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arXiv:1001.3564 · Physical Review A

Non-Markovian dynamics of a damped driven two-state system

Pinja Haikka, Sabrina Maniscalco

Published May 6, 2010• 76 citations
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Abstract

We study a driven two-state system interacting with a generic structured environment. We outline the derivation of the time-local microscopic non-Markovian master equation, in the limit of weak coupling between the system and the reservoir, and we derive its analytic solution for general reservoir spectra in the regime of validity of the secular approximation. We also consider the non-Markovian master equation without the secular approximation and study the effect of nonsecular terms on the system dynamics for two classes of reservoir spectra: the Ohmic and the Lorentzian reservoir. Finally, we derive the analytic conditions for complete positivity of the dynamical map, with and without the secular approximation. Interestingly, the complete positivity conditions have a transparent physical interpretation in terms of the characteristic time scales of phase diffusion and relaxation processes.

DOI
10.1103/physreva.81.052103

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We study a driven two-state system interacting with a generic structured environment. We outline the derivation of the time-local microscopic non-Markovian master equation, in the limit of weak coupling between the system and the reservoir, and we derive its analytic solution for general reservoir spectra in the regime of validity of the secular approximation. We also consider the non-Markovian master equation without the secular approximation and study the effect of nonsecular terms on the system dynamics for two classes of reservoir spectra: the Ohmic and the Lorentzian reservoir. Finally, we derive the analytic conditions for complete positivity of the dynamical map, with and without the secular approximation. Interestingly, the complete positivity conditions have a transparent physical interpretation in terms of the characteristic time scales of phase diffusion and relaxation processes.
By use of the measure, the backflow of information presented recently, we study the non-Markovianity of the dynamics for a two-level system interacting with a zero-temperature structured environment via amplitude-phase coupling. In the limit of weak coupling between the system and its reservoir, the time-local non-Markovian master equation for the reduced state of the system is derived. Under the secular approximation, the exact analytic solution is obtained. Numerical simulations show that the amplitude and phase dampings can produce destructive interference to the backflow of information, leading to the weaker non-Markovianity of the compound dynamics compared with the dynamics of a single amplitude or phase damping model. We also study the characteristics of the initial-state pairs that maximize the backflow of information.
The driven two-level system is a useful model to describe many quantum objects, particularly in quantum information processing. However, the exact master equation for such a system has barely been explored. Making use of the Feynman-Vernon influence functional theory, we derive an exact non-Markovian master equation for the driven two-level system and show the lost feature in the perturbative treatment for this system. The perturbative treatment leads to the time-convolutionless (TCL) and Nakajima-Zwanzig (NZ) master equations. So to this end we derive the TCL and NZ master equations for the system and compare the dynamics given by the three master equations. We find the validity condition for the TCL and NZ master equations. Based on the exact non-Markovian master equation, we analyze the regime of validity for the secular approximation in the time-convolutionless master equation and discuss the leading corrections of the nonsecular terms to the quantum dynamics. Significant effects are found in the dynamics of the driven system.
We present a systematic thermodynamic analysis of nonsecular GKLS master equations. When some energy transitions in the system are comparable with the dissipative rate, the secular approximation is not valid, and the positivity of the dynamics must be ensured via other approximations. The dynamics then presents features reminiscent from strong coupling to the environment: e.g. the equilibrium state with an environment at thermal equilibrium is not a Gibbs state of the local system Hamiltonian and the dynamics couples energy coherences and populations. Nonetheless, we build a unified, consistent thermodynamic framework for those dynamics. We focus on two approximations beyond the full secular approximation (the local and the more accurate geometric-arithmetic approximations), and then employ systematic perturbation theory on microscopic expressions for the first and second law of thermodynamics which relate irreversibility to the increase of system-environment correlations. We show that, in spite of the weak system-bath coupling, the system-bath interaction energy participates to the energy balance, and is directly linked to the Lamb-shift Hamiltonian. We compare this microscopic entropy production with the definition based on the contractivity of the reduced system dynamics (Spohn inequality). We show that, unlike for secular master equations, the two entropy production rates differ because of the presence of non-vanishing stationary coherences in the energy eigenbasis. However, in the case of a single thermal bath, the difference is purely transient, and no work can be cyclically extracted from the steady-state despite its non-Gibbs form. Finally, we illustrate our results with simple examples, clarifying and completing the thermodynamic picture of Markovian dynamics in the quantum regime.
In this paper, we investigate the dissipative dynamics of a driven two-level quantum dot weakly coupled with a structured reservoir that is characterized by a double-peaked spectral function. We discuss the time-dependent dissipation coefficients and the Bloch vector by using a time-local non-markovian master equation. It is shown that the decay rates display temporarily negative values that can be manipulated by the distance between the two peaks in the spectral function. For the strong pumping case, the nonsecular effect gives rise to the non-markovian dynamics of the Bloch vector. However, for the weak pumping case, the non-markovian dynamics show up when contributions from secular and nonsecular terms are comparable. In the long time limit, the signature of non-markovian dynamics disappears and the behavior obeys Fermi’s golden rule.
We present a method to derive an exact master equation for a bosonic system coupled to a set of other bosonic systems, which plays the role of the reservoir, under the strong-coupling regime, i.e., without resorting to either the rotating-wave or secular approximations. Working with phase-space distribution functions, we verify that the dynamics have two different behaviors. Considering that the initial state is a concentrated wave packet in phase space, we see that the center of this wave packet follows classical mechanics while its shape gets distorted. Moreover, we show that this distortion is caused by the counter-rotating terms as well as thermal fluctuations. Finally, we discuss conditions for non-Markovian dynamics.