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Physical Review A

Collision-limited lifetimes of atom traps

John E. Bjorkholm

Published Aug 1, 1988• 58 citations
Publisher

Abstract

We carry out a simple calculation of the rate at which atoms confined within an atom trap are kicked out of the trap by elastic collisions with background gas molecules. The calculated rates are in good agreement with the observed rates and are remarkably insensitive to the trap depth.
DOI
10.1103/physreva.38.1599

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Near-threshold photodissociation of Br2{\mathrm{Br}}_{2}Br2​ from a supersonic beam produces slow bromine atoms that are trapped in the magnetic-field minimum formed between two opposing permanent magnets. Here we quantify the dominant trap-loss rate due to collisions with two sources of residual gas: the background limited by the vacuum chamber base pressure and the carrier gas during the supersonic gas pulse. The loss rate due to collisions with residual Ar in the background follows pseudo-first-order kinetics and the bimolecular rate coefficient for collisional loss from the trap is determined by measurement of this rate as a function of the background Ar pressure. This rate coefficient is smaller than the total elastic collision rate coefficient, as it only samples those collisions that lead to trap loss, and is determined to be $\ensuremath{\langle}\ensuremath{\nu}\ensuremath{\sigma}\ensuremath{\rangle}=(1.12\ifmmode\pm\else\textpm\fi{}0.09)\ifmmode\times\else\texttimes\fi{}{10}^{\ensuremath{-}9}\phantom{\rule{0.28em}{0ex}}{\mathrm{cm}}^{3}\phantom{\rule{0.16em}{0ex}}{\mathrm{s}}^{\ensuremath{-}1}$. The calculated differential cross section can be used with this value to estimate a trap depth of $293\ifmmode\pm\else\textpm\fi{}24\phantom{\rule{0.28em}{0ex}}\mathrm{mK}$. Carrier-gas collisions occur only during the tail of the supersonic beam pulse. Using the differential cross section verified by the background-gas collision measurements provides an estimate of the peak molecular-beam density of $(3.0\ifmmode\pm\else\textpm\fi{}0.3)\ifmmode\times\else\texttimes\fi{}{10}^{13}\phantom{\rule{0.28em}{0ex}}{\mathrm{cm}}^{\ensuremath{-}3}$, in good agreement with the prediction of a simple supersonic expansion model. Finally, we estimate the trap-loss rate due to Majorana transitions to be negligible, owing to the relatively large trapped-atom phase-space volume.
We present measurements and calculations of the trap loss rate for laser-cooled 87Rb^{87}\text{R}\text{b}87Rb atoms confined in either a magneto-optic trap (MOT) or a magnetic quadrupole trap when exposed to a room-temperature background gas of Ar. We study the loss rate as a function of trap depth and find that copious glancing elastic collisions, which occur in the so-called quantum diffractive regime and impart very little energy to the trapped atoms, result in significant differences in the loss rate for the MOT compared to a pure magnetic trap due solely to the difference in potential depth. This finding highlights the importance of knowing the trap depth when attempting to infer the total collision cross section from measurements of trap loss rates. Moreover, this variation in trap loss rate with trap depth can be used to extract information about the differential cross section.
Grazing collisions with background gas are the major cause of trap loss and trap heating in atom traps. To first order, these effects do not depend on the trap density. In collisionally opaque trapped atom clouds, however, scattered atoms with an energy E larger than the effective trap depth Eeff,{\mathcal{E}}_{\mathrm{eff}},Eeff​, which are destined to escape from the atom cloud, will have a finite probability for a secondary collision. This results in a contribution to the heating rate that depends on the column density 〈nl〉〈\mathrm{nl}〉〈nl〉 of the trapped atoms, i.e., the product of density and characteristic size of the trap. For alkali-metal atom traps, secondary collisions are quite important due to the strong long-range interaction with like atoms. We derive a simple analytical expression for the secondary heating rate, showing a dependency proportional to 〈nl〉Eeff1/2.〈\mathrm{nl}〉 {\mathcal{E}}_{\mathrm{eff}}^{1/2}.〈nl〉Eeff1/2​. When extrapolating to a vanishing column density, only primary collisions with the background gas will contribute to the heating rate. This contribution is rather small, due to the weak long-range interaction of the usual background gas species in an ultrahigh-vacuum system---He, Ne, or Ar---with the trapped alkali-metal atoms. We conclude that the transition between trap-loss collisions and heating collisions is determined by a cutoff energy $200 \ensuremath{\mu}\mathrm{K}<~{\mathcal{E}}_{\mathrm{eff}}<~400 \ensuremath{\mu}\mathrm{K},$ much smaller than the actual trap depth E\mathcal{E}E in most magnetic traps. Atoms with an energy Eeff<E<E{\mathcal{E}}_{\mathrm{eff}}<E<\mathcal{E}Eeff​<E<E escape into the Oort cloud: a mechanism of effective traploss in the microkelvin range of trap temperatures. We present results of secondary heating rates for the alkali-metal atoms Li through Cs as a function of the effective trap depth, the column density of the trap, and the species in the background gas. The predictions of our model are in good agreement with the experimental data of Myatt for heating rates in high-density 87Rb{}^{87}\mathrm{Rb}87Rb-atom magnetic traps at JILA, including the effect of the rf shield and the composition of the background gas. It is shown that collisions with atoms from the Oort cloud also contribute to the heating rate. For 85Rb{}^{85}\mathrm{Rb}85Rb the calculated heating rate is below the experimentally observed value at JILA, supporting the idea that inelastic collisions in the trap are the major source of heating.