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Journal of Experimental and Theoretical Physics Letters

Resonance fluorescence in an atom + dielectric microsphere system excited by a single photon

В. В. Климов, Vladilen S Letokhov

Published Jul 1, 1998• 3 citations
Publisher

Abstract

The resonance interaction of a two-level atom with a continuum of free-space modes modified by the presence of a dielectric microsphere (modified free-space modes — MFSMs) is studied. In the case that quantized MFSMs are initially excited within the contour of one of the resonance modes of the microsphere, the spectrum of emitted photons depends strongly on the excitation method. Under optimal excitation conditions efficient excitation of the atom accompanied by the formation of a Rabi doublet in the fluorescence spectrum occur. As the excitation conditions depart from optimality, the spectrum becomes a triplet. If the departure from optimality of excitation is large, the atom remains essentially unexcited, and the fluorescence spectrum has a singlet character.

DOI
10.1134/1.567833

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Physical Review Letters•Sep 25, 1989•40 citations
The resonance interaction of a two-level atom with a continuum of free-space modes modified by the presence of a dielectric microsphere (modified free-space modes — MFSMs) is studied. In the case that quantized MFSMs are initially excited within the contour of one of the resonance modes of the microsphere, the spectrum of emitted photons depends strongly on the excitation method. Under optimal excitation conditions efficient excitation of the atom accompanied by the formation of a Rabi doublet in the fluorescence spectrum occur. As the excitation conditions depart from optimality, the spectrum becomes a triplet. If the departure from optimality of excitation is large, the atom remains essentially unexcited, and the fluorescence spectrum has a singlet character.
A strong resonant interaction of a two-level atom with a dielectric microsphere is studied on the basis of quantum electrodynamics. The initial condition considered is one in which the atom is initially excited and the resonant mode of the microsphere has been excited by a single photon. The spectrum of two emitted photons depends strongly on the method used to excite the microsphere, i.e., on the spatial distribution of the photon energy. The most characteristic feature of the two-photon fluorescence spectrum is a strong energy correlation of the emitted photons. This correlation is expressed in the fact that the energies of the emitted photons are related by the equation of an ellipse (ω+ω 2−2ω vA )2+3(ω 1−ω 2)2= 4Ω Rabi 2 . The relation between the results obtained and the predictions of the theory of dressed states is discussed.
The interaction is considered between a two-level atom and the continuum of electric field modes falling within the profile of one of the resonance modes of a dielectric microsphere (a whispering gallery mode). Subject to minimal assumptions, simple equations are obtained on first principles, which describe the spectral properties of the one-photon continuum and the relaxation processes occurring therein. If the initial state of the atom is excited, a doublet structure is formed in the emitted photon spectrum, provided that the interaction is strong enough. If it is the microsphere that is excited at the initial instant, the excited photon spectrum depends substantially on the excitation method used. When excitation is optimal, the atom is effectively excited, and a Rabi-doublet is then formed in the fluorescence spectrum. When the excitation conditions are other than optimal, the spectrum becomes of triplet character, and when the deviation from the optimal excitation conditions is strong enough, the atom practically fails to get excited, and the fluorescence spectrum is of singlet type. A considerable part of the results obtained is of a general nature and can easily be applied to other cases of strong interaction between atoms and resonators.
The strong resonance interaction of a two-level atom with the continuum of quantized electromagnetic modes falling within the contour of a resonance mode of a dielectric microsphere is considered within the framework of quantum electrodynamics. Analytical solutions are derived. As an initial condition, we consider the case when, at time t = 0, the atom is excited and the resonance modes of the microsphere contain a single-photon wavepacket. It is shown that the properties of the emitted photon pair depend crucially on space-time properties of the photon wavepacket contained in the resonator. When the mean square of the electric field of the photon wavepacket at the initial instant of time at the atom position is close to the vacuum value, the radiation of an atom is similar to a spontaneous one and the emitted photon pair has no correlations. On the contrary, if the mean square of the electric field of the photon wavepacket at the initial instant of time at the atom position is substantially greater than the vacuum value, the radiation of an atom has a stimulated nature and the emitted photon pair has very complicated strong correlations. The relationship between the results obtained and the predictions of the dressed states theory are briefly discussed. The results obtained are of a general character and can be applied to the description of the resonant interaction of an excited atom and an excited resonator of an arbitrary shape.
We consider the possible physical processes that may arise in a three-level atom when only two of its levels interact with a strong electromagnetic field and when the atomic transition frequency is nearly equal to once and twice the frequency of the laser field, respectively. There have been found pronounced cooperative effects in the spectrum of the two-level system, which is in resonance with the laser field, arising from the presence of the third level. The excitation spectra describing the transitions from the first excited state into the second excited state and from that to the ground state consist, apart from the two central peaks, of two pairs of sidebands which are induced by the laser field of the neighbouring system. Detailed expressions of the spectral functions for the physical processes of one- and two-photon resonance fluorescence have been derived and discussed in the limit of high photon densities. The excitation spectrum of the low frequency modes has been considered and discussed in detail. It is found that quantum beats in spontaneous emission may appear in the spectra of the one- and two-photon resonance fluorescence arising from the interference between the two atomic transition frequencies and the frequency of the laser field. The importance of the low frequency modes that occur in the processes in question has been pointed out.
We have studied the fluorescence spectra arising from the interaction of a three-level atom with two strong electromagnetic fields whose initially populated modes are equal to the two atomic transition frequencies, respectively. The Green's function formalism has been used to calculate the excitation spectrum of the system. An expression for the spectral function describing the excitation spectrum of the system has been derived in a closed form in the limit of high photon densities. Numerical computation of the expression for the spectral function indicates that at each transition frequency there may exist either one pair or two pairs or three pairs of sidebands, in addition to the central peak, depending upon the relative strength of the Rabi frequencies involved.
The spectrum of the resonance fluorescence light from a single two-level atom in a small, high-quality, optical cavity is calculated. The coupling between the atom and cavity is made sufficiently strong compared to the dissipation that single quantum frequency splitting (vacuum Rabi splitting) occurs. Under high excitation qualitatively new fluorescent spectra are predicted. The usual three-peaked resonance fluorescence spectrum now has sidebands whose width is given by the Jaynes-Cummings atom-cavity coupling coefficient rather than by the system dissipation.