase diffusion and relaxation processes.
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Quantum systems coupled to environments exhibit intricate dynamics. The master equation gives a Markov approximation of the dynamics, allowing for analytic and numerical treatments. It is ubiquitous in theoretical and applied quantum sciences. The accuracy of the master equation approximation was so far proven in the regime where time must not exceed an upper bound depending on the system-environment interaction strength (weak coupling regime). Here, we show that the Markov approximation is valid for fixed coupling strength and for all times. We also construct a new approximate markovian dynamics -- a completely positive, trace preserving semigroup -- which is asymptotically in time exact, to all orders in the coupling.