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Optics Express

Effects of nonlinear phase modulation on Bragg scattering in the low-conversion regime

Lasse Mejling, Daniel S. Cargill, Colin J. McKinstrie, Karsten K. Rottwitt, Richard O. Moore

Published Nov 19, 2012• 13 citations
Publisher

Abstract

In this paper, we consider the effects of nonlinear phase modulation on frequency conversion by four-wave mixing (Bragg scattering) in the low-conversion regime. We derive the Green functions for this process using the time-domain collision method, for partial collisions, in which the four fields interact at the beginning or the end of the fiber, and complete collisions, in which the four fields interact at the midpoint of the fiber. If the Green function is separable, there is only one output Schmidt mode, which is free from temporal entanglement. We find that nonlinear phase modulation always chirps the input and output Schmidt modes and renders the Green function formally nonseparable. However, by pre-chirping the pumps, one can reduce the chirps of the Schmidt modes and enable approximate separability. Thus, even in the presence of nonlinear phase modulation, frequency conversion with arbitrary pulse reshaping is possible, as predicted previously [Opt. Express 20, 8367-8396 (2012)].

DOI
10.1364/oe.20.027454

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In this paper, we consider the effects of nonlinear phase modulation on frequency conversion by four-wave mixing (Bragg scattering) in the low-conversion regime. We derive the Green functions for this process using the time-domain collision method, for partial collisions, in which the four fields interact at the beginning or the end of the fiber, and complete collisions, in which the four fields interact at the midpoint of the fiber. If the Green function is separable, there is only one output Schmidt mode, which is free from temporal entanglement. We find that nonlinear phase modulation always chirps the input and output Schmidt modes and renders the Green function formally nonseparable. However, by pre-chirping the pumps, one can reduce the chirps of the Schmidt modes and enable approximate separability. Thus, even in the presence of nonlinear phase modulation, frequency conversion with arbitrary pulse reshaping is possible, as predicted previously [Opt. Express 20, 8367-8396 (2012)].
Recently, we solved the coupled-mode equations for Bragg scattering (BS) in the low- and high-conversion regimes, but without the effects of nonlinear phase modulation (NPM). We now present solutions and Green functions in the low-conversion regime that include NPM. We find that NPM does not change the lowest-order conversion efficiency, but prevents complete separability (freedom from temporal entanglement). This problem is overcome to some degree by pre-chirping the pumps, which mitigates the effects of NPM. We conclude that arbitrary reshaping of the output modes and nearly complete separability are still possible, even when the effects of NPM are included. Finally, the effects of using different input signals are considered, and we conclude that using the natural input modes of the system drastically increases the efficiency.
In this paper we consider frequency translation enabled by Bragg scattering, a four-wave mixing process. First we introduce the theoretical background of the Green function formalism and the Schmidt decomposition. Next the Green functions for the low-conversion regime are derived perturbatively in the frequency domain, using the methods developed for three-wave mixing, then transformed to the time domain. These results are also derived and verified using an alternative time-domain method, the results of which are more general. For the first time we include the effects of convecting pumps, a more realistic assumption, and show that separability and arbitrary reshaping is possible. This is confirmed numerically for Gaussian pumps as well as higher-order Hermite-Gaussian pumps.
This PhD thesis treats applications of nonlinear optical effects for quantum information processing. The two main applications are four-wave mixing in the form of Bragg scattering (BS) for quantum-state-preserving frequency conversion, and sum-frequency generation (SFG) in second-order nonlinear materials for heralded entanglement. BS is shown to be separable in the input and output modes in the low-conversion regime, the regime of small pump powers or short interaction times. The selective frequency conversion of a signal is found to only depend on one of the pumps, while the temporal output of the converted idler depends on the other pump. This allows for temporal-mode-multiplexing. When the effects of nonlinear phase modulation (NPM) are included, the phases of the natural input and output modes are changed, reducing the separability. These effects are to some degree mediated by pre-chirping the pumps. In the high-conversion regime without the effects of NPM, exact Green functions for BS are derived. In this limit, separability is possible for conversion efficiencies up to 60 %. However, the system still allows for selective frequency conversion as well as re-shaping of the output. One way to obtain a 100 % conversion efficiency is to use multiple stages of frequency conversion, but this setup suffers from the combined effects of NPM. This problem is circumvented by using asymmetrically pumped BS, where one pump is continuous wave. For this setup, NPM is found to only lead to linear phase shifts of the input and output modes, corresponding to shifts of the central frequencies of the fields. The trade-off is that one is only able to select which signals are converted, or change the shape of the output idler. Finally, entanglement swapping using SFG was investigated. Considering two pairs of entangled photons, the process of up-converting one photon from each pair leads to heralded entangled pairs by successful detection of the up-converted photon. It was seen that this was indeed possible in the case of anti-correlated phasematching in the up-conversion crystal. Possible ways of increasing the probability of an up-conversion event were investigated briefly.
We present a quantum-mechanical model that describes fiber-based frequency conversion by four-wave-mixing Bragg scattering in the presence of Raman interactions. In the case of continuous-wave pumps, we find closed-form expressions for the conversion efficiency and photon statistics characterized by the second-order correlation function. For pulsed pumps, we derive a highly general model based on Green functions and provide a numerical solution method using a split-step scheme. In both cases, we find that noise from spontaneous Raman scattering can pose a serious challenge to this type of frequency conversion if the pumps are less than 30 THz from the quantum fields. However, this impact can be mitigated with cross-polarized pumps and, on the anti-Stokes side, through fiber cooling.
We study quantum frequency translation and two-color photon interference enabled by the Bragg scattering four-wave mixing process in optical fiber. Using realistic model parameters, we computationally and analytically determine the Green function and Schmidt modes for cases with various pump-pulse lengths. These cases can be categorized as either "non-discriminatory" or "discriminatory" in regards to their propensity to exhibit high-efficiency translation or high-visibility two-photon interference for many different shapes of input wave packets or for only a few input wave packets, respectively. Also, for a particular case, the Schmidt mode set was found to be nearly equal to a Hermite-Gaussian function set. The methods and results also apply with little modification to frequency conversion by sum-frequency conversion in optical crystals.