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Digest on Nonlinear Optics: Materials, Phenomena and Devices

Novel fluorescent spectra from an atom strongly coupled to a driven cavity

Craig M. Savage

Published Jan 1, 1990• 0 citations
Publisher

Abstract

Recently there has been both theoretical [1-3] and experimental [4] interest in atoms strongly coupled to single mode optical cavities. Strong coupling means that the energy level splitting due to a single quantum of excitation is comparable to the dissipative linewidth of the system. Single quantum frequency splitting has been observed for as few as 20 atoms strongly coupled to a cavity [4].

DOI
10.1109/nlo.1990.695818

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Recently there has been both theoretical [1-3] and experimental [4] interest in atoms strongly coupled to single mode optical cavities. Strong coupling means that the energy level splitting due to a single quantum of excitation is comparable to the dissipative linewidth of the system. Single quantum frequency splitting has been observed for as few as 20 atoms strongly coupled to a cavity [4].
The spectrum of the resonance fluorescence light from a single two-level atom in a small, high-quality, optical cavity is calculated. The coupling between the atom and cavity is made sufficiently strong compared to the dissipation that single quantum frequency splitting (vacuum Rabi splitting) occurs. Under high excitation qualitatively new fluorescent spectra are predicted. The usual three-peaked resonance fluorescence spectrum now has sidebands whose width is given by the Jaynes-Cummings atom-cavity coupling coefficient rather than by the system dissipation.
There is increasing interest in the photon statistics and spectroscopic properties of the radiation from atoms confined in an optical cavity. Effects such as the cavity enhancement and inhibition of spontaneous emission, which were first observed using microwave cavities, have recently been measured at optical frequencies.1 Recent measurements of squeezing and the dynamic effects of single-quantum-level splittings also demonstrate the possibilities for quantum-statistical studies of coupled atom-cavity systems at optical frequencies.2 We study a single two-level atom confined inside an optical cavity which is driven by coherent light in resonance with both cavity and atom. For weak driving field intensities we have calculated the spectrum of the light transmitted by the cavity and fluorescence out the sides of the cavity.
In the near-concentric regime, the transverse modes of an optical cavity have small mode volumes with a beam waist on the order of the atomic cross section. This shows potential for strong interaction between single atoms and light, which is a key component in distributed quantum computing architectures [1] . Furthermore, with centimetresized near-concentric cavities, the frequency spacing of the transverse modes ranges from tens of MHz to a GHz, matching well with the hyperfine or the Zeeman level splitting of an atom [2] . This near-degeneracy in resonant frequencies close to the critical point allows to explore the physics of atomic nonlinearities with multiple photonic modes strongly coupled to different hyperfine or magnetic energy levels of a quantum emitter.
In this dissertation we study the interaction of a single atom with a single mode of the electromagnetic field in an optical cavity. We emphasize strong coupling conditions, where the dipole coupling strength is larger than the dissipation rates of the cavity and the atom. By exciting the coupled atom and cavity mode with an external field, the excited-state spectroscopy of the coupled system is explored. Both quantum mechanical and semiclassical calculations are performed and their results are compared. In the limit of a weak driving field, both results show a two-peak ("vacuum" Rabi) spectrum. With increased strength of the driving field, differences are observed. The quantum calculation shows a multi-peak ( two "vacuum" Rabi peaks plus additional peaks) spectrum, while the semiclassical calculation does not. These additional peaks are produced by transitions between the excited states of the Jaynes-Cummings IV Hamiltonian indicative of the quantum nature of the coupled atom-cavity-mode system.
For the most part, quantum statistical processes in quantum optics are investigated in a weak-coupling regime, but it has become possible recently to realize experimentally optical systems for which the internal coupling coefficient g is comparable to the external dissipative rates. Within, this context, the subject of our investigation is the quantum dynamical processes for a small collection of N two-state atoms strongly coupled to a single mode of a high-finesse optical cavity. For this system, we record input-output characteristics for steady-state operation with 3 ⪝ N ⪝ 65 intracavity atoms and observe optical bistability for N⪞15 atoms.1