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Journal of the Optical Society of America

Classical Coherence Formulation of Second-Harmonic Generation in the Optical Parametric Amplifier

Joel L. Zuckerman, John B. DeVelis

Published Feb 1, 1968• 1 citation
Publisher

Abstract

In this paper we extend the formulation of the propagation of higher-order coherence functions in nonlinear media to include optical parametric amplification. It is shown that, in the strictly monochromatic limit the coherence formulation leads exactly to the solutions previously reported. This is demonstrated for complete phase matching. In addition, the quasi-monochromatic case is also considered and suggests that measurements of the higher-order coherence functions can give information about the nonlinear medium.

DOI
10.1364/josa.58.000175

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In this paper we extend the formulation of the propagation of higher-order coherence functions in nonlinear media to include optical parametric amplification. It is shown that, in the strictly monochromatic limit the coherence formulation leads exactly to the solutions previously reported. This is demonstrated for complete phase matching. In addition, the quasi-monochromatic case is also considered and suggests that measurements of the higher-order coherence functions can give information about the nonlinear medium.
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In this paper we define the normalized coherence function of arbitrary order (m, n), in a manner which seems to be a natural generalization of that defined for the second-order coherence function. Both classical and quantized optical fields are considered and the results are compared. It is shown that for classical fields and also for quantized optical fields having nonnegative definite diagonal coherent state representations of the density operator, the modulus of these normalized coherence functions is bounded by the values 0 and 1. This definition differs from the one recently given by Glauber for quantized optical fields, where the normalized coherence functions may take arbitrarily large values even for fields having nonnegative definite diagonal representations of the density operator. Conditions for ``complete coherence,'' i.e., those under which the modulus of the normalized coherence function attains the limiting value 1, are discussed. Some consequences of stationarity and quasi-monochromaticity are also discussed.
Before discussing nonlinear optics with quantized fields, it is useful to have a look at what happens with classical electromagnetic fields in nonlinear dielectric media. The theory of nonlinear optics was originally developed using classical fields by Armstrong, Bloembergen, Ducuing and Pershan in 1962, stimulated by an experiment by Franken, Hill, Peters and Weinreich in which a second harmonic of a laser field was produced by shining the laser into a crystal. This classical theory is sufficient for many applications. For the most part, quantized fields were introduced later, although a quantum theory for the parametric amplifier, a nonlinear device in which three modes are coupled, was developed by Louisell, Yariv and Siegman as early as 1961. In any case, a study of the classical theory will give us an idea of some of the effects to look for when we formulate the more complicated quantum theory. What we will present here is a very short introduction to the subject. Our intent is to use the classical theory to present some of the basic concepts and methods of nonlinear optics. Further information can be found in the list of additional reading at the end of the chapter. The discussion here is based primarily on the presentations in the books by N. Bloembergen and by R. W. Boyd. Linear polarizability We wish to survey some of the effects caused by the linear polarizability of a dielectric medium. When an electric field E ( r , t ) is applied to a dielectric medium, a polarization, that is, a dipole moment per unit volume, is created in the medium.
Nonlinear interaction of light with matter is described from the quantum-statistical point of view. The cases of two-photon absorption, Raman transition, sum-frequency generation, parametric amplification, and incoherent scattering are discussed. It is shown that the nonlinear optical effects depend strongly on the statistical properties of the light fields. The rate of nonlinear absorption, generation, and amplification is higher for chaotic than for coherent, and also higher for multimode than for single-mode pump fields. Measurements of the statistics of the output fields may yield information about the statistics of the input fields and the properties of the medium.