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Physical Review Letters

Resonance fluorescence spectrum of an atom strongly coupled to a cavity

Craig M. Savage

Published Sep 25, 1989• 40 citations
Publisher

Abstract

The spectrum of the resonance fluorescence light from a single two-level atom in a small, high-quality, optical cavity is calculated. The coupling between the atom and cavity is made sufficiently strong compared to the dissipation that single quantum frequency splitting (vacuum Rabi splitting) occurs. Under high excitation qualitatively new fluorescent spectra are predicted. The usual three-peaked resonance fluorescence spectrum now has sidebands whose width is given by the Jaynes-Cummings atom-cavity coupling coefficient rather than by the system dissipation.

DOI
10.1103/physrevlett.63.1376

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The spectrum of the resonance fluorescence light from a single two-level atom in a small, high-quality, optical cavity is calculated. The coupling between the atom and cavity is made sufficiently strong compared to the dissipation that single quantum frequency splitting (vacuum Rabi splitting) occurs. Under high excitation qualitatively new fluorescent spectra are predicted. The usual three-peaked resonance fluorescence spectrum now has sidebands whose width is given by the Jaynes-Cummings atom-cavity coupling coefficient rather than by the system dissipation.
Resonance fluorescence of a driven Jaynes-Cummings system is studied theoretically when the cavity is driven by a classical field of arbitrary strength. In the regime of strong atom-cavity coupling, there occur anomalous resonance peaks at $\ifmmode\pm\else\textpm\fi{}\sqrt{2}{g}^{\ensuremath{'}},\ifmmode\pm\else\textpm\fi{}\sqrt{3}{g}^{\ensuremath{'}},$ etc., with the modified vacuum Rabi frequency ${g}^{\ensuremath{'}}.$ These new peaks and the observed shift of the vacuum Rabi splitting are to be explained in the language of the quasienergy levels induced dynamically by the strong driving field. In the presence of significant damping the spectrum reflects the photon-number distribution inside the cavity, and particularly, a bimodality of the distribution results in a unique quintuplet resonance fluorescence spectrum.
The standard theory of resonance fluorescence is a weak-coupling theory.1 If n ¯ is the mean photon number for the driving field, g is the atom field coupling constant, and γ is the Einstein A coefficient, formally the standard theory of resonance fluorescence assumes the limit n ¯ → ∞ , g/ γ → 0, with the ratio of Rabi frequency to atomic linewidth 2 n ¯ n g / γ finite. The limit g/γ → 0 allows the variation of the Rabi frequency 2 n g across the photon number distribution of the driving field to be neglected. By placing the atom inside an optical cavity the ratio g/γ can be changed. In this paper we calculate spectra for intracavity resonance fluorescence in the strong-coupling limit g/γ ≫ 1, g/κ ≫ 1, where κ is the cavity linewidth. We consider a single two-level atom interacting on resonance with a single cavity mode driven by a resonant coherent field. The cavity subtends a small solid angle at the atom, so that the spontaneous emission into free-space modes is not negligible. We calculate the spectrum of the light transmitted by the cavity (the transmitted spectrum) and the spectrum of the light radiated by the atom into free space (the fluorescent spectrum). The transmitted and fluorescent spectra show fundamental differences from the (weak-coupling) spectrum of free-space resonance fluorescence.
In this dissertation we study the interaction of a single atom with a single mode of the electromagnetic field in an optical cavity. We emphasize strong coupling conditions, where the dipole coupling strength is larger than the dissipation rates of the cavity and the atom. By exciting the coupled atom and cavity mode with an external field, the excited-state spectroscopy of the coupled system is explored. Both quantum mechanical and semiclassical calculations are performed and their results are compared. In the limit of a weak driving field, both results show a two-peak ("vacuum" Rabi) spectrum. With increased strength of the driving field, differences are observed. The quantum calculation shows a multi-peak ( two "vacuum" Rabi peaks plus additional peaks) spectrum, while the semiclassical calculation does not. These additional peaks are produced by transitions between the excited states of the Jaynes-Cummings IV Hamiltonian indicative of the quantum nature of the coupled atom-cavity-mode system.
Spectra of the atomic resonance fluorescence and of the cavity-transmitted light in a driven Jaynes-Cummings system are studied theoretically, where the cavity is driven by a classical field of arbitrary strength. In the regime of strong atom-cavity coupling, anomalous resonance peaks occur at $\ifmmode\pm\else\textpm\fi{}\sqrt{n}{g}^{\ensuremath{'}} (n=2,3,\dots{}),$ with the modified vacuum Rabi frequency ${g}^{\ensuremath{'}},$ both in the atomic fluorescence and the cavity transmission. These peaks as well as the observed shift of the vacuum Rabi splitting are explained in terms of the quasienergy levels induced dynamically by the strong driving field. For a stronger driving field, it is shown that the spectrum of the cavity transmission deviates from that of the atomic fluorescence. In the presence of significant damping, the spectrum of the cavity transmission approaches a singlet structure in the strong driving-field limit, and it is found additionally that a bimodal photon-number distribution, which results in a unique quintuplet spectrum of the atomic fluorescence, does not show up in the cavity transmission.
We have studied the fluorescence spectra arising from the interaction of a three-level atom with two strong electromagnetic fields whose initially populated modes are equal to the two atomic transition frequencies, respectively. The Green's function formalism has been used to calculate the excitation spectrum of the system. An expression for the spectral function describing the excitation spectrum of the system has been derived in a closed form in the limit of high photon densities. Numerical computation of the expression for the spectral function indicates that at each transition frequency there may exist either one pair or two pairs or three pairs of sidebands, in addition to the central peak, depending upon the relative strength of the Rabi frequencies involved.